Observation of chiral phonons
Chirality is associated with the breaking of symmetry, often described as left- or right-handed behavior. Such asymmetry can be seen, for example, in the electronic responses of particular materials or the reactions between particular chemical species. Zhu et al. observed a chiral phonon mode in a m...
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| Published in | Science (American Association for the Advancement of Science) Vol. 359; no. 6375; pp. 579 - 582 |
|---|---|
| Main Authors | , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
United States
The American Association for the Advancement of Science
02.02.2018
American Association for the Advancement of Science (AAAS) |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Chirality is associated with the breaking of symmetry, often described as left- or right-handed behavior. Such asymmetry can be seen, for example, in the electronic responses of particular materials or the reactions between particular chemical species. Zhu
et al.
observed a chiral phonon mode in a monolayer of the transition metal dichalcogenide WSe
2
, detected spectroscopically as the circular dichroism of the phonon-assisted transition of holes. Phonon chirality could be used to control the electron-phonon coupling and/or the phonon-driven topological states of solids.
Science
, this issue p.
579
A chiral response of phonons is observed in a monolayer of tungsten diselenide.
Chirality reveals symmetry breaking of the fundamental interaction of elementary particles. In condensed matter, for example, the chirality of electrons governs many unconventional transport phenomena such as the quantum Hall effect. Here we show that phonons can exhibit intrinsic chirality in monolayer tungsten diselenide. The broken inversion symmetry of the lattice lifts the degeneracy of clockwise and counterclockwise phonon modes at the corners of the Brillouin zone. We identified the phonons by the intervalley transfer of holes through hole-phonon interactions during the indirect infrared absorption, and we confirmed their chirality by the infrared circular dichroism arising from pseudoangular momentum conservation. The chiral phonons are important for electron-phonon coupling in solids, phonon-driven topological states, and energy-efficient information processing. |
|---|---|
| AbstractList | Chirality reveals symmetry breaking of the fundamental interaction of elementary particles. In condensed matter, for example, the chirality of electrons governs many unconventional transport phenomena such as the quantum Hall effect. Here we show that phonons can exhibit intrinsic chirality in monolayer tungsten diselenide. The broken inversion symmetry of the lattice lifts the degeneracy of clockwise and counterclockwise phonon modes at the corners of the Brillouin zone. We identified the phonons by the intervalley transfer of holes through hole-phonon interactions during the indirect infrared absorption, and we confirmed their chirality by the infrared circular dichroism arising from pseudoangular momentum conservation. The chiral phonons are important for electron-phonon coupling in solids, phonon-driven topological states, and energy-efficient information processing. A phonon merry-go-roundChirality is associated with the breaking of symmetry, often described as left- or right-handed behavior. Such asymmetry can be seen, for example, in the electronic responses of particular materials or the reactions between particular chemical species. Zhu et al. observed a chiral phonon mode in a monolayer of the transition metal dichalcogenide WSe2, detected spectroscopically as the circular dichroism of the phonon-assisted transition of holes. Phonon chirality could be used to control the electron-phonon coupling and/or the phonon-driven topological states of solids.Science, this issue p. 579Chirality reveals symmetry breaking of the fundamental interaction of elementary particles. In condensed matter, for example, the chirality of electrons governs many unconventional transport phenomena such as the quantum Hall effect. Here we show that phonons can exhibit intrinsic chirality in monolayer tungsten diselenide. The broken inversion symmetry of the lattice lifts the degeneracy of clockwise and counterclockwise phonon modes at the corners of the Brillouin zone. We identified the phonons by the intervalley transfer of holes through hole-phonon interactions during the indirect infrared absorption, and we confirmed their chirality by the infrared circular dichroism arising from pseudoangular momentum conservation. The chiral phonons are important for electron-phonon coupling in solids, phonon-driven topological states, and energy-efficient information processing. Chirality is associated with the breaking of symmetry, often described as left- or right-handed behavior. Such asymmetry can be seen, for example, in the electronic responses of particular materials or the reactions between particular chemical species. Zhu et al. observed a chiral phonon mode in a monolayer of the transition metal dichalcogenide WSe 2 , detected spectroscopically as the circular dichroism of the phonon-assisted transition of holes. Phonon chirality could be used to control the electron-phonon coupling and/or the phonon-driven topological states of solids. Science , this issue p. 579 A chiral response of phonons is observed in a monolayer of tungsten diselenide. Chirality reveals symmetry breaking of the fundamental interaction of elementary particles. In condensed matter, for example, the chirality of electrons governs many unconventional transport phenomena such as the quantum Hall effect. Here we show that phonons can exhibit intrinsic chirality in monolayer tungsten diselenide. The broken inversion symmetry of the lattice lifts the degeneracy of clockwise and counterclockwise phonon modes at the corners of the Brillouin zone. We identified the phonons by the intervalley transfer of holes through hole-phonon interactions during the indirect infrared absorption, and we confirmed their chirality by the infrared circular dichroism arising from pseudoangular momentum conservation. The chiral phonons are important for electron-phonon coupling in solids, phonon-driven topological states, and energy-efficient information processing. Chirality reveals symmetry breaking of the fundamental interaction of elementary particles. In condensed matter, for example, the chirality of electrons governs many unconventional transport phenomena such as the quantum Hall effect. Here we show that phonons can exhibit intrinsic chirality in monolayer tungsten diselenide. The broken inversion symmetry of the lattice lifts the degeneracy of clockwise and counterclockwise phonon modes at the corners of the Brillouin zone. We identified the phonons by the intervalley transfer of holes through hole-phonon interactions during the indirect infrared absorption, and we confirmed their chirality by the infrared circular dichroism arising from pseudoangular momentum conservation. The chiral phonons are important for electron-phonon coupling in solids, phonon-driven topological states, and energy-efficient information processing.Chirality reveals symmetry breaking of the fundamental interaction of elementary particles. In condensed matter, for example, the chirality of electrons governs many unconventional transport phenomena such as the quantum Hall effect. Here we show that phonons can exhibit intrinsic chirality in monolayer tungsten diselenide. The broken inversion symmetry of the lattice lifts the degeneracy of clockwise and counterclockwise phonon modes at the corners of the Brillouin zone. We identified the phonons by the intervalley transfer of holes through hole-phonon interactions during the indirect infrared absorption, and we confirmed their chirality by the infrared circular dichroism arising from pseudoangular momentum conservation. The chiral phonons are important for electron-phonon coupling in solids, phonon-driven topological states, and energy-efficient information processing. |
| Author | Zhang, Lifa Xiao, Jun Kaindl, Robert A. Li, Lain-Jong Yang, Chih-Wen Wang, Yuan Zhu, Hanyu Yi, Jun Li, Ming-Yang Zhang, Xiang |
| Author_xml | – sequence: 1 givenname: Hanyu orcidid: 0000-0003-3376-5352 surname: Zhu fullname: Zhu, Hanyu organization: Nanoscale Science and Engineering Center, University of California, Berkeley, CA 94720, USA., Materials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, CA 94720, USA – sequence: 2 givenname: Jun orcidid: 0000-0003-2186-6615 surname: Yi fullname: Yi, Jun organization: Nanoscale Science and Engineering Center, University of California, Berkeley, CA 94720, USA – sequence: 3 givenname: Ming-Yang orcidid: 0000-0001-8392-9752 surname: Li fullname: Li, Ming-Yang organization: Physical Sciences and Engineering Division, King Abdullah University of Science and Technology, Thuwal 23955-6900, Kingdom of Saudi Arabia – sequence: 4 givenname: Jun surname: Xiao fullname: Xiao, Jun organization: Nanoscale Science and Engineering Center, University of California, Berkeley, CA 94720, USA – sequence: 5 givenname: Lifa orcidid: 0000-0001-6108-1404 surname: Zhang fullname: Zhang, Lifa organization: Department of Physics, Nanjing Normal University, Nanjing, Jiangsu 210023, China – sequence: 6 givenname: Chih-Wen surname: Yang fullname: Yang, Chih-Wen organization: Physical Sciences and Engineering Division, King Abdullah University of Science and Technology, Thuwal 23955-6900, Kingdom of Saudi Arabia – sequence: 7 givenname: Robert A. orcidid: 0000-0003-3639-5625 surname: Kaindl fullname: Kaindl, Robert A. organization: Materials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, CA 94720, USA – sequence: 8 givenname: Lain-Jong orcidid: 0000-0002-4059-7783 surname: Li fullname: Li, Lain-Jong organization: Physical Sciences and Engineering Division, King Abdullah University of Science and Technology, Thuwal 23955-6900, Kingdom of Saudi Arabia – sequence: 9 givenname: Yuan orcidid: 0000-0001-7892-2812 surname: Wang fullname: Wang, Yuan organization: Nanoscale Science and Engineering Center, University of California, Berkeley, CA 94720, USA., Materials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, CA 94720, USA – sequence: 10 givenname: Xiang orcidid: 0000-0002-3272-894X surname: Zhang fullname: Zhang, Xiang organization: Nanoscale Science and Engineering Center, University of California, Berkeley, CA 94720, USA., Materials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, CA 94720, USA |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/29420291$$D View this record in MEDLINE/PubMed https://www.osti.gov/biblio/1436889$$D View this record in Osti.gov |
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| ContentType | Journal Article |
| Copyright | Copyright © 2018 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works. Copyright © 2018 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works |
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| DOI | 10.1126/science.aar2711 |
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| Snippet | Chirality is associated with the breaking of symmetry, often described as left- or right-handed behavior. Such asymmetry can be seen, for example, in the... Chirality reveals symmetry breaking of the fundamental interaction of elementary particles. In condensed matter, for example, the chirality of electrons... A phonon merry-go-roundChirality is associated with the breaking of symmetry, often described as left- or right-handed behavior. Such asymmetry can be seen,... |
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| SubjectTerms | Asymmetry Brillouin zones Broken symmetry Chemical reactions Chemical speciation Chirality Circular dichroism Condensed matter physics Coupling Data processing Dichroism Elementary particles Energy efficiency Hall effect Handedness Information processing Infrared absorption Lattice vibration Lifts Monolayers Phonons Quantum Hall effect Selenides Symmetry Transport phenomena Tungsten Tungsten compounds |
| Title | Observation of chiral phonons |
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