Upconversion carbon quantum dots as visible light responsive component for efficient enhancement of photocatalytic performance
[Display omitted] It finds that CQDs synthesized by hydrothermal method possess obvious upconversion properties that could transfer low energy photons to high energy photons, resulting in enhanced visible light response and utilization. Herein, carbon quantum dots (CQDs) modified TiO2 photocatylysts...
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| Published in | Journal of colloid and interface science Vol. 496; pp. 425 - 433 |
|---|---|
| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
United States
Elsevier Inc
15.06.2017
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| Subjects | |
| Online Access | Get full text |
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| Abstract | [Display omitted]
It finds that CQDs synthesized by hydrothermal method possess obvious upconversion properties that could transfer low energy photons to high energy photons, resulting in enhanced visible light response and utilization. Herein, carbon quantum dots (CQDs) modified TiO2 photocatylysts were successfully prepared by a facile sol-gel method. Photophysical and surficial properties of the as-prepared composite photocatalyst were investigated in details. Furthermore, photocatalytic performance was tested by degrading methylene blue (MB) under visible light irradiation. The degradation efficiency of methylene blue (MB) is as high as 90% within 120min, which is 3.6 times higher than that of pure TiO2. |
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| AbstractList | [Display omitted]
It finds that CQDs synthesized by hydrothermal method possess obvious upconversion properties that could transfer low energy photons to high energy photons, resulting in enhanced visible light response and utilization. Herein, carbon quantum dots (CQDs) modified TiO2 photocatylysts were successfully prepared by a facile sol-gel method. Photophysical and surficial properties of the as-prepared composite photocatalyst were investigated in details. Furthermore, photocatalytic performance was tested by degrading methylene blue (MB) under visible light irradiation. The degradation efficiency of methylene blue (MB) is as high as 90% within 120min, which is 3.6 times higher than that of pure TiO2. It finds that CQDs synthesized by hydrothermal method possess obvious upconversion properties that could transfer low energy photons to high energy photons, resulting in enhanced visible light response and utilization. Herein, carbon quantum dots (CQDs) modified TiO2 photocatylysts were successfully prepared by a facile sol-gel method. Photophysical and surficial properties of the as-prepared composite photocatalyst were investigated in details. Furthermore, photocatalytic performance was tested by degrading methylene blue (MB) under visible light irradiation. The degradation efficiency of methylene blue (MB) is as high as 90% within 120min, which is 3.6 times higher than that of pure TiO2. It finds that CQDs synthesized by hydrothermal method possess obvious upconversion properties that could transfer low energy photons to high energy photons, resulting in enhanced visible light response and utilization. Herein, carbon quantum dots (CQDs) modified TiO photocatylysts were successfully prepared by a facile sol-gel method. Photophysical and surficial properties of the as-prepared composite photocatalyst were investigated in details. Furthermore, photocatalytic performance was tested by degrading methylene blue (MB) under visible light irradiation. The degradation efficiency of methylene blue (MB) is as high as 90% within 120min, which is 3.6 times higher than that of pure TiO . It finds that CQDs synthesized by hydrothermal method possess obvious upconversion properties that could transfer low energy photons to high energy photons, resulting in enhanced visible light response and utilization. Herein, carbon quantum dots (CQDs) modified TiO2 photocatylysts were successfully prepared by a facile sol-gel method. Photophysical and surficial properties of the as-prepared composite photocatalyst were investigated in details. Furthermore, photocatalytic performance was tested by degrading methylene blue (MB) under visible light irradiation. The degradation efficiency of methylene blue (MB) is as high as 90% within 120min, which is 3.6 times higher than that of pure TiO2.It finds that CQDs synthesized by hydrothermal method possess obvious upconversion properties that could transfer low energy photons to high energy photons, resulting in enhanced visible light response and utilization. Herein, carbon quantum dots (CQDs) modified TiO2 photocatylysts were successfully prepared by a facile sol-gel method. Photophysical and surficial properties of the as-prepared composite photocatalyst were investigated in details. Furthermore, photocatalytic performance was tested by degrading methylene blue (MB) under visible light irradiation. The degradation efficiency of methylene blue (MB) is as high as 90% within 120min, which is 3.6 times higher than that of pure TiO2. |
| Author | Zhao, Qidong Wang, Shaobin Ke, Jun Li, Xinyong Liu, Baojun Liu, Shaomin |
| Author_xml | – sequence: 1 givenname: Jun surname: Ke fullname: Ke, Jun organization: State Key Laboratory of Fine Chemical, Key Laboratory of Industrial Ecology and Environmental Engineering (MOE), School of Environmental Science and Technology, Dalian University of Technology, Dalian 116024, China – sequence: 2 givenname: Xinyong surname: Li fullname: Li, Xinyong email: xyli@dlut.edu.cn organization: State Key Laboratory of Fine Chemical, Key Laboratory of Industrial Ecology and Environmental Engineering (MOE), School of Environmental Science and Technology, Dalian University of Technology, Dalian 116024, China – sequence: 3 givenname: Qidong surname: Zhao fullname: Zhao, Qidong organization: State Key Laboratory of Fine Chemical, Key Laboratory of Industrial Ecology and Environmental Engineering (MOE), School of Environmental Science and Technology, Dalian University of Technology, Dalian 116024, China – sequence: 4 givenname: Baojun surname: Liu fullname: Liu, Baojun organization: State Key Laboratory of Fine Chemical, Key Laboratory of Industrial Ecology and Environmental Engineering (MOE), School of Environmental Science and Technology, Dalian University of Technology, Dalian 116024, China – sequence: 5 givenname: Shaomin surname: Liu fullname: Liu, Shaomin organization: Department of Chemical Engineering, Curtin University, Perth, GPO Box U1987, WA 6845, Australia – sequence: 6 givenname: Shaobin surname: Wang fullname: Wang, Shaobin email: shaobin.wang@curtin.edu.au organization: Department of Chemical Engineering, Curtin University, Perth, GPO Box U1987, WA 6845, Australia |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/28254609$$D View this record in MEDLINE/PubMed |
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It finds that CQDs synthesized by hydrothermal method possess obvious upconversion properties that could transfer low energy photons to high... It finds that CQDs synthesized by hydrothermal method possess obvious upconversion properties that could transfer low energy photons to high energy photons,... |
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| SubjectTerms | Carbon materials carbon quantum dots energy hot water treatment irradiation methylene blue Photocatalysis photocatalysts photons Quantum dots sol-gel processing titanium dioxide Upconversion |
| Title | Upconversion carbon quantum dots as visible light responsive component for efficient enhancement of photocatalytic performance |
| URI | https://dx.doi.org/10.1016/j.jcis.2017.01.121 https://www.ncbi.nlm.nih.gov/pubmed/28254609 https://www.proquest.com/docview/1874441527 https://www.proquest.com/docview/2116863391 |
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