Metal-organic frameworks as heterogeneous photocatalysts: advantages and challenges
The use of metal organic frameworks (MOFs) as heterogeneous photocatalysts is critically reviewed. First we revisit the general assumption of MOFs behaving truly as semiconductors, demonstrating that such semiconducting behaviour only occurs in a very limited subset of materials. Further, the main a...
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| Published in | CrystEngComm Vol. 16; no. 23; pp. 4919 - 4926 |
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| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
| Published |
01.01.2014
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| Subjects | |
| Online Access | Get full text |
| ISSN | 1466-8033 1466-8033 |
| DOI | 10.1039/c4ce00032c |
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| Abstract | The use of metal organic frameworks (MOFs) as heterogeneous photocatalysts is critically reviewed. First we revisit the general assumption of MOFs behaving truly as semiconductors, demonstrating that such semiconducting behaviour only occurs in a very limited subset of materials. Further, the main approaches for efficient light harvesting and active site engineering in MOF-based photocatalysts are discussed. Finally, the main advantages of MOFs as photocatalysts and the challenges that need to be addressed in order to improve catalytic performance are evaluated.
The use of metal organic frameworks as photocatalysts is critically reviewed and their main advantages and challenges are evaluated. |
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| AbstractList | The use of metal organic frameworks (MOFs) as heterogeneous photocatalysts is critically reviewed. First we revisit the general assumption of MOFs behaving truly as semiconductors, demonstrating that such semiconducting behaviour only occurs in a very limited subset of materials. Further, the main approaches for efficient light harvesting and active site engineering in MOF-based photocatalysts are discussed. Finally, the main advantages of MOFs as photocatalysts and the challenges that need to be addressed in order to improve catalytic performance are evaluated. The use of metal organic frameworks (MOFs) as heterogeneous photocatalysts is critically reviewed. First we revisit the general assumption of MOFs behaving truly as semiconductors, demonstrating that such semiconducting behaviour only occurs in a very limited subset of materials. Further, the main approaches for efficient light harvesting and active site engineering in MOF-based photocatalysts are discussed. Finally, the main advantages of MOFs as photocatalysts and the challenges that need to be addressed in order to improve catalytic performance are evaluated. The use of metal organic frameworks as photocatalysts is critically reviewed and their main advantages and challenges are evaluated. |
| Author | van der Veen, M Nasalevich, M. A Gascon, J Kapteijn, F |
| AuthorAffiliation | Catalysis Engineering Department of Chemical Engineering Delft University of Technology |
| AuthorAffiliation_xml | – name: Department of Chemical Engineering – name: Catalysis Engineering – name: Delft University of Technology |
| Author_xml | – sequence: 1 givenname: M. A surname: Nasalevich fullname: Nasalevich, M. A – sequence: 2 givenname: M surname: van der Veen fullname: van der Veen, M – sequence: 3 givenname: F surname: Kapteijn fullname: Kapteijn, F – sequence: 4 givenname: J surname: Gascon fullname: Gascon, J |
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| Snippet | The use of metal organic frameworks (MOFs) as heterogeneous photocatalysts is critically reviewed. First we revisit the general assumption of MOFs behaving... |
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| SubjectTerms | Catalysis Catalysts Harvesting Metal-organic frameworks Performance enhancement Performance evaluation Photocatalysis Photocatalysts Semiconductors |
| Title | Metal-organic frameworks as heterogeneous photocatalysts: advantages and challenges |
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