Colloidal organic matter from wastewater treatment plant effluents: Characterization and role in metal distribution
Colloidal organic matter from wastewater treatment plants was characterized and examined with respect to its role in metal distribution by using tangential flow ultrafiltration, liquid chromatography coupled with organic carbon and UV detectors, and an asymmetrical flow field-flow fractionation (AFl...
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| Published in | Water research (Oxford) Vol. 44; no. 1; pp. 340 - 350 |
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| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Kidlington
Elsevier Ltd
01.01.2010
Elsevier IWA Publishing/Elsevier |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Colloidal organic matter from wastewater treatment plants was characterized and examined with respect to its role in metal distribution by using tangential flow ultrafiltration, liquid chromatography coupled with organic carbon and UV detectors, and an asymmetrical flow field-flow fractionation (AFlFFF) multidetection platform. Results revealed that a humic-like fraction of low aromaticity with an average molar mass ranging from 1600 to 2600Da was the main colloidal component. High molar mass fractions (HMM), with molar mass ranges between 20 and 200kDa, were present in lower proportions. Ag, Cd, Cu, Cr, Mn and Zn were found mainly in the dissolved phase (<0.45μm) and their distribution between colloidal and truly dissolved fractions was strongly influenced by the distribution of dissolved organic carbon. AFlFFF coupled to ICP-MS showed that Ag, Cd, Cu, Cr, Mn and Zn associate to the low molar mass fraction of the colloidal pool, whereas Al, Fe and Pb were equally bound to low and high molar mass fractions. |
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| AbstractList | Colloidal organic matter from wastewater treatment plants was characterized and examined with respect to its role in metal distribution by using tangential flow ultrafiltration, liquid chromatography coupled with organic carbon and UV detectors, and an asymmetrical flow field-flow fractionation (AFlFFF) multidetection platform. Results revealed that a humic-like fraction of low aromaticity with an average molar mass ranging from 1600 to 2600Da was the main colloidal component. High molar mass fractions (HMM), with molar mass ranges between 20 and 200kDa, were present in lower proportions. Ag, Cd, Cu, Cr, Mn and Zn were found mainly in the dissolved phase (<0.45microm) and their distribution between colloidal and truly dissolved fractions was strongly influenced by the distribution of dissolved organic carbon. AFlFFF coupled to ICP-MS showed that Ag, Cd, Cu, Cr, Mn and Zn associate to the low molar mass fraction of the colloidal pool, whereas Al, Fe and Pb were equally bound to low and high molar mass fractions. Colloidal organic matter from wastewater treatment plants was characterized and examined with respect to its role in metal distribution by using tangential flow ultrafiltration, liquid chromatography coupled with organic carbon and UV detectors, and an asymmetrical flow field-flow fractionation (AFlFFF) multidetection platform. Results revealed that a humic-like fraction of low aromaticity with an average molar mass ranging from 1600 to 2600Da was the main colloidal component. High molar mass fractions (HMM), with molar mass ranges between 20 and 200kDa, were present in lower proportions. Ag, Cd, Cu, Cr, Mn and Zn were found mainly in the dissolved phase (<0.45μm) and their distribution between colloidal and truly dissolved fractions was strongly influenced by the distribution of dissolved organic carbon. AFlFFF coupled to ICP-MS showed that Ag, Cd, Cu, Cr, Mn and Zn associate to the low molar mass fraction of the colloidal pool, whereas Al, Fe and Pb were equally bound to low and high molar mass fractions. Colloidal organic matter from wastewater treatment plants was characterized and examined with respect to its role in metal distribution by using tangential flow ultrafiltration, liquid chromatography coupled with organic carbon and UV detectors, and an asymmetrical flow field-flow fractionation (AFlFFF) multidetection platform. Results revealed that a humic-like fraction of low aromaticity with an average molar mass ranging from 1600 to 2600Da was the main colloidal component. High molar mass fractions (HMM), with molar mass ranges between 20 and 200kDa, were present in lower proportions. Ag, Cd, Cu, Cr, Mn and Zn were found mainly in the dissolved phase (<0.45 mu m) and their distribution between colloidal and truly dissolved fractions was strongly influenced by the distribution of dissolved organic carbon. AFlFFF coupled to ICP-MS showed that Ag, Cd, Cu, Cr, Mn and Zn associate to the low molar mass fraction of the colloidal pool, whereas Al, Fe and Pb were equally bound to low and high molar mass fractions. Colloidal organic matter from wastewater treatment plants was characterized and examined with respect to its role in metal distribution by using tangential flow ultrafiltration, liquid chromatography coupled with organic carbon and UV detectors, and an asymmetrical flow field-flow fractionation (AFlFFF) multidetection platform. Results revealed that a humic-like fraction of low aromaticity with an average molar mass ranging from 1600 to 2600 Da was the main colloidal component. High molar mass fractions (HMM), with molar mass ranges between 20 and 200 kDa, were present in lower proportions. Ag, Cd, Cu, Cr, Mn and Zn were found mainly in the dissolved phase (<0.45 μm) and their distribution between colloidal and truly dissolved fractions was strongly influenced by the distribution of dissolved organic carbon. AFlFFF coupled to ICP-MS showed that Ag, Cd, Cu, Cr, Mn and Zn associate to the low molar mass fraction of the colloidal pool, whereas Al, Fe and Pb were equally bound to low and high molar mass fractions Colloidal organic matter from wastewater treatment plants was characterized and examined with respect to its role in metal distribution by using tangential flow ultrafiltration, liquid chromatography coupled with organic carbon and UV detectors, and an asymmetrical flow field-flow fractionation (AFlFFF) multidetection platform. Results revealed that a humic-like fraction of low aromaticity with an average molar mass ranging from 1600 to 2600Da was the main colloidal component. High molar mass fractions (HMM), with molar mass ranges between 20 and 200kDa, were present in lower proportions. Ag, Cd, Cu, Cr, Mn and Zn were found mainly in the dissolved phase (<0.45microm) and their distribution between colloidal and truly dissolved fractions was strongly influenced by the distribution of dissolved organic carbon. AFlFFF coupled to ICP-MS showed that Ag, Cd, Cu, Cr, Mn and Zn associate to the low molar mass fraction of the colloidal pool, whereas Al, Fe and Pb were equally bound to low and high molar mass fractions. |
| Author | Sigg, Laura Worms, Isabelle A.M. Dubascoux, Stephane Lespes, Gaetane Al-Gorani Szigeti, Zsofia Traber, Jacqueline Slaveykova, Vera I. |
| Author_xml | – sequence: 1 givenname: Isabelle A.M. surname: Worms fullname: Worms, Isabelle A.M. organization: Environmental Biophysical Chemistry, GR-SLV-IIE-ENAC, Ecole Polytechnique Fédérale de Lausanne (EPFL), Station 2, 1015 Lausanne, Switzerland – sequence: 2 givenname: Zsofia surname: Al-Gorani Szigeti fullname: Al-Gorani Szigeti, Zsofia organization: Environmental Biophysical Chemistry, GR-SLV-IIE-ENAC, Ecole Polytechnique Fédérale de Lausanne (EPFL), Station 2, 1015 Lausanne, Switzerland – sequence: 3 givenname: Stephane surname: Dubascoux fullname: Dubascoux, Stephane organization: LCABIE CNRS UMR 5254 IPREM, Université de Pau and des Pays de l'Adour, Helioparc, Avenue du Président Pierre Angot, 64053 Pau, France – sequence: 4 givenname: Gaetane surname: Lespes fullname: Lespes, Gaetane organization: LCABIE CNRS UMR 5254 IPREM, Université de Pau and des Pays de l'Adour, Helioparc, Avenue du Président Pierre Angot, 64053 Pau, France – sequence: 5 givenname: Jacqueline surname: Traber fullname: Traber, Jacqueline organization: Eawag, Swiss Federal Institute of Aquatic Science and Technology, Ueberlandstrasse 133, PO Box 611, CH-8600 Duebendorf, Switzerland – sequence: 6 givenname: Laura surname: Sigg fullname: Sigg, Laura organization: Eawag, Swiss Federal Institute of Aquatic Science and Technology, Ueberlandstrasse 133, PO Box 611, CH-8600 Duebendorf, Switzerland – sequence: 7 givenname: Vera I. surname: Slaveykova fullname: Slaveykova, Vera I. email: vera.slaveykova@epfl.ch organization: Environmental Biophysical Chemistry, GR-SLV-IIE-ENAC, Ecole Polytechnique Fédérale de Lausanne (EPFL), Station 2, 1015 Lausanne, Switzerland |
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| Keywords | Metal binding Wastewater effluent Tangential flow ultrafiltration Asymmetrical flow field-flow fractionation LC-OCD Colloids fractionation Organic matter Pollutant behavior Liquid chromatography Flow field Sewage treatment plant Asymmetrical flow field-flow Waste water Dissolved matter Dissolved organic carbon Membrane separation Ultraviolet detector ICP mass spectroscopy Ultrafiltration Lead Colloid particle Speciation |
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| SubjectTerms | Analytical chemistry Applied sciences Asymmetrical flow field-flow fractionation Cadmium Carbon Chemical Sciences Chromium Colloids Colloids - analysis Colloids - chemistry Dissolution Environmental Sciences Exact sciences and technology LC-OCD Manganese Metal binding Metals - analysis Other industrial wastes. Sewage sludge Pollution Silver Tangential flow ultrafiltration Ultrafiltration Waste Disposal, Fluid - methods Wastes Wastewater effluent Wastewater treatment Water Pollutants, Chemical - analysis Water Pollutants, Chemical - chemistry Water treatment and pollution |
| Title | Colloidal organic matter from wastewater treatment plant effluents: Characterization and role in metal distribution |
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