Ultra-Microporous Triptycene-based Polyimide Membranes for High-Performance Gas Separation
A highly permeable and highly selective polyimide of intrinsic microporosity is prepared using a 9,10‐diisopropyl‐triptycene contortion center. The three‐dimensionality and shape‐persistence of triptycene afford exceptional sieving‐based gas separation performance transcending the latest permeabilit...
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| Published in | Advanced materials (Weinheim) Vol. 26; no. 22; pp. 3688 - 3692 |
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| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
| Published |
Germany
Blackwell Publishing Ltd
11.06.2014
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| Subjects | |
| Online Access | Get full text |
| ISSN | 0935-9648 1521-4095 1521-4095 |
| DOI | 10.1002/adma.201306229 |
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| Abstract | A highly permeable and highly selective polyimide of intrinsic microporosity is prepared using a 9,10‐diisopropyl‐triptycene contortion center. The three‐dimensionality and shape‐persistence of triptycene afford exceptional sieving‐based gas separation performance transcending the latest permeability/selectivity trade‐offs for industrial gas separations involving oxygen and hydrogen. |
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| AbstractList | A highly permeable and highly selective polyimide of intrinsic microporosity is prepared using a 9,10-diisopropyl-triptycene contortion center. The three-dimensionality and shape-persistence of triptycene afford exceptional sieving-based gas separation performance transcending the latest permeability/selectivity trade-offs for industrial gas separations involving oxygen and hydrogen. |
| Author | Ghanem, Bader S. Swaidan, Raja Pinnau, Ingo Litwiller, Eric |
| Author_xml | – sequence: 1 givenname: Bader S. surname: Ghanem fullname: Ghanem, Bader S. organization: Advanced Membranes and Porous Materials Center, Physical Sciences and Engineering Division, King Abdullah University of Science and Technology (KAUST), Al-Jazri Building, KSA, 23955-6900, Thuwal – sequence: 2 givenname: Raja surname: Swaidan fullname: Swaidan, Raja organization: Advanced Membranes and Porous Materials Center, Physical Sciences and Engineering Division, King Abdullah University of Science and Technology (KAUST), Al-Jazri Building, KSA, 23955-6900, Thuwal – sequence: 3 givenname: Eric surname: Litwiller fullname: Litwiller, Eric organization: Advanced Membranes and Porous Materials Center, Physical Sciences and Engineering Division, King Abdullah University of Science and Technology (KAUST), Al-Jazri Building, KSA, 23955-6900, Thuwal – sequence: 4 givenname: Ingo surname: Pinnau fullname: Pinnau, Ingo email: Ingo.Pinnau@kaust.edu.sa organization: Advanced Membranes and Porous Materials Center, Physical Sciences and Engineering Division, King Abdullah University of Science and Technology (KAUST), Al-Jazri Building, KSA, 23955-6900, Thuwal |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/24619501$$D View this record in MEDLINE/PubMed |
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| Copyright | 2014 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim |
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| Issue | 22 |
| Keywords | intrinsic microporosity polyimide gas separations triptycene molecular sieving |
| Language | English |
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| References_xml | – reference: N. T. Tsui, A. J. Paraskos, L. Torun, T. M. Swager, E. L. Thomas, Macromolecules 2006, 39, 3350. – reference: b) N. B. McKeown, P. M. Budd, D. Book, Macromol. Rapid Comm. 2007, 28, 995. – reference: M. Carta, R. Malpass-Evans, M. Croad, Y. Rogan, J. C. Jansen, P. Bernardo, F. Bazzarelli, N. B. McKeown, Science 2013, 339, 303. – reference: Y. J. Cho, H. B. Park, Macromol. Rapid Comm. 2011, 32, 579. – reference: T. M. Swager, Accounts Chem. Res. 2008, 41, 1181. – reference: M. Ghosh, K. L. Mittal, Polyimides: fundamentals and applications, Marcel Dekker, New York USA 1996. – reference: Q. S. Zong, C. F. Chen, Org. Lett. 2006, 8, 211. – reference: N. Ritter, I. Senkovska, S. Kaskel, J. Weber, Macromolecules 2011, 44, 2025. – reference: b) P. M. Budd, B. S. Ghanem, S. Makhseed, N. B. McKeown, K. J. Msayib, C. E. Tattershall, Chem. Commun. 2004, 2, 230. – reference: C. Zhang, Y. Liu, B. Y. Li, B. Tan, C. F. Chen, H. B. Xu, X. L. 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| Snippet | A highly permeable and highly selective polyimide of intrinsic microporosity is prepared using a 9,10‐diisopropyl‐triptycene contortion center. The... A highly permeable and highly selective polyimide of intrinsic microporosity is prepared using a 9,10-diisopropyl-triptycene contortion center. The... |
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| SubjectTerms | Gas separation gas separations intrinsic microporosity Materials selection Membranes Microporosity molecular sieving Permeability polyimide Polyimide resins Selectivity Tradeoffs triptycene |
| Title | Ultra-Microporous Triptycene-based Polyimide Membranes for High-Performance Gas Separation |
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