Promoted cobalt metal catalysts suitable for the production of lower olefins from natural gas
Due to the surge of natural gas production, feedstocks for chemicals shift towards lighter hydrocarbons, particularly methane. The success of a Gas-to-Chemicals process via synthesis gas (CO and H ) depends on the ability of catalysts to suppress methane and carbon dioxide formation. We designed a C...
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| Published in | Nature communications Vol. 10; no. 1; p. 167 |
|---|---|
| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
England
Nature Publishing Group
11.01.2019
Nature Publishing Group UK Nature Portfolio |
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| Abstract | Due to the surge of natural gas production, feedstocks for chemicals shift towards lighter hydrocarbons, particularly methane. The success of a Gas-to-Chemicals process via synthesis gas (CO and H
) depends on the ability of catalysts to suppress methane and carbon dioxide formation. We designed a Co/Mn/Na/S catalyst, which gives rise to negligible Water-Gas-Shift activity and a hydrocarbon product spectrum deviating from the Anderson-Schulz-Flory distribution. At 240 °C and 1 bar, it shows a C
-C
olefins selectivity of 54%. At 10 bar, it displays 30% and 59% selectivities towards lower olefins and fuels, respectively. The spent catalyst consists of 10 nm Co nanoparticles with hcp Co metal phase. We propose a synergistic effect of Na plus S, which act as electronic promoters on the Co surface, thus improving selectivities towards lower olefins and fuels while largely reducing methane and carbon dioxide formation. |
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| AbstractList | The conversion of natural gas to chemicals and fuels via the Fischer-Tropsch synthesis process, depends on the ability of catalyst materials to suppress the formation of methane and carbon dioxide. Here, the authors develop a Co1Mn3-Na2S catalyst, which has a hydrocarbon product spectrum deviating from the Anderson–Schulz–Flory distribution. Due to the surge of natural gas production, feedstocks for chemicals shift towards lighter hydrocarbons, particularly methane. The success of a Gas-to-Chemicals process via synthesis gas (CO and H 2 ) depends on the ability of catalysts to suppress methane and carbon dioxide formation. We designed a Co/Mn/Na/S catalyst, which gives rise to negligible Water-Gas-Shift activity and a hydrocarbon product spectrum deviating from the Anderson–Schulz–Flory distribution. At 240 °C and 1 bar, it shows a C 2 -C 4 olefins selectivity of 54%. At 10 bar, it displays 30% and 59% selectivities towards lower olefins and fuels, respectively. The spent catalyst consists of 10 nm Co nanoparticles with hcp Co metal phase. We propose a synergistic effect of Na plus S, which act as electronic promoters on the Co surface, thus improving selectivities towards lower olefins and fuels while largely reducing methane and carbon dioxide formation. The conversion of natural gas to chemicals and fuels via the Fischer-Tropsch synthesis process, depends on the ability of catalyst materials to suppress the formation of methane and carbon dioxide. Here, the authors develop a Co 1 Mn 3 -Na 2 S catalyst, which has a hydrocarbon product spectrum deviating from the Anderson–Schulz–Flory distribution. Due to the surge of natural gas production, feedstocks for chemicals shift towards lighter hydrocarbons, particularly methane. The success of a Gas-to-Chemicals process via synthesis gas (CO and H ) depends on the ability of catalysts to suppress methane and carbon dioxide formation. We designed a Co/Mn/Na/S catalyst, which gives rise to negligible Water-Gas-Shift activity and a hydrocarbon product spectrum deviating from the Anderson-Schulz-Flory distribution. At 240 °C and 1 bar, it shows a C -C olefins selectivity of 54%. At 10 bar, it displays 30% and 59% selectivities towards lower olefins and fuels, respectively. The spent catalyst consists of 10 nm Co nanoparticles with hcp Co metal phase. We propose a synergistic effect of Na plus S, which act as electronic promoters on the Co surface, thus improving selectivities towards lower olefins and fuels while largely reducing methane and carbon dioxide formation. Abstract Due to the surge of natural gas production, feedstocks for chemicals shift towards lighter hydrocarbons, particularly methane. The success of a Gas-to-Chemicals process via synthesis gas (CO and H 2 ) depends on the ability of catalysts to suppress methane and carbon dioxide formation. We designed a Co/Mn/Na/S catalyst, which gives rise to negligible Water-Gas-Shift activity and a hydrocarbon product spectrum deviating from the Anderson–Schulz–Flory distribution. At 240 °C and 1 bar, it shows a C 2 -C 4 olefins selectivity of 54%. At 10 bar, it displays 30% and 59% selectivities towards lower olefins and fuels, respectively. The spent catalyst consists of 10 nm Co nanoparticles with hcp Co metal phase. We propose a synergistic effect of Na plus S, which act as electronic promoters on the Co surface, thus improving selectivities towards lower olefins and fuels while largely reducing methane and carbon dioxide formation. Due to the surge of natural gas production, feedstocks for chemicals shift towards lighter hydrocarbons, particularly methane. The success of a Gas-to-Chemicals process via synthesis gas (CO and H2) depends on the ability of catalysts to suppress methane and carbon dioxide formation. We designed a Co/Mn/Na/S catalyst, which gives rise to negligible Water-Gas-Shift activity and a hydrocarbon product spectrum deviating from the Anderson–Schulz–Flory distribution. At 240 °C and 1 bar, it shows a C2-C4 olefins selectivity of 54%. At 10 bar, it displays 30% and 59% selectivities towards lower olefins and fuels, respectively. The spent catalyst consists of 10 nm Co nanoparticles with hcp Co metal phase. We propose a synergistic effect of Na plus S, which act as electronic promoters on the Co surface, thus improving selectivities towards lower olefins and fuels while largely reducing methane and carbon dioxide formation.The conversion of natural gas to chemicals and fuels via the Fischer-Tropsch synthesis process, depends on the ability of catalyst materials to suppress the formation of methane and carbon dioxide. Here, the authors develop a Co1Mn3-Na2S catalyst, which has a hydrocarbon product spectrum deviating from the Anderson–Schulz–Flory distribution. |
| ArticleNumber | 167 |
| Author | van Deelen, Tom W Weckhuysen, Bert M Xie, Jingxiu Louwerse, Manuel J Paalanen, Pasi P de Jong, Krijn P |
| Author_xml | – sequence: 1 givenname: Jingxiu orcidid: 0000-0001-7383-9016 surname: Xie fullname: Xie, Jingxiu organization: Inorganic Chemistry and Catalysis, Debye Institute for Nanomaterial Science, Utrecht University, Universiteitsweg 99, 3584 CG, Utrecht, The Netherlands – sequence: 2 givenname: Pasi P surname: Paalanen fullname: Paalanen, Pasi P organization: Inorganic Chemistry and Catalysis, Debye Institute for Nanomaterial Science, Utrecht University, Universiteitsweg 99, 3584 CG, Utrecht, The Netherlands – sequence: 3 givenname: Tom W orcidid: 0000-0002-3666-4576 surname: van Deelen fullname: van Deelen, Tom W organization: Inorganic Chemistry and Catalysis, Debye Institute for Nanomaterial Science, Utrecht University, Universiteitsweg 99, 3584 CG, Utrecht, The Netherlands – sequence: 4 givenname: Bert M orcidid: 0000-0001-5245-1426 surname: Weckhuysen fullname: Weckhuysen, Bert M organization: Inorganic Chemistry and Catalysis, Debye Institute for Nanomaterial Science, Utrecht University, Universiteitsweg 99, 3584 CG, Utrecht, The Netherlands – sequence: 5 givenname: Manuel J surname: Louwerse fullname: Louwerse, Manuel J organization: Inorganic Chemistry and Catalysis, Debye Institute for Nanomaterial Science, Utrecht University, Universiteitsweg 99, 3584 CG, Utrecht, The Netherlands – sequence: 6 givenname: Krijn P surname: de Jong fullname: de Jong, Krijn P email: K.P.deJong@uu.nl organization: Inorganic Chemistry and Catalysis, Debye Institute for Nanomaterial Science, Utrecht University, Universiteitsweg 99, 3584 CG, Utrecht, The Netherlands. K.P.deJong@uu.nl |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/30635560$$D View this record in MEDLINE/PubMed |
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| Snippet | Due to the surge of natural gas production, feedstocks for chemicals shift towards lighter hydrocarbons, particularly methane. The success of a... Abstract Due to the surge of natural gas production, feedstocks for chemicals shift towards lighter hydrocarbons, particularly methane. The success of a... The conversion of natural gas to chemicals and fuels via the Fischer-Tropsch synthesis process, depends on the ability of catalyst materials to suppress the... |
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| SubjectTerms | Alkenes Carbon dioxide Carbon monoxide Catalysis Catalysts Chemicals Cobalt Fuels Gas production Hydrocarbons Metals Methane Nanoparticles Natural gas Organic chemistry Selectivity Synergistic effect Synthesis gas |
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| Title | Promoted cobalt metal catalysts suitable for the production of lower olefins from natural gas |
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