Fabrication of Polysulfone-Surface Functionalized Mesoporous Silica Nanocomposite Membranes for Removal of Heavy Metal Ions from Wastewater

Membranes are an efficient way to treat emulsified heavy metal-based wastewater, but they generally come with a trade-off between permeability and selectivity. In this research, the amine and sulphonic groups on the inner and outer surface of mesoporous silica nanoparticles (MSNs) were first modifie...

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Published inMembranes (Basel) Vol. 11; no. 12; p. 935
Main Authors Alotaibi, Abdullah A, Shukla, Arun Kumar, Mrad, Mohamed Habib, Alswieleh, Abdullah M, Alotaibi, Khalid M
Format Journal Article
LanguageEnglish
Published Switzerland MDPI AG 26.11.2021
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Abstract Membranes are an efficient way to treat emulsified heavy metal-based wastewater, but they generally come with a trade-off between permeability and selectivity. In this research, the amine and sulphonic groups on the inner and outer surface of mesoporous silica nanoparticles (MSNs) were first modified by a chemical approach. Then, MSNs with amine and sulphonic groups were utilized as new inorganic nanofiller to fabricate mixed matrix polysulfone (PSU) nanocomposite membranes using the classical phase inversion approach. The resultant nanoparticles and membranes were characterized by their physico-chemical characteristics as well as determination of pure water permeability along with cadmium and zinc ion removal. Embedding nanoparticles resulted in a significant rise in the water permeability as a result of changes in the surface properties and porosity of the membrane. Furthermore, the efficiency of developed membranes to remove cadmium and zinc was significantly improved by more than 90% due to the presence of functional groups on nanoparticles. The functionalized-MSNs/PSU nanocomposite membrane has the potential to be an effective industrial effluent removal membrane.
AbstractList Membranes are an efficient way to treat emulsified heavy metal-based wastewater, but they generally come with a trade-off between permeability and selectivity. In this research, the amine and sulphonic groups on the inner and outer surface of mesoporous silica nanoparticles (MSNs) were first modified by a chemical approach. Then, MSNs with amine and sulphonic groups were utilized as new inorganic nanofiller to fabricate mixed matrix polysulfone (PSU) nanocomposite membranes using the classical phase inversion approach. The resultant nanoparticles and membranes were characterized by their physico-chemical characteristics as well as determination of pure water permeability along with cadmium and zinc ion removal. Embedding nanoparticles resulted in a significant rise in the water permeability as a result of changes in the surface properties and porosity of the membrane. Furthermore, the efficiency of developed membranes to remove cadmium and zinc was significantly improved by more than 90% due to the presence of functional groups on nanoparticles. The functionalized-MSNs/PSU nanocomposite membrane has the potential to be an effective industrial effluent removal membrane.
Author Alotaibi, Khalid M
Alswieleh, Abdullah M
Alotaibi, Abdullah A
Mrad, Mohamed Habib
Shukla, Arun Kumar
AuthorAffiliation 2 King Abdullah Institute for Nanotechnology, King Saud University, Riyadh 11451, Saudi Arabia; ashukla@ksu.edu.sa
3 Department of Chemistry, College of Science, King Saud University, Riyadh 11451, Saudi Arabia
1 Department of Chemistry, College of Sciences and Humanities, Shaqra University, Ad-Dawadmi 11911, Saudi Arabia; aaalotaibi@su.edu.sa (A.A.A.); m.mrad@su.edu.sa (M.H.M.)
AuthorAffiliation_xml – name: 2 King Abdullah Institute for Nanotechnology, King Saud University, Riyadh 11451, Saudi Arabia; ashukla@ksu.edu.sa
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– name: 1 Department of Chemistry, College of Sciences and Humanities, Shaqra University, Ad-Dawadmi 11911, Saudi Arabia; aaalotaibi@su.edu.sa (A.A.A.); m.mrad@su.edu.sa (M.H.M.)
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BackLink https://www.ncbi.nlm.nih.gov/pubmed/34940436$$D View this record in MEDLINE/PubMed
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Issue 12
Keywords heavy metal removal
nanocomposite membrane
functionalized mesoporous silica nanoparticles
polysulfone
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SSID ssj0000605630
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Snippet Membranes are an efficient way to treat emulsified heavy metal-based wastewater, but they generally come with a trade-off between permeability and selectivity....
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Open Access Repository
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StartPage 935
SubjectTerms Aqueous solutions
Cadmium
Cellulose acetate
Chemicals
Embedding
Fabrication
Functional groups
functionalized mesoporous silica nanoparticles
heavy metal removal
Heavy metals
Industrial effluents
Industrial wastewater
Membranes
Metal ions
Morphology
nanocomposite membrane
Nanocomposites
Nanomaterials
Nanoparticles
Nitrates
Permeability
Polymers
Polysulfone
Polysulfone resins
Porosity
Scanning electron microscopy
Selectivity
Silica
Silicon dioxide
Sulfonic acid
Surface properties
Transmission electron microscopy
Wastewater
Wastewater treatment
Zinc
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Title Fabrication of Polysulfone-Surface Functionalized Mesoporous Silica Nanocomposite Membranes for Removal of Heavy Metal Ions from Wastewater
URI https://www.ncbi.nlm.nih.gov/pubmed/34940436
https://www.proquest.com/docview/2612813312
https://search.proquest.com/docview/2613292790
https://pubmed.ncbi.nlm.nih.gov/PMC8706919
https://doaj.org/article/d7cf0dd481e64753b7cb8cf6df75969b
Volume 11
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