Ternary Sulfur/Polyacrylonitrile/SiO₂ Composite Cathodes for High-Performance Sulfur/Lithium Ion Full Batteries
In the present study, a novel sulfur/lithium-ion full battery was assembled while using ternary sulfur/polyacrylonitrile/SiO₂ (S/PAN/SiO₂) composite as the cathode and prelithiated graphite as the anode. For anode, Stabilized Lithium Metal Powder (SLMP) was successfully transformed into lithiated gr...
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Published in | Polymers Vol. 10; no. 8; p. 930 |
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Language | English |
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Abstract | In the present study, a novel sulfur/lithium-ion full battery was assembled while using ternary sulfur/polyacrylonitrile/SiO₂ (S/PAN/SiO₂) composite as the cathode and prelithiated graphite as the anode. For anode, Stabilized Lithium Metal Powder (SLMP) was successfully transformed into lithiated graphite anode. For cathode, scanning electron microscopy (SEM) and transmission electron microscopy (TEM) revealed that SiO₂ was uniformly distributed on S/PAN composites, where SiO₂ served as an effective additive due to its ultra high absorb ability and enhanced ability in trapping soluble polysulfide. The tested half-cell based on S/PAN/SiO₂ composite revealed high discharge capacity of 1106 mAh g
after 100 cycles at 0.2 C. The full cell based on prelithiated graphite//S/PAN/SiO₂ composite system delivered a specific capacity of 810 mAh g
over 100 cycles. |
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AbstractList | In the present study, a novel sulfur/lithium-ion full battery was assembled while using ternary sulfur/polyacrylonitrile/SiO2 (S/PAN/SiO2) composite as the cathode and prelithiated graphite as the anode. For anode, Stabilized Lithium Metal Powder (SLMP) was successfully transformed into lithiated graphite anode. For cathode, scanning electron microscopy (SEM) and transmission electron microscopy (TEM) revealed that SiO2 was uniformly distributed on S/PAN composites, where SiO2 served as an effective additive due to its ultra high absorb ability and enhanced ability in trapping soluble polysulfide. The tested half-cell based on S/PAN/SiO2 composite revealed high discharge capacity of 1106 mAh g−1 after 100 cycles at 0.2 C. The full cell based on prelithiated graphite//S/PAN/SiO2 composite system delivered a specific capacity of 810 mAh g−1 over 100 cycles. In the present study, a novel sulfur/lithium-ion full battery was assembled while using ternary sulfur/polyacrylonitrile/SiO 2 (S/PAN/SiO 2 ) composite as the cathode and prelithiated graphite as the anode. For anode, Stabilized Lithium Metal Powder (SLMP) was successfully transformed into lithiated graphite anode. For cathode, scanning electron microscopy (SEM) and transmission electron microscopy (TEM) revealed that SiO 2 was uniformly distributed on S/PAN composites, where SiO 2 served as an effective additive due to its ultra high absorb ability and enhanced ability in trapping soluble polysulfide. The tested half-cell based on S/PAN/SiO 2 composite revealed high discharge capacity of 1106 mAh g −1 after 100 cycles at 0.2 C. The full cell based on prelithiated graphite//S/PAN/SiO 2 composite system delivered a specific capacity of 810 mAh g −1 over 100 cycles. In the present study, a novel sulfur/lithium-ion full battery was assembled while using ternary sulfur/polyacrylonitrile/SiO₂ (S/PAN/SiO₂) composite as the cathode and prelithiated graphite as the anode. For anode, Stabilized Lithium Metal Powder (SLMP) was successfully transformed into lithiated graphite anode. For cathode, scanning electron microscopy (SEM) and transmission electron microscopy (TEM) revealed that SiO₂ was uniformly distributed on S/PAN composites, where SiO₂ served as an effective additive due to its ultra high absorb ability and enhanced ability in trapping soluble polysulfide. The tested half-cell based on S/PAN/SiO₂ composite revealed high discharge capacity of 1106 mAh g after 100 cycles at 0.2 C. The full cell based on prelithiated graphite//S/PAN/SiO₂ composite system delivered a specific capacity of 810 mAh g over 100 cycles. |
Author | Tan, Taizhe Chen, Zhihong Zhang, Yongguang Shan, Zhenzhen He, Yusen |
AuthorAffiliation | 1 School of Materials Science and Engineering, Hebei University of Technology, Tianjin 300130, China; hyshebut@163.com (Y.H.); shanzhenzhenhebut@163.com (Z.S.) 2 Synergy Innovation Institute of GDUT, Heyuan 517000, China; taizhetan@gdut.edu.cn 3 Shenyang Institute of Automation, Chinese Academy of Sciences, Guangzhou 511458, China |
AuthorAffiliation_xml | – name: 3 Shenyang Institute of Automation, Chinese Academy of Sciences, Guangzhou 511458, China – name: 1 School of Materials Science and Engineering, Hebei University of Technology, Tianjin 300130, China; hyshebut@163.com (Y.H.); shanzhenzhenhebut@163.com (Z.S.) – name: 2 Synergy Innovation Institute of GDUT, Heyuan 517000, China; taizhetan@gdut.edu.cn |
Author_xml | – sequence: 1 givenname: Yusen surname: He fullname: He, Yusen email: hyshebut@163.com organization: School of Materials Science and Engineering, Hebei University of Technology, Tianjin 300130, China. hyshebut@163.com – sequence: 2 givenname: Zhenzhen surname: Shan fullname: Shan, Zhenzhen email: shanzhenzhenhebut@163.com organization: School of Materials Science and Engineering, Hebei University of Technology, Tianjin 300130, China. shanzhenzhenhebut@163.com – sequence: 3 givenname: Taizhe surname: Tan fullname: Tan, Taizhe email: taizhetan@gdut.edu.cn organization: Synergy Innovation Institute of GDUT, Heyuan 517000, China. taizhetan@gdut.edu.cn – sequence: 4 givenname: Zhihong surname: Chen fullname: Chen, Zhihong email: chenzhihong1227@sina.com organization: Shenyang Institute of Automation, Chinese Academy of Sciences, Guangzhou 511458, China. chenzhihong1227@sina.com – sequence: 5 givenname: Yongguang surname: Zhang fullname: Zhang, Yongguang email: yongguangzhang@hebut.edu.cn organization: School of Materials Science and Engineering, Hebei University of Technology, Tianjin 300130, China. yongguangzhang@hebut.edu.cn |
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Keywords | ternary sulfur/polyacrylonitrile/SiO2 composite sulfur/lithium-ion full battery prelithiated graphite anode stabilized lithium metal powder electrochemical performance |
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Snippet | In the present study, a novel sulfur/lithium-ion full battery was assembled while using ternary sulfur/polyacrylonitrile/SiO₂ (S/PAN/SiO₂) composite as the... In the present study, a novel sulfur/lithium-ion full battery was assembled while using ternary sulfur/polyacrylonitrile/SiO2 (S/PAN/SiO2) composite as the... In the present study, a novel sulfur/lithium-ion full battery was assembled while using ternary sulfur/polyacrylonitrile/SiO 2 (S/PAN/SiO 2 ) composite as the... |
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SubjectTerms | Additives Anodes Carbon Cathodes electrochemical performance Electrodes Electrolytes Energy Fourier transforms Graphite Lithium Lithium ions Metal powders Microscopy Morphology Polyacrylonitrile prelithiated graphite anode Rechargeable batteries Scanning electron microscopy Silicon dioxide Spectrum analysis stabilized lithium metal powder Sulfur sulfur/lithium-ion full battery ternary sulfur/polyacrylonitrile/SiO2 composite Transmission electron microscopy |
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Title | Ternary Sulfur/Polyacrylonitrile/SiO₂ Composite Cathodes for High-Performance Sulfur/Lithium Ion Full Batteries |
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