Effective separation of propylene/propane binary mixtures by ZIF-8 membranes

► The first example for effective separation of C 3H 6/C 3H 8 mixtures by ZIF membranes. ► Excellent separation performance well beyond existing membranes. ► A novel process for preparation of high quality ZIF-8 membranes. ► Excellent membrane reproducibility, thermal and long-term stability. The se...

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Published in	Journal of membrane science Vol. 390; pp. 93 - 98
Main Authors	Pan, Yichang, Li, Tao, Lestari, Gabriella, Lai, Zhiping
Format	Journal Article
Language	English
Published	Amsterdam Elsevier B.V 15.02.2012 Elsevier
Subjects	artificial membranes carbon Chemistry Colloidal state and disperse state Exact sciences and technology General and physical chemistry Hydrothermal seeded growth industry Membranes Molecular sieving permeability polymers propane propylene Propylene/propane separation thermal stability ZIF membrane ZIF-8 Propylene/propane separation ZIF membrane Molecular sieving ZIF-8 Hydrothermal seeded growth Polymeric membrane Five membered ring Experimental data Separation Nitrogen heterocycle Permeability Thermal stability Petrochemical industry Binary mixture Hydrothermal growth Propene Reproducibility Imidazole Membrane Inorganic membrane Propane
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Abstract	► The first example for effective separation of C 3H 6/C 3H 8 mixtures by ZIF membranes. ► Excellent separation performance well beyond existing membranes. ► A novel process for preparation of high quality ZIF-8 membranes. ► Excellent membrane reproducibility, thermal and long-term stability. The separation of propylene/propane mixtures is one of the most important but challenging processes in the petrochemical industry. A novel zeolitic imidazole framework (ZIF-8) membrane prepared by a facile hydrothermal seeded growth method showed excellent separation performances for a wide range of propylene/propane mixtures. The membrane showed a permeability of propylene up to 200 barrers and a propylene to propane separation factor up to 50 at optimal separation conditions, well surpassing the “upper-bound trade-off” lines of existing polymer and carbon membranes. The experimental data also showed that the membranes had excellent reproducibility, long-term stability and thermal stability.
AbstractList	The separation of propylene/propane mixtures is one of the most important but challenging processes in the petrochemical industry. A novel zeolitic imidazole framework (ZIF-8) membrane prepared by a facile hydrothermal seeded growth method showed excellent separation performances for a wide range of propylene/propane mixtures. The membrane showed a permeability of propylene up to 200barrers and a propylene to propane separation factor up to 50 at optimal separation conditions, well surpassing the “upper-bound trade-off” lines of existing polymer and carbon membranes. The experimental data also showed that the membranes had excellent reproducibility, long-term stability and thermal stability. The separation of propylene/propane mixtures is one of the most important but challenging processes in the petrochemical industry. A novel zeolitic imidazole framework (ZIF-8) membrane prepared by a facile hydrothermal seeded growth method showed excellent separation performances for a wide range of propylene/propane mixtures. The membrane showed a permeability of propylene up to 200 barrers and a propylene to propane separation factor up to 50 at optimal separation conditions, well surpassing the "upper-bound trade-off" lines of existing polymer and carbon membranes. The experimental data also showed that the membranes had excellent reproducibility, long-term stability and thermal stability. ► The first example for effective separation of C 3H 6/C 3H 8 mixtures by ZIF membranes. ► Excellent separation performance well beyond existing membranes. ► A novel process for preparation of high quality ZIF-8 membranes. ► Excellent membrane reproducibility, thermal and long-term stability. The separation of propylene/propane mixtures is one of the most important but challenging processes in the petrochemical industry. A novel zeolitic imidazole framework (ZIF-8) membrane prepared by a facile hydrothermal seeded growth method showed excellent separation performances for a wide range of propylene/propane mixtures. The membrane showed a permeability of propylene up to 200 barrers and a propylene to propane separation factor up to 50 at optimal separation conditions, well surpassing the “upper-bound trade-off” lines of existing polymer and carbon membranes. The experimental data also showed that the membranes had excellent reproducibility, long-term stability and thermal stability.
Author	Lestari, Gabriella Pan, Yichang Li, Tao Lai, Zhiping
Author_xml	– sequence: 1 givenname: Yichang surname: Pan fullname: Pan, Yichang – sequence: 2 givenname: Tao surname: Li fullname: Li, Tao – sequence: 3 givenname: Gabriella surname: Lestari fullname: Lestari, Gabriella – sequence: 4 givenname: Zhiping surname: Lai fullname: Lai, Zhiping email: zhiping.lai@kaust.edu.sa
BackLink	http://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=25918458$$DView record in Pascal Francis
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Keywords	Propylene/propane separation ZIF membrane Molecular sieving ZIF-8 Hydrothermal seeded growth Polymeric membrane Five membered ring Experimental data Separation Nitrogen heterocycle Permeability Thermal stability Petrochemical industry Binary mixture Hydrothermal growth Propene Reproducibility Imidazole Membrane Inorganic membrane Propane
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Snippet	► The first example for effective separation of C 3H 6/C 3H 8 mixtures by ZIF membranes. ► Excellent separation performance well beyond existing membranes. ► A... The separation of propylene/propane mixtures is one of the most important but challenging processes in the petrochemical industry. A novel zeolitic imidazole...
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SubjectTerms	artificial membranes carbon Chemistry Colloidal state and disperse state Exact sciences and technology General and physical chemistry Hydrothermal seeded growth industry Membranes Molecular sieving permeability polymers propane propylene Propylene/propane separation thermal stability ZIF membrane ZIF-8
Title	Effective separation of propylene/propane binary mixtures by ZIF-8 membranes
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