Application of carbon materials in redox flow batteries

The redox flow battery (RFB) has been the subject of state-of-the-art research by several groups around the world. Most work commonly involves the application of various low-cost carbon-polymer composites, carbon felts, cloth, paper and their different variations for the electrode materials of the R...

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Published inJournal of power sources Vol. 253; pp. 150 - 166
Main Authors Chakrabarti, M.H., Brandon, N.P., Hajimolana, S.A., Tariq, F., Yufit, V., Hashim, M.A., Hussain, M.A., Low, C.T.J., Aravind, P.V.
Format Journal Article
LanguageEnglish
Published Amsterdam Elsevier B.V 01.05.2014
Elsevier
Subjects
Applied sciences
Carbon
Carbon-based electrodes
Cloth
Corrosion
Direct energy conversion and energy accumulation
Electric batteries
Electrical engineering. Electrical power engineering
Electrical power engineering
Electrical resistivity
Electrochemical conversion: primary and secondary batteries, fuel cells
Electrodes
Exact sciences and technology
Failure
Graphene
Nanostructure
Nanotechnology
Redox flow battery
X-ray tomography
X-ray tomography
Carbon-based electrodes
Graphene
Nanotechnology
Redox flow battery
Material flow
X ray radiography
Carbon electrode
Secondary cell
X Ray tomography
Application
Carbon
Online AccessGet full text

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Abstract The redox flow battery (RFB) has been the subject of state-of-the-art research by several groups around the world. Most work commonly involves the application of various low-cost carbon-polymer composites, carbon felts, cloth, paper and their different variations for the electrode materials of the RFB. Usually, the carbon-polymer composite electrode has relatively high bulk resistivity and can be easily corroded when the polarised potential on the anode is more positive than that of oxygen evolution and this kind of heterogeneous corrosion may lead to battery failure due to electrolyte leakage. Therefore, carbon electrodes with high electrical conductivity, acid-resistance and electrochemical stability are highly desirable. This review discusses such issues in depth and presents an overview on future research directions that may help commercialise RFB technology. A comprehensive discussion is provided on the advances made using nanotechnology and it is envisaged that if this is combined with ionic liquid technology, major advantages could be realised. In addition the identification of RFB failure mechanisms by means of X-ray computed nano tomography is expected to bring added benefits to the technology. •A comprehensive coverage on carbon materials used in redox flow batteries is given.•The influence of nanotechnology and graphene is discussed in detail.•The importance of studying RFB degradation mechanisms is emphasised.
AbstractList The redox flow battery (RFB) has been the subject of state-of-the-art research by several groups around the world. Most work commonly involves the application of various low-cost carbon-polymer composites, carbon felts, cloth, paper and their different variations for the electrode materials of the RFB. Usually, the carbon-polymer composite electrode has relatively high bulk resistivity and can be easily corroded when the polarised potential on the anode is more positive than that of oxygen evolution and this kind of heterogeneous corrosion may lead to battery failure due to electrolyte leakage. Therefore, carbon electrodes with high electrical conductivity, acid-resistance and electrochemical stability are highly desirable. This review discusses such issues in depth and presents an overview on future research directions that may help commercialise RFB technology. A comprehensive discussion is provided on the advances made using nanotechnology and it is envisaged that if this is combined with ionic liquid technology, major advantages could be realised. In addition the identification of RFB failure mechanisms by means of X-ray computed nano tomography is expected to bring added benefits to the technology.
The redox flow battery (RFB) has been the subject of state-of-the-art research by several groups around the world. Most work commonly involves the application of various low-cost carbon-polymer composites, carbon felts, cloth, paper and their different variations for the electrode materials of the RFB. Usually, the carbon-polymer composite electrode has relatively high bulk resistivity and can be easily corroded when the polarised potential on the anode is more positive than that of oxygen evolution and this kind of heterogeneous corrosion may lead to battery failure due to electrolyte leakage. Therefore, carbon electrodes with high electrical conductivity, acid-resistance and electrochemical stability are highly desirable. This review discusses such issues in depth and presents an overview on future research directions that may help commercialise RFB technology. A comprehensive discussion is provided on the advances made using nanotechnology and it is envisaged that if this is combined with ionic liquid technology, major advantages could be realised. In addition the identification of RFB failure mechanisms by means of X-ray computed nano tomography is expected to bring added benefits to the technology. •A comprehensive coverage on carbon materials used in redox flow batteries is given.•The influence of nanotechnology and graphene is discussed in detail.•The importance of studying RFB degradation mechanisms is emphasised.
Author Hajimolana, S.A.
Yufit, V.
Aravind, P.V.
Hashim, M.A.
Chakrabarti, M.H.
Brandon, N.P.
Low, C.T.J.
Hussain, M.A.
Tariq, F.
Author_xml – sequence: 1
  givenname: M.H.
  surname: Chakrabarti
  fullname: Chakrabarti, M.H.
  email: mohammedharun77@yahoo.com, harun_chakrabarti@hotmail.com
  organization: Department of Chemical Engineering, Faculty of Engineering, University of Malaya, Kuala Lumpur 50603, Malaysia
– sequence: 2
  givenname: N.P.
  surname: Brandon
  fullname: Brandon, N.P.
  organization: Department of Earth Science and Engineering, Imperial College London, South Kensington, London SW7 2AZ, UK
– sequence: 3
  givenname: S.A.
  surname: Hajimolana
  fullname: Hajimolana, S.A.
  organization: Department of Chemical Engineering, Faculty of Engineering, University of Malaya, Kuala Lumpur 50603, Malaysia
– sequence: 4
  givenname: F.
  surname: Tariq
  fullname: Tariq, F.
  organization: Department of Earth Science and Engineering, Imperial College London, South Kensington, London SW7 2AZ, UK
– sequence: 5
  givenname: V.
  surname: Yufit
  fullname: Yufit, V.
  organization: Department of Earth Science and Engineering, Imperial College London, South Kensington, London SW7 2AZ, UK
– sequence: 6
  givenname: M.A.
  surname: Hashim
  fullname: Hashim, M.A.
  organization: Department of Chemical Engineering, Faculty of Engineering, University of Malaya, Kuala Lumpur 50603, Malaysia
– sequence: 7
  givenname: M.A.
  surname: Hussain
  fullname: Hussain, M.A.
  organization: Department of Chemical Engineering, Faculty of Engineering, University of Malaya, Kuala Lumpur 50603, Malaysia
– sequence: 8
  givenname: C.T.J.
  surname: Low
  fullname: Low, C.T.J.
  organization: Electrochemical Engineering Laboratory, Energy Technology Research Group, Faculty of Engineering and the Environment, University of Southampton, Highfield, Southampton SO17 1BJ, UK
– sequence: 9
  givenname: P.V.
  surname: Aravind
  fullname: Aravind, P.V.
  organization: Process and Energy Department, Delft University of Technology, Leeghwaterstraat 44, CA Delft 2628, The Netherlands
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Keywords X-ray tomography
Carbon-based electrodes
Graphene
Nanotechnology
Redox flow battery
Material flow
X ray radiography
Carbon electrode
Secondary cell
X Ray tomography
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Carbon
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Snippet The redox flow battery (RFB) has been the subject of state-of-the-art research by several groups around the world. Most work commonly involves the application...
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SubjectTerms Applied sciences
Carbon
Carbon-based electrodes
Cloth
Corrosion
Direct energy conversion and energy accumulation
Electric batteries
Electrical engineering. Electrical power engineering
Electrical power engineering
Electrical resistivity
Electrochemical conversion: primary and secondary batteries, fuel cells
Electrodes
Exact sciences and technology
Failure
Graphene
Nanostructure
Nanotechnology
Redox flow battery
X-ray tomography
Title Application of carbon materials in redox flow batteries
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