Highly Efficient Electrocatalysts for Oxygen Reduction Based on 2D Covalent Organic Polymers Complexed with Non-precious Metals
A class of 2D covalent organic polymers (COPs) incorporating a metal (such as Fe, Co, Mn) with precisely controlled locations of nitrogen heteroatoms and holes were synthesized from various N‐containing metal–organic complexes (for example, metal–porphyrin complexes) by a nickel‐catalyzed Yamamoto r...
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| Published in | Angewandte Chemie International Edition Vol. 53; no. 9; pp. 2433 - 2437 |
|---|---|
| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Weinheim
WILEY-VCH Verlag
24.02.2014
WILEY‐VCH Verlag Wiley Wiley Subscription Services, Inc |
| Edition | International ed. in English |
| Subjects | |
| Online Access | Get full text |
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| Abstract | A class of 2D covalent organic polymers (COPs) incorporating a metal (such as Fe, Co, Mn) with precisely controlled locations of nitrogen heteroatoms and holes were synthesized from various N‐containing metal–organic complexes (for example, metal–porphyrin complexes) by a nickel‐catalyzed Yamamoto reaction. Subsequent carbonization of the metal‐incorporated COPs led to the formation of COP‐derived graphene analogues, which acted as efficient electrocatalysts for oxygen reduction in both alkaline and acid media with a good stability and free from any methanol‐crossover/CO‐poisoning effects.
Metal‐containing (M=Fe, Co, Mn) 2D covalent organic polymers with precisely controlled locations of N heteroatoms and holes were synthesized from metal–porphyrin complexes by a nickel‐catalyzed Yamamoto reaction. Subsequent carbonization led to graphene analogues, which are efficient electrocatalysts for oxygen reduction in both alkaline and acid media and are free from methanol‐crossover/CO poisoning. |
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| AbstractList | A class of 2D covalent organic polymers (COPs) incorporating a metal (such as Fe, Co, Mn) with precisely controlled locations of nitrogen heteroatoms and holes were synthesized from various N-containing metal-organic complexes (for example, metal-porphyrin complexes) by a nickel-catalyzed Yamamoto reaction. Subsequent carbonization of the metal-incorporated COPs led to the formation of COP-derived graphene analogues, which acted as efficient electrocatalysts for oxygen reduction in both alkaline and acid media with a good stability and free from any methanol-crossover/CO-poisoning effects. A class of 2D covalent organic polymers (COPs) incorporating a metal (such as Fe, Co, Mn) with precisely controlled locations of nitrogen heteroatoms and holes were synthesized from various N-containing metal-organic complexes (for example, metal-porphyrin complexes) by a nickel-catalyzed Yamamoto reaction. Subsequent carbonization of the metal-incorporated COPs led to the formation of COP-derived graphene analogues, which acted as efficient electrocatalysts for oxygen reduction in both alkaline and acid media with a good stability and free from any methanol-crossover/CO-poisoning effects. Metal-containing (M=Fe, Co, Mn) 2D covalent organic polymers with precisely controlled locations of Nheteroatoms and holes were synthesized from metal-porphyrin complexes by a nickel-catalyzed Yamamoto reaction. Subsequent carbonization led to graphene analogues, which are efficient electrocatalysts for oxygen reduction in both alkaline and acid media and are free from methanol-crossover/CO poisoning. A class of 2D covalent organic polymers (COPs) incorporating a metal (such as Fe, Co, Mn) with precisely controlled locations of nitrogen heteroatoms and holes were synthesized from various N‐containing metal–organic complexes (for example, metal–porphyrin complexes) by a nickel‐catalyzed Yamamoto reaction. Subsequent carbonization of the metal‐incorporated COPs led to the formation of COP‐derived graphene analogues, which acted as efficient electrocatalysts for oxygen reduction in both alkaline and acid media with a good stability and free from any methanol‐crossover/CO‐poisoning effects. Metal‐containing (M=Fe, Co, Mn) 2D covalent organic polymers with precisely controlled locations of N heteroatoms and holes were synthesized from metal–porphyrin complexes by a nickel‐catalyzed Yamamoto reaction. Subsequent carbonization led to graphene analogues, which are efficient electrocatalysts for oxygen reduction in both alkaline and acid media and are free from methanol‐crossover/CO poisoning. A class of 2D covalent organic polymers (COPs) incorporating a metal (such as Fe, Co, Mn) with precisely controlled locations of nitrogen heteroatoms and holes were synthesized from various N-containing metal-organic complexes (for example, metal-porphyrin complexes) by a nickel-catalyzed Yamamoto reaction. Subsequent carbonization of the metal-incorporated COPs led to the formation of COP-derived graphene analogues, which acted as efficient electrocatalysts for oxygen reduction in both alkaline and acid media with a good stability and free from any methanol-crossover/CO-poisoning effects. [PUBLICATION ABSTRACT] A class of 2D covalent organic polymers (COPs) incorporating a metal (such as Fe, Co, Mn) with precisely controlled locations of nitrogen heteroatoms and holes were synthesized from various N-containing metal-organic complexes (for example, metal-porphyrin complexes) by a nickel-catalyzed Yamamoto reaction. Subsequent carbonization of the metal-incorporated COPs led to the formation of COP-derived graphene analogues, which acted as efficient electrocatalysts for oxygen reduction in both alkaline and acid media with a good stability and free from any methanol-crossover/CO-poisoning effects.A class of 2D covalent organic polymers (COPs) incorporating a metal (such as Fe, Co, Mn) with precisely controlled locations of nitrogen heteroatoms and holes were synthesized from various N-containing metal-organic complexes (for example, metal-porphyrin complexes) by a nickel-catalyzed Yamamoto reaction. Subsequent carbonization of the metal-incorporated COPs led to the formation of COP-derived graphene analogues, which acted as efficient electrocatalysts for oxygen reduction in both alkaline and acid media with a good stability and free from any methanol-crossover/CO-poisoning effects. A class of 2D covalent organic polymers (COPs) incorporating a metal (such as Fe, Co, Mn) with precisely controlled locations of nitrogen heteroatoms and holes were synthesized from various N-containing metal-organic complexes (for example, metal-porphyrin complexes) by a nickel-catalyzed Yamamoto reaction. Subsequent carbonization of the metal-incorporated COPs led to the formation of COP-derived graphene analogues, which acted as efficient electro-catalysts for oxygen reduction in both alkaline and acid media with a good stability and free from any methanol-crossover/CO-poisoning effects. |
| Author | Dai, Liming Xue, Yuhua Cao, Dapeng Xiang, Zhonghua Chen, Jian-Feng Huang, Ling |
| Author_xml | – sequence: 1 givenname: Zhonghua surname: Xiang fullname: Xiang, Zhonghua organization: Centre of Advanced Science and Engineering for Carbon (Case4Carbon), Department of Macromolecular Science and Engineering, Case Western Reserve University, 10900 Euclid Avenue, Cleveland, OH 44106 (USA) – sequence: 2 givenname: Yuhua surname: Xue fullname: Xue, Yuhua organization: Centre of Advanced Science and Engineering for Carbon (Case4Carbon), Department of Macromolecular Science and Engineering, Case Western Reserve University, 10900 Euclid Avenue, Cleveland, OH 44106 (USA) – sequence: 3 givenname: Dapeng surname: Cao fullname: Cao, Dapeng email: caodp@mail.buct.edu.cn organization: State Key Lab of Organic-Inorganic Composites, Beijing University of Chemical Technology, Beijing 100029 (P.R. China) – sequence: 4 givenname: Ling surname: Huang fullname: Huang, Ling organization: State Key Lab of Organic-Inorganic Composites, Beijing University of Chemical Technology, Beijing 100029 (P.R. China) – sequence: 5 givenname: Jian-Feng surname: Chen fullname: Chen, Jian-Feng organization: State Key Lab of Organic-Inorganic Composites, Beijing University of Chemical Technology, Beijing 100029 (P.R. China) – sequence: 6 givenname: Liming surname: Dai fullname: Dai, Liming email: liming.dai@case.edu organization: Centre of Advanced Science and Engineering for Carbon (Case4Carbon), Department of Macromolecular Science and Engineering, Case Western Reserve University, 10900 Euclid Avenue, Cleveland, OH 44106 (USA) |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/24477972$$D View this record in MEDLINE/PubMed |
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| CODEN | ACIEAY |
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| Keywords | ENERGY-CONVERSION graphene analogues covalent organic polymers GRAPHENE NANOMATERIALS electrocatalysts oxygen reduction reaction CARBON NANOTUBE ARRAYS CATALYSTS metal-organic frameworks |
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| SSID | ssj0028806 |
| Score | 2.5982988 |
| Snippet | A class of 2D covalent organic polymers (COPs) incorporating a metal (such as Fe, Co, Mn) with precisely controlled locations of nitrogen heteroatoms and holes... |
| Source | Web of Science |
| SourceID | proquest pubmed webofscience crossref wiley istex |
| SourceType | Aggregation Database Index Database Enrichment Source Publisher |
| StartPage | 2433 |
| SubjectTerms | Carbonization Chemistry Chemistry, Multidisciplinary Covalence covalent organic polymers Electrocatalysts Graphene graphene analogues metal-organic frameworks Metals Nickel Oxygen oxygen reduction reaction Physical Sciences Polymers Reduction Science & Technology Two dimensional |
| Title | Highly Efficient Electrocatalysts for Oxygen Reduction Based on 2D Covalent Organic Polymers Complexed with Non-precious Metals |
| URI | https://api.istex.fr/ark:/67375/WNG-3MNF4X90-L/fulltext.pdf https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fanie.201308896 http://gateway.webofknowledge.com/gateway/Gateway.cgi?GWVersion=2&SrcApp=Summon&SrcAuth=ProQuest&DestApp=WOS&DestLinkType=FullRecord&UT=000336834000015 https://www.ncbi.nlm.nih.gov/pubmed/24477972 https://www.proquest.com/docview/1500559443 https://www.proquest.com/docview/1503548073 https://www.proquest.com/docview/1700990917 |
| Volume | 53 |
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