CO2 Sequestration Through Aqueous Carbonation of Electric Arc Furnace Slag
Electric Arc Furnace slag (EAF slag) reuse is currently limited by its inconsistent chemical composition and volume instability. However, the alkaline composition suggests the possibility to use this material for carbon capture and storage. This study investigated the CO2 uptake of EAF slag using a...
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| Published in | Journal of Advanced Concrete Technology Vol. 22; no. 4; pp. 207 - 218 |
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| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Tokyo
Japan Concrete Institute
12.04.2024
Japan Science and Technology Agency |
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| Abstract | Electric Arc Furnace slag (EAF slag) reuse is currently limited by its inconsistent chemical composition and volume instability. However, the alkaline composition suggests the possibility to use this material for carbon capture and storage. This study investigated the CO2 uptake of EAF slag using a direct aqueous carbonation technique. The process was implemented at room temperature and ambient pressure, with minimized energy consumption. The CO2-reactive phases were identified through X-ray diffraction analysis. Different CO2 quantification techniques were employed: thermogravimetric analysis, acid digestion and thermal decomposition. The replicability of experiments and quantification techniques was assessed through analysis of variance and pairwise comparisons. The average CO2 uptake and coefficient of variation resulted respectively 7.9% and 9.0%, with a carbonation degree of about 34%, proving that this simple mineralization process can be promising even in mild conditions. |
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| AbstractList | Electric Arc Furnace slag (EAF slag) reuse is currently limited by its inconsistent chemical composition and volume instability. However, the alkaline composition suggests the possibility to use this material for carbon capture and storage. This study investigated the CO2 uptake of EAF slag using a direct aqueous carbonation technique. The process was implemented at room temperature and ambient pressure, with minimized energy consumption. The CO2-reactive phases were identified through X-ray diffraction analysis. Different CO2 quantification techniques were employed: thermogravimetric analysis, acid digestion and thermal decomposition. The replicability of experiments and quantification techniques was assessed through analysis of variance and pairwise comparisons. The average CO2 uptake and coefficient of variation resulted respectively 7.9% and 9.0%, with a carbonation degree of about 34%, proving that this simple mineralization process can be promising even in mild conditions. |
| Author | Palmero, Paola Humbert, Pedro Bonfante, Francesca Tulliani, Jean-Marc Christian Garufi, Davide Ferrara, Giuseppe |
| Author_xml | – sequence: 1 fullname: Bonfante, Francesca organization: Department of Applied Science and Technology (DISAT), INSTM R.U. Lince Laboratory, Politecnico di Torino, Turin 10129, Italy – sequence: 2 fullname: Ferrara, Giuseppe organization: Department of Applied Science and Technology (DISAT), INSTM R.U. Lince Laboratory, Politecnico di Torino, Turin 10129, Italy – sequence: 3 fullname: Humbert, Pedro organization: Innovation Centre for Sustainable Construction, CRH, Amsterdam, 1083 HL, The Netherlands – sequence: 4 fullname: Garufi, Davide organization: Innovation Centre for Sustainable Construction, CRH, Amsterdam, 1083 HL, The Netherlands – sequence: 5 fullname: Tulliani, Jean-Marc Christian organization: Department of Applied Science and Technology (DISAT), INSTM R.U. Lince Laboratory, Politecnico di Torino, Turin 10129, Italy – sequence: 6 fullname: Palmero, Paola organization: Department of Applied Science and Technology (DISAT), INSTM R.U. Lince Laboratory, Politecnico di Torino, Turin 10129, Italy |
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A. and Ortega-López, V., (2017). “EAF slag in asphalt mixes: A brief review of its possible re-use.” Resources, Conservation and Recycling, 120, 176-185. 18) Huntzinger, D. N., Gierke, J. S., Sutter, L. L., Kawatra, S. K. and Eisele, T. C., (2009). “Carbon dioxide sequestration in cement kiln dust through mineral carbonation.” Environmental Science and Technology, 43(6), 1986-1992. 47) Zhang, Y., Yu, L., Cui, K., Wang, H. and Fu, T., (2023). “Carbon capture and storage technology by steel-making slags: Recent progress and future challenges.” Chemical Engineering Journal, 455, 140552. 35) RILEM, (2022). “Technical Committee 309-MCP on accelerated mineral carbonation for the production of construction materials [online].” Paris, Réunion Internationale des Laboratoires et Experts des Matériaux, Systèmes de Construction et Ouvrages (RILEM). 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| References_xml | – reference: 4) Bonenfant, D., Kharoune, L., Sauvé, S., Hausler, R., Niquette, P., Mimeault, M. and Kharoune, M., (2008). “CO2 sequestration potential of steel slags at ambient pressure and temperature.” Industrial and Engineering Chemistry Research, 47(20), 7610-7616. – reference: 29) Mo, L., Zhang, F. and Deng, M., (2016). “Mechanical performance and microstructure of the calcium carbonate binders produced by carbonating steel slag paste under CO2 curing.” Cement and Concrete Research, 88, 217-226. – reference: 47) Zhang, Y., Yu, L., Cui, K., Wang, H. and Fu, T., (2023). “Carbon capture and storage technology by steel-making slags: Recent progress and future challenges.” Chemical Engineering Journal, 455, 140552. – reference: 13) Ghacham, A. B., Pasquier, L.-C., Cecchi, E., Blais, J.-F. and Mercier, G., (2017). “Valorization of waste concrete through CO2 mineral carbonation: Optimizing parameters and improving reactivity using concrete separation.” Journal of Cleaner Production, 166, 869-878. – reference: 21) IEA, (2021). “Net zero by 2050.” Paris: International Energy Agency (IEA). – reference: 43) WSA, (2010). “Steel industry co-products [online].” Brussels, World Steel Association (WSA). Available from: <https://worldsteel.org/steel-topics/environment-climate-change/steel-industry-co-products/ > [Accessed 28 September 2023]. – reference: 10) Fang, Y., Su, W., Zhang, Y., Zhang, M., Ding, X. and Wang, Q., (2022). “Effect of accelerated precarbonation on hydration activity and volume stability of steel slag as a supplementary cementitious material.” Journal of Thermal Analysis and Calorimetry, 147(11), 6181-6191. – reference: 14) Gobetti, A., Cornacchia, G. and Ramorino, G., (2022). “Reuse of electric arc furnace slag as filler for nitrile butadiene rubber.” JOM, 74(4), 1329-1339. – reference: 17) Humbert, P. S., Castro-Gomes, J. P. and Savastano, H., (2019). “Clinker-free CO2 cured steel slag based binder: Optimal conditions and potential applications.” Construction and Building Materials, 210, 413-421. – reference: 3) Baciocchi, R., Costa, G., Di Gianfilippo, M., Pollettini, A. and Pomi, R., (2011). “Wet versus slurry carbonation of EAF steel slag.” Greenhouse Gases: Science and Technology, 1(4), 312-319. – reference: 37) Steinour, H. H., (1959). “Some effects of carbon dioxide on mortars and concrete-discussion.” Journal of the American Concrete Institute, 30(2), 905-907. – reference: 26) Mahoutian, M., Chaallal, O. and Shao, Y., (2018). “Pilot production of steel slag masonry blocks.” Canadian Journal of Civil Engineering, 45(7), 537-546. – reference: 36) Skaf, M., Manso, J. M., Aragón, Á., Fuente-Alonso, J. A. and Ortega-López, V., (2017). “EAF slag in asphalt mixes: A brief review of its possible re-use.” Resources, Conservation and Recycling, 120, 176-185. – reference: 15) Huijgen, W. J. J. and Comans, R. N. J., (2006). “Carbonation of steel slag for CO2 sequestration: Leaching of products and reaction mechanisms.” Environmental Science and Technology, 40(8), 2790-2796. – reference: 32) Pan, S. Y., Chiang, P. C., Chen, Y. H., Tan, C. S. and Chang, E. E., (2014). “Kinetics of carbonation reaction of basic oxygen furnace slags in a rotating packed bed using the surface coverage model: Maximization of carbonation conversion.” Applied Energy, 113, 267-276. – reference: 25) Liu, G., Schollbach, K., van der Laan, S., Tang, P. and Florea, M. V. A., (2020). “Recycling and utilization of high volume converter steel slag into CO2 activated mortars - The role of slag particle size.” Resources, Conservation and Recycling, 160, 104883. – reference: 40) Unluer, C. and Al-Tabbaa, A., (2013). “Impact of hydrated magnesium carbonate additives on the carbonation of reactive MgO cements.” Cement and Concrete Research, 54, 87-97. – reference: 30) Moon, E. J. and Choi, Y. C., (2018). “Development of carbon-capture binder using stainless steel argon oxygen decarburization slag activated by carbonation.” Journal of Cleaner Production, 180, 642-654. – reference: 46) Zhang, D., Ghouleh, Z. and Shao, Y., (2017). “Review on carbonation curing of cement-based materials.” Journal of CO2 Utilization, 21, 119-131. – reference: 1) Baciocchi, R., Costa, G., Di Bartolomeo, E., Pollettini, A. and Pomi, R., (2010). “Carbonation of stainless steel slag as a process for CO2 storage and slag valorization.” Waste and Biomass Valorization, 1(4), 467-477. – reference: 44) WSA, (2019). “World steel in figures 2019.” Brussels, World Steel Association (WSA). Available from: <https://worldsteel.org/wp-content/uploads/2019-World-Steel-in-Figures.pdf?x82173 > [Accessed 4 October 2022]. – reference: 16) Huijgen, W. J. J., Witkamp, G. J. and Comans, R. N. J., (2005). “Mineral CO2 sequestration by steel slag carbonation.” Environmental Science and Technology, 39(24), 9676-9682. – reference: 18) Huntzinger, D. N., Gierke, J. S., Sutter, L. L., Kawatra, S. K. and Eisele, T. C., (2009). “Carbon dioxide sequestration in cement kiln dust through mineral carbonation.” Environmental Science and Technology, 43(6), 1986-1992. – reference: 22) Juckes, L. M., (2003). “The volume stability of modern steelmaking slags.” Mineral Processing and Extractive Metallurgy. 112, 177-197. – reference: 11) Ferrara, G., Belli, A., Keulen, A., Tulliani, J. C. and Palmero, P., (2023). “Testing procedures for CO2 uptake assessment of accelerated carbonation products: Experimental application on basic oxygen furnace steel slag samples.” Construction and Building Materials, 406, 133384. – reference: 12) Ghacham, A. 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| Snippet | Electric Arc Furnace slag (EAF slag) reuse is currently limited by its inconsistent chemical composition and volume instability. However, the alkaline... |
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| SubjectTerms | Acid digestion Carbon dioxide Carbon sequestration Carbonation Chemical composition Coefficient of variation Electric arc furnaces Energy consumption Pressure Room temperature Slag Thermal decomposition Thermogravimetric analysis Variance analysis |
| Title | CO2 Sequestration Through Aqueous Carbonation of Electric Arc Furnace Slag |
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