Adsorption of anionic azo-dyes from aqueous solutions onto graphene oxide: Equilibrium, kinetic and thermodynamic studies

[Display omitted] In the present study, graphene oxide (GO) was used for the adsorption of anionic azo-dyes such as Acid Orange 8 (AO8) and Direct Red 23 (DR23) from aqueous solutions. GO was characterized by Fourier Transform-Infrared Spectroscopy (FTIR), X-ray Photoelectron Spectroscopy (XPS), The...

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Published in	Journal of colloid and interface science Vol. 496; pp. 188 - 200
Main Authors	Konicki, Wojciech, Aleksandrzak, Małgorzata, Moszyński, Dariusz, Mijowska, Ewa
Format	Journal Article
Language	English
Published	United States Elsevier Inc 15.06.2017
Subjects	Adsorption Anionic dyes aqueous solutions atomic force microscopy azo dyes data analysis endothermy equations Fourier transform infrared spectroscopy Graphene oxide heat production Kinetics scanning electron microscopy temperature Thermodynamics thermogravimetry transmission electron microscopy X-ray diffraction X-ray photoelectron spectroscopy zeta potential Thermodynamics Anionic dyes Graphene oxide Kinetics Adsorption
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Abstract	[Display omitted] In the present study, graphene oxide (GO) was used for the adsorption of anionic azo-dyes such as Acid Orange 8 (AO8) and Direct Red 23 (DR23) from aqueous solutions. GO was characterized by Fourier Transform-Infrared Spectroscopy (FTIR), X-ray Photoelectron Spectroscopy (XPS), Thermogravimetric Analysis (TGA), Atomic Force Microscopy (AFM), X-ray Diffraction (XRD), Scanning Electron Microscopy (SEM), High-Resolution Transmission Electron Microscopy (HRTEM) and zeta potential measurements. The influence of dye initial concentration, temperature and pH on AO8 and DR23 adsorption onto GO was investigated. Equilibrium data were analyzed by model equations such as Langmuir Freundlich, Temkin, Dubinin-Radushkevich and Redlich-Peterson isotherms and were best represented by Langmuir and Redlich-Peterson isotherm model. Kinetic adsorption data were analyzed using the pseudo-first-order kinetic model, the pseudo-second-order kinetic model and the intraparticle diffusion model. The adsorption kinetics well fitted using a pseudo-second-order kinetic model. Thermodynamics parameters, ΔG°, ΔH° and ΔS°, were calculated, indicating that the adsorption of AO8 and DR23 onto GO was spontaneous process. The adsorption process of AO8 onto GO was exothermic, while the adsorption of DR23 onto GO was endothermic in nature.
AbstractList	In the present study, graphene oxide (GO) was used for the adsorption of anionic azo-dyes such as Acid Orange 8 (AO8) and Direct Red 23 (DR23) from aqueous solutions. GO was characterized by Fourier Transform-Infrared Spectroscopy (FTIR), X-ray Photoelectron Spectroscopy (XPS), Thermogravimetric Analysis (TGA), Atomic Force Microscopy (AFM), X-ray Diffraction (XRD), Scanning Electron Microscopy (SEM), High-Resolution Transmission Electron Microscopy (HRTEM) and zeta potential measurements. The influence of dye initial concentration, temperature and pH on AO8 and DR23 adsorption onto GO was investigated. Equilibrium data were analyzed by model equations such as Langmuir Freundlich, Temkin, Dubinin-Radushkevich and Redlich-Peterson isotherms and were best represented by Langmuir and Redlich-Peterson isotherm model. Kinetic adsorption data were analyzed using the pseudo-first-order kinetic model, the pseudo-second-order kinetic model and the intraparticle diffusion model. The adsorption kinetics well fitted using a pseudo-second-order kinetic model. Thermodynamics parameters, ΔG°, ΔH° and ΔS°, were calculated, indicating that the adsorption of AO8 and DR23 onto GO was spontaneous process. The adsorption process of AO8 onto GO was exothermic, while the adsorption of DR23 onto GO was endothermic in nature.In the present study, graphene oxide (GO) was used for the adsorption of anionic azo-dyes such as Acid Orange 8 (AO8) and Direct Red 23 (DR23) from aqueous solutions. GO was characterized by Fourier Transform-Infrared Spectroscopy (FTIR), X-ray Photoelectron Spectroscopy (XPS), Thermogravimetric Analysis (TGA), Atomic Force Microscopy (AFM), X-ray Diffraction (XRD), Scanning Electron Microscopy (SEM), High-Resolution Transmission Electron Microscopy (HRTEM) and zeta potential measurements. The influence of dye initial concentration, temperature and pH on AO8 and DR23 adsorption onto GO was investigated. Equilibrium data were analyzed by model equations such as Langmuir Freundlich, Temkin, Dubinin-Radushkevich and Redlich-Peterson isotherms and were best represented by Langmuir and Redlich-Peterson isotherm model. Kinetic adsorption data were analyzed using the pseudo-first-order kinetic model, the pseudo-second-order kinetic model and the intraparticle diffusion model. The adsorption kinetics well fitted using a pseudo-second-order kinetic model. Thermodynamics parameters, ΔG°, ΔH° and ΔS°, were calculated, indicating that the adsorption of AO8 and DR23 onto GO was spontaneous process. The adsorption process of AO8 onto GO was exothermic, while the adsorption of DR23 onto GO was endothermic in nature. [Display omitted] In the present study, graphene oxide (GO) was used for the adsorption of anionic azo-dyes such as Acid Orange 8 (AO8) and Direct Red 23 (DR23) from aqueous solutions. GO was characterized by Fourier Transform-Infrared Spectroscopy (FTIR), X-ray Photoelectron Spectroscopy (XPS), Thermogravimetric Analysis (TGA), Atomic Force Microscopy (AFM), X-ray Diffraction (XRD), Scanning Electron Microscopy (SEM), High-Resolution Transmission Electron Microscopy (HRTEM) and zeta potential measurements. The influence of dye initial concentration, temperature and pH on AO8 and DR23 adsorption onto GO was investigated. Equilibrium data were analyzed by model equations such as Langmuir Freundlich, Temkin, Dubinin-Radushkevich and Redlich-Peterson isotherms and were best represented by Langmuir and Redlich-Peterson isotherm model. Kinetic adsorption data were analyzed using the pseudo-first-order kinetic model, the pseudo-second-order kinetic model and the intraparticle diffusion model. The adsorption kinetics well fitted using a pseudo-second-order kinetic model. Thermodynamics parameters, ΔG°, ΔH° and ΔS°, were calculated, indicating that the adsorption of AO8 and DR23 onto GO was spontaneous process. The adsorption process of AO8 onto GO was exothermic, while the adsorption of DR23 onto GO was endothermic in nature. In the present study, graphene oxide (GO) was used for the adsorption of anionic azo-dyes such as Acid Orange 8 (AO8) and Direct Red 23 (DR23) from aqueous solutions. GO was characterized by Fourier Transform-Infrared Spectroscopy (FTIR), X-ray Photoelectron Spectroscopy (XPS), Thermogravimetric Analysis (TGA), Atomic Force Microscopy (AFM), X-ray Diffraction (XRD), Scanning Electron Microscopy (SEM), High-Resolution Transmission Electron Microscopy (HRTEM) and zeta potential measurements. The influence of dye initial concentration, temperature and pH on AO8 and DR23 adsorption onto GO was investigated. Equilibrium data were analyzed by model equations such as Langmuir Freundlich, Temkin, Dubinin-Radushkevich and Redlich-Peterson isotherms and were best represented by Langmuir and Redlich-Peterson isotherm model. Kinetic adsorption data were analyzed using the pseudo-first-order kinetic model, the pseudo-second-order kinetic model and the intraparticle diffusion model. The adsorption kinetics well fitted using a pseudo-second-order kinetic model. Thermodynamics parameters, ΔG°, ΔH° and ΔS°, were calculated, indicating that the adsorption of AO8 and DR23 onto GO was spontaneous process. The adsorption process of AO8 onto GO was exothermic, while the adsorption of DR23 onto GO was endothermic in nature.
Author	Konicki, Wojciech Aleksandrzak, Małgorzata Mijowska, Ewa Moszyński, Dariusz
Author_xml	– sequence: 1 givenname: Wojciech surname: Konicki fullname: Konicki, Wojciech email: w.konicki@am.szczecin.pl organization: Department of Integrated Transport Technology and Environmental Protection, Maritime University of Szczecin, H. Pobożnego St. 11, 70-507 Szczecin, Poland – sequence: 2 givenname: Małgorzata surname: Aleksandrzak fullname: Aleksandrzak, Małgorzata organization: Institute of Chemical and Environment Engineering, West Pomeranian University of Technology, Pułaskiego St. 10, 70-322 Szczecin, Poland – sequence: 3 givenname: Dariusz surname: Moszyński fullname: Moszyński, Dariusz organization: Institute of Chemical and Environment Engineering, West Pomeranian University of Technology, Pułaskiego St. 10, 70-322 Szczecin, Poland – sequence: 4 givenname: Ewa surname: Mijowska fullname: Mijowska, Ewa organization: Institute of Chemical and Environment Engineering, West Pomeranian University of Technology, Pułaskiego St. 10, 70-322 Szczecin, Poland
BackLink	https://www.ncbi.nlm.nih.gov/pubmed/28232292$$D View this record in MEDLINE/PubMed
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Snippet	[Display omitted] In the present study, graphene oxide (GO) was used for the adsorption of anionic azo-dyes such as Acid Orange 8 (AO8) and Direct Red 23... In the present study, graphene oxide (GO) was used for the adsorption of anionic azo-dyes such as Acid Orange 8 (AO8) and Direct Red 23 (DR23) from aqueous...
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SubjectTerms	Adsorption Anionic dyes aqueous solutions atomic force microscopy azo dyes data analysis endothermy equations Fourier transform infrared spectroscopy Graphene oxide heat production Kinetics scanning electron microscopy temperature Thermodynamics thermogravimetry transmission electron microscopy X-ray diffraction X-ray photoelectron spectroscopy zeta potential
Title	Adsorption of anionic azo-dyes from aqueous solutions onto graphene oxide: Equilibrium, kinetic and thermodynamic studies
URI	https://dx.doi.org/10.1016/j.jcis.2017.02.031 https://www.ncbi.nlm.nih.gov/pubmed/28232292 https://www.proquest.com/docview/1872579108 https://www.proquest.com/docview/2116873878
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