Ligand Tuning of Localized Surface Plasmon Resonances in Antimony-Doped Tin Oxide Nanocrystals

Aliovalent-doped metal oxide nanocrystals exhibiting localized surface plasmons (LSPRs) are applied in systems that require reflection/scattering/absorption in infrared and optical transparency in visible. Indium tin oxide (ITO) is currently leading the field, but indium resources are known to be ve...

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Published inNanomaterials (Basel, Switzerland) Vol. 12; no. 19; p. 3469
Main Authors Balitskii, Olexiy, Mashkov, Oleksandr, Barabash, Anastasiia, Rehm, Viktor, Afify, Hany A., Li, Ning, Hammer, Maria S., Brabec, Christoph J., Eigen, Andreas, Halik, Marcus, Yarema, Olesya, Yarema, Maksym, Wood, Vanessa, Stifter, David, Heiss, Wolfgang
Format Journal Article
LanguageEnglish
Published Basel MDPI AG 01.10.2022
MDPI
Subjects
Acids
Alternative energy sources
Antimony
Chloride
colloids
Crystals
Doping
Ethanol
Evans, W.H
Glazing
Indium
Indium tin oxides
Infrared reflection
Lewis acid
Ligands
Metal oxides
Nanocrystals
plasmonics
Plasmons
Semiconductors
Surface plasmon resonance
Tin
Tuning
Germany
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Abstract Aliovalent-doped metal oxide nanocrystals exhibiting localized surface plasmons (LSPRs) are applied in systems that require reflection/scattering/absorption in infrared and optical transparency in visible. Indium tin oxide (ITO) is currently leading the field, but indium resources are known to be very restricted. Antimony-doped tin oxide (ATO) is a cheap candidate to substitute the ITO, but it exhibits less advantageous electronic properties and limited control of the LSPRs. To date, LSPR tuning in ATO NCs has been achieved electrochemically and by aliovalent doping, with a significant decrease in doping efficiency with an increasing doping level. Here, we synthesize plasmonic ATO nanocrystals (NCs) via a solvothermal route and demonstrate ligand exchange to tune the LSPR energies. Attachment of ligands acting as Lewis acids and bases results in LSPR peak shifts with a doping efficiency overcoming those by aliovalent doping. Thus, this strategy is of potential interest for plasmon implementations, which are of potential interest for infrared upconversion, smart glazing, heat absorbers, or thermal barriers.
AbstractList Aliovalent-doped metal oxide nanocrystals exhibiting localized surface plasmons (LSPRs) are applied in systems that require reflection/scattering/absorption in infrared and optical transparency in visible. Indium tin oxide (ITO) is currently leading the field, but indium resources are known to be very restricted. Antimony-doped tin oxide (ATO) is a cheap candidate to substitute the ITO, but it exhibits less advantageous electronic properties and limited control of the LSPRs. To date, LSPR tuning in ATO NCs has been achieved electrochemically and by aliovalent doping, with a significant decrease in doping efficiency with an increasing doping level. Here, we synthesize plasmonic ATO nanocrystals (NCs) via a solvothermal route and demonstrate ligand exchange to tune the LSPR energies. Attachment of ligands acting as Lewis acids and bases results in LSPR peak shifts with a doping efficiency overcoming those by aliovalent doping. Thus, this strategy is of potential interest for plasmon implementations, which are of potential interest for infrared upconversion, smart glazing, heat absorbers, or thermal barriers.
Audience Academic
Author Yarema, Maksym
Li, Ning
Yarema, Olesya
Halik, Marcus
Afify, Hany A
Barabash, Anastasiia
Brabec, Christoph J
Eigen, Andreas
Hammer, Maria S
Wood, Vanessa
Stifter, David
Heiss, Wolfgang
Mashkov, Oleksandr
Rehm, Viktor
Balitskii, Olexiy
AuthorAffiliation 8 Institute for Electronics, Department of Information Technology and Electrical Engineering, ETH Zürich, 8092 Zürich, Switzerland
9 Center for Surface and Nanoanalytics (ZONA), Johannes Kepler University Linz, 4040 Linz, Austria
4 Institute-Materials for Electronics and Energy Technology (i-MEET), Department of Materials Science and Engineering, Friedrich-Alexander-Universität Erlangen-Nürnberg, Martensstraße 7, 91058 Erlangen, Germany
5 Department of Laser Sciences and Interactions, National Institute of Laser Enhanced Sciences (NILES), Cairo University, Giza 12613, Egypt
7 Organic Materials & Devices, Department of Material Science, Interdisciplinary Center for Nanostructured Films (IZNF), Friedrich-Alexander University Erlangen-Nürnberg (FAU), Cauerstrasse 3, 91058 Erlangen, Germany
2 Department of Electronics, Lviv Ivan Franko National University, Dragomanov Str., 50, 79005 Lviv, Ukraine
1 Institute-Materials for Electronics and Energy Technology (i-MEET), Department of Materials Scienc
AuthorAffiliation_xml – name: 7 Organic Materials & Devices, Department of Material Science, Interdisciplinary Center for Nanostructured Films (IZNF), Friedrich-Alexander University Erlangen-Nürnberg (FAU), Cauerstrasse 3, 91058 Erlangen, Germany
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RelatedPersons Evans, W.H
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Snippet Aliovalent-doped metal oxide nanocrystals exhibiting localized surface plasmons (LSPRs) are applied in systems that require reflection/scattering/absorption in...
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SubjectTerms Acids
Alternative energy sources
Antimony
Chloride
colloids
Crystals
Doping
Ethanol
Evans, W.H
Glazing
Indium
Indium tin oxides
Infrared reflection
Lewis acid
Ligands
Metal oxides
Nanocrystals
plasmonics
Plasmons
Semiconductors
Surface plasmon resonance
Tin
Tuning
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Title Ligand Tuning of Localized Surface Plasmon Resonances in Antimony-Doped Tin Oxide Nanocrystals
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https://search.proquest.com/docview/2725196649
https://pubmed.ncbi.nlm.nih.gov/PMC9565614
https://doaj.org/article/06704581b7b94916a715c84d254b6344
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