Methyltrioxorhenium Catalysis in Nonconventional Solvents: A Great Catalyst in a Safe Reaction Medium

The requirement that chemical processes are sustainabable, reflected in waste reduction and the use of safe reagents and reaction conditions, is becoming even more stringent as a result of pressure by society and governments to preserve the environment and protect human health. Catalysis offers nume...

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Published inChemSusChem Vol. 3; no. 5; pp. 524 - 540
Main Authors Crucianelli, Marcello, Saladino, Raffaele, De Angelis, Francesco
Format Journal Article
LanguageEnglish
Published Weinheim WILEY-VCH Verlag 25.05.2010
WILEY‐VCH Verlag
Subjects
Catalysis
Green Chemistry Technology - methods
ionic liquids
Ionic Liquids - chemistry
Organometallic Compounds - chemistry
oxidation
Oxidation-Reduction
rhenium
Solvents - chemistry
sustainable chemistry
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Abstract The requirement that chemical processes are sustainabable, reflected in waste reduction and the use of safe reagents and reaction conditions, is becoming even more stringent as a result of pressure by society and governments to preserve the environment and protect human health. Catalysis offers numerous benefits related to green chemistry, including lowered energetic reaction requirements; catalytic, rather than stoichiometric, amounts of materials; increased selectivity; lowered consumption of processing and separation agents; and, in many cases, the use of less‐toxic compounds. Our research group has for a long time been studying methyltrioxorhenium in the oxyfunctionalization of different substrates, by using H2O2 or its urea‐hydrogen peroxide complex as the primary oxidant. In this Review paper we aim to provide a full literature account on the catalytic activity and selectivity of methyltrioxorhenium in the oxyfunctionalization reaction, either in nonconventional solvents or under solvent‐free conditions, with a particular emphasis on the use of ionic liquids as green reaction media. Oxyfunctionalization reactions with methyltrioxorhenium (MTO), one of the most‐studied organometallic rhenium derivatives, are the subject of this Review. A detailed account is given of the catalytic activity and selectivity of MTO in nonconventional solvents or under solvent‐free conditions, using H2O2 or urea‐hydrogen peroxide complex as primary oxidants.
AbstractList The requirement that chemical processes are sustainable, reflected in waste reduction and the use of safe reagents and reaction conditions, is becoming even more stringent as a result of pressure by society and governments to preserve the environment and protect human health. Catalysis offers numerous benefits related to green chemistry, including lowered energetic reaction requirements; catalytic, rather than stoichiometric, amounts of materials; increased selectivity; lowered consumption of processing and separation agents; and, in many cases, the use of less-toxic compounds. Our research group has for a long time been studying methyltrioxorhenium in the oxyfunctionalization of different substrates, by using H(2)O(2) or its urea-hydrogen peroxide complex as the primary oxidant. In this Review paper we aim to provide a full literature account on the catalytic activity and selectivity of methyltrioxorhenium in the oxyfunctionalization reaction, either in nonconventional solvents or under solvent-free conditions, with a particular emphasis on the use of ionic liquids as green reaction media.The requirement that chemical processes are sustainable, reflected in waste reduction and the use of safe reagents and reaction conditions, is becoming even more stringent as a result of pressure by society and governments to preserve the environment and protect human health. Catalysis offers numerous benefits related to green chemistry, including lowered energetic reaction requirements; catalytic, rather than stoichiometric, amounts of materials; increased selectivity; lowered consumption of processing and separation agents; and, in many cases, the use of less-toxic compounds. Our research group has for a long time been studying methyltrioxorhenium in the oxyfunctionalization of different substrates, by using H(2)O(2) or its urea-hydrogen peroxide complex as the primary oxidant. In this Review paper we aim to provide a full literature account on the catalytic activity and selectivity of methyltrioxorhenium in the oxyfunctionalization reaction, either in nonconventional solvents or under solvent-free conditions, with a particular emphasis on the use of ionic liquids as green reaction media.
The requirement that chemical processes are sustainable, reflected in waste reduction and the use of safe reagents and reaction conditions, is becoming even more stringent as a result of pressure by society and governments to preserve the environment and protect human health. Catalysis offers numerous benefits related to green chemistry, including lowered energetic reaction requirements; catalytic, rather than stoichiometric, amounts of materials; increased selectivity; lowered consumption of processing and separation agents; and, in many cases, the use of less-toxic compounds. Our research group has for a long time been studying methyltrioxorhenium in the oxyfunctionalization of different substrates, by using H(2)O(2) or its urea-hydrogen peroxide complex as the primary oxidant. In this Review paper we aim to provide a full literature account on the catalytic activity and selectivity of methyltrioxorhenium in the oxyfunctionalization reaction, either in nonconventional solvents or under solvent-free conditions, with a particular emphasis on the use of ionic liquids as green reaction media.
The requirement that chemical processes are sustainabable, reflected in waste reduction and the use of safe reagents and reaction conditions, is becoming even more stringent as a result of pressure by society and governments to preserve the environment and protect human health. Catalysis offers numerous benefits related to green chemistry, including lowered energetic reaction requirements; catalytic, rather than stoichiometric, amounts of materials; increased selectivity; lowered consumption of processing and separation agents; and, in many cases, the use of less‐toxic compounds. Our research group has for a long time been studying methyltrioxorhenium in the oxyfunctionalization of different substrates, by using H2O2 or its urea‐hydrogen peroxide complex as the primary oxidant. In this Review paper we aim to provide a full literature account on the catalytic activity and selectivity of methyltrioxorhenium in the oxyfunctionalization reaction, either in nonconventional solvents or under solvent‐free conditions, with a particular emphasis on the use of ionic liquids as green reaction media. Oxyfunctionalization reactions with methyltrioxorhenium (MTO), one of the most‐studied organometallic rhenium derivatives, are the subject of this Review. A detailed account is given of the catalytic activity and selectivity of MTO in nonconventional solvents or under solvent‐free conditions, using H2O2 or urea‐hydrogen peroxide complex as primary oxidants.
The requirement that chemical processes are sustainabable, reflected in waste reduction and the use of safe reagents and reaction conditions, is becoming even more stringent as a result of pressure by society and governments to preserve the environment and protect human health. Catalysis offers numerous benefits related to green chemistry, including lowered energetic reaction requirements; catalytic, rather than stoichiometric, amounts of materials; increased selectivity; lowered consumption of processing and separation agents; and, in many cases, the use of less‐toxic compounds. Our research group has for a long time been studying methyltrioxorhenium in the oxyfunctionalization of different substrates, by using H 2 O 2 or its urea‐hydrogen peroxide complex as the primary oxidant. In this Review paper we aim to provide a full literature account on the catalytic activity and selectivity of methyltrioxorhenium in the oxyfunctionalization reaction, either in nonconventional solvents or under solvent‐free conditions, with a particular emphasis on the use of ionic liquids as green reaction media.
Author De Angelis, Francesco
Crucianelli, Marcello
Saladino, Raffaele
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  surname: Crucianelli
  fullname: Crucianelli, Marcello
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  organization: Dipartimento di Chimica, Ingegneria Chimica e Materiali, Università dell'Aquila, Via Vetoio, 67100 L'Aquila (Italy), Fax: (+39) 0862-433753
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  surname: Saladino
  fullname: Saladino, Raffaele
  email: saladino@unitus.it
  organization: Dipartimento di Agrobiologia ed Agrochimica, Università della Tuscia, Via S. Camillo de Lellis, 01100 Viterbo (Italy), Fax: (+39) 0761-357242
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  givenname: Francesco
  surname: De Angelis
  fullname: De Angelis, Francesco
  organization: Dipartimento di Chimica, Ingegneria Chimica e Materiali, Università dell'Aquila, Via Vetoio, 67100 L'Aquila (Italy), Fax: (+39) 0862-433753
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2005; 690
1991; 113
1997; 119
2005; 296
2006; 79
1995; 34
2000; 41
2003; 59
1972
1998; 555
1999; 40
2005; 61
1996; 35
2004; 689
2007; 333
1988 1988; 100 27
2006; 62
2000
2002; 187
1997; 97
2002; 102
2000; 55
1993; 32
2002; 43
2007; 692
1996; 61
2007; 9
1994; 33
1999; 99
2009; 360
2007; 5
2007; 63
2008; 64
2008; 350
2008; 151
2003; 44
1992; 4
1979; 18
1994; 116
1989; 372
2000; 65
2002; 35
1997; 68
2006; 14
2004; 45
2002; 8
1998
1995; 117
2008
2009; 694
1997
2007
2005
2000; 153
2003
1999; 145
2008; 51
2007; 10
1996; 15
2008; 284
2005; 46
1999
1994; 86
2009; 28
1998; 37
2009; 73
2006; 40
2007; 270
2002; 67
1996 1996; 108 35
1999; 399
2009; 6
1993 1993; 105 32
2008; 257
2008; 42
2007 2007; 119 46
2005; 16
2006; 348
2005; 18
2008 2001; 3 3
1996; 118
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Anastas P. T. (e_1_2_9_4_2) 1998
Anastas P. T. (e_1_2_9_83_2) 1998
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– start-page: 1
  volume-title: Green Chemistry: Frontiers in Benign Chemical Synthesis and Process
  year: 1998
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Snippet The requirement that chemical processes are sustainabable, reflected in waste reduction and the use of safe reagents and reaction conditions, is becoming even...
The requirement that chemical processes are sustainable, reflected in waste reduction and the use of safe reagents and reaction conditions, is becoming even...
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SubjectTerms Catalysis
Green Chemistry Technology - methods
ionic liquids
Ionic Liquids - chemistry
Organometallic Compounds - chemistry
oxidation
Oxidation-Reduction
rhenium
Solvents - chemistry
sustainable chemistry
Title Methyltrioxorhenium Catalysis in Nonconventional Solvents: A Great Catalyst in a Safe Reaction Medium
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https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fcssc.201000022
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