Highly ordered ultralong magnetic nanowires wrapped in stacked graphene layers

We report on the synthesis and magnetic characterization of ultralong (1 cm) arrays of highly ordered coaxial nanowires with nickel cores and graphene stacking shells (also known as metal-filled carbon nanotubes). Carbon-containing nickel nanowires are first grown on a nanograted surface by magnetro...

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Published inBeilstein journal of nanotechnology Vol. 3; no. 1; pp. 846 - 851
Main Authors El Mel, Abdel-Aziz, Duvail, Jean-Luc, Gautron, Eric, Xu, Wei, Choi, Chang-Hwan, Angleraud, Benoit, Granier, Agnès, Tessier, Pierre-Yves
Format Journal Article
LanguageEnglish
Published Germany Karlsruhe Institute of Technology 2012
Beilstein-Institut
Subjects
carbon
Condensed Matter
ferromagnetic
graphene
Letter
Materials Science
nanofabrication
Nanoscience
Nanotechnology
nanowires
nickel
phase separation
Physics
nickel
phase separation
ferromagnetic
nanowires
carbon
nanofabrication
graphene
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Abstract We report on the synthesis and magnetic characterization of ultralong (1 cm) arrays of highly ordered coaxial nanowires with nickel cores and graphene stacking shells (also known as metal-filled carbon nanotubes). Carbon-containing nickel nanowires are first grown on a nanograted surface by magnetron sputtering. Then, a post-annealing treatment favors the metal-catalyzed crystallization of carbon into stacked graphene layers rolled around the nickel cores. The observed uniaxial magnetic anisotropy field oriented along the nanowire axis is an indication that the shape anisotropy dominates the dipolar coupling between the wires. We further show that the thermal treatment induces a decrease in the coercivity of the nanowire arrays. This reflects an enhancement of the quality of the nickel nanowires after annealing attributed to a decrease of the roughness of the nickel surface and to a reduction of the defect density. This new type of graphene-ferromagnetic-metal nanowire appears to be an interesting building block for spintronic applications.
AbstractList We report on the synthesis and magnetic characterization of ultralong (1 cm) arrays of highly ordered coaxial nanowires with nickel cores and graphene stacking shells (also known as metal-filled carbon nanotubes). Carbon-containing nickel nanowires are first grown on a nanograted surface by magnetron sputtering. Then, a post-annealing treatment favors the metal-catalyzed crystallization of carbon into stacked graphene layers rolled around the nickel cores. The observed uniaxial magnetic anisotropy field oriented along the nanowire axis is an indication that the shape anisotropy dominates the dipolar coupling between the wires. We further show that the thermal treatment induces a decrease in the coercivity of the nanowire arrays. This reflects an enhancement of the quality of the nickel nanowires after annealing attributed to a decrease of the roughness of the nickel surface and to a reduction of the defect density. This new type of graphene-ferromagnetic-metal nanowire appears to be an interesting building block for spintronic applications.
Author Angleraud, Benoit
Gautron, Eric
Granier, Agnès
El Mel, Abdel-Aziz
Duvail, Jean-Luc
Choi, Chang-Hwan
Tessier, Pierre-Yves
Xu, Wei
AuthorAffiliation 1 Institut des Matériaux Jean Rouxel, IMN, Université de Nantes, CNRS, 2 rue de la Houssinière, BP 32229, 44322 Nantes cedex 3, France, Telephone: +33 240 376 434, Fax: +33 240 373 959
2 Department of Mechanical Engineering, Stevens Institute of Technology, Hoboken, NJ 07030, USA
AuthorAffiliation_xml – name: 2 Department of Mechanical Engineering, Stevens Institute of Technology, Hoboken, NJ 07030, USA
– name: 1 Institut des Matériaux Jean Rouxel, IMN, Université de Nantes, CNRS, 2 rue de la Houssinière, BP 32229, 44322 Nantes cedex 3, France, Telephone: +33 240 376 434, Fax: +33 240 373 959
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Issue 1
Keywords nickel
phase separation
ferromagnetic
nanowires
carbon
nanofabrication
graphene
Language English
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SubjectTerms carbon
Condensed Matter
ferromagnetic
graphene
Letter
Materials Science
nanofabrication
Nanoscience
Nanotechnology
nanowires
nickel
phase separation
Physics
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Title Highly ordered ultralong magnetic nanowires wrapped in stacked graphene layers
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