Strongly Veined Carbon Nanoleaves as a Highly Efficient Metal-Free Electrocatalyst
Effective integration of one‐dimensional carbon nanofibers (CNF) and two‐dimensional carbon sheets into three‐dimensional (3D) conductive frameworks is essential for their practical applications as electrode materials. Herein, a novel “vein‐leaf”‐type 3D complex of carbon nanofibers with nitrogen‐do...
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| Published in | Angewandte Chemie International Edition Vol. 53; no. 27; pp. 6905 - 6909 |
|---|---|
| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Weinheim
WILEY-VCH Verlag
01.07.2014
WILEY‐VCH Verlag Wiley Subscription Services, Inc |
| Edition | International ed. in English |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Effective integration of one‐dimensional carbon nanofibers (CNF) and two‐dimensional carbon sheets into three‐dimensional (3D) conductive frameworks is essential for their practical applications as electrode materials. Herein, a novel “vein‐leaf”‐type 3D complex of carbon nanofibers with nitrogen‐doped graphene (NG) was prepared through a simple thermal condensation of urea and bacterial cellulose. During the formation of the 3D complex CNF@NG, the graphene species was tethered to CNF via carbon–carbon bonds. Such an interconnected 3D network facilitates both the electron transfer and mass diffusion for electrochemical reactions.
“Green” leaves: A novel “vein‐leaf”‐type 3D complex of carbon nanofibers with nitrogen‐doped graphene (CNF@NG) was prepared through thermolysis of biomass materials. The interconnected 3D network of CNF@NG facilitates both the electron transfer and mass diffusion for electrochemical reactions. As a result, the CNF@NG complexes demonstrate remarkable electrocatalytic activities toward the oxygen reduction reaction (ORR). |
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| AbstractList | Abstract
Effective integration of one‐dimensional carbon nanofibers (CNF) and two‐dimensional carbon sheets into three‐dimensional (3D) conductive frameworks is essential for their practical applications as electrode materials. Herein, a novel “vein‐leaf”‐type 3D complex of carbon nanofibers with nitrogen‐doped graphene (NG) was prepared through a simple thermal condensation of urea and bacterial cellulose. During the formation of the 3D complex CNF@NG, the graphene species was tethered to CNF via carbon–carbon bonds. Such an interconnected 3D network facilitates both the electron transfer and mass diffusion for electrochemical reactions. Effective integration of one‐dimensional carbon nanofibers (CNF) and two‐dimensional carbon sheets into three‐dimensional (3D) conductive frameworks is essential for their practical applications as electrode materials. Herein, a novel “vein‐leaf”‐type 3D complex of carbon nanofibers with nitrogen‐doped graphene (NG) was prepared through a simple thermal condensation of urea and bacterial cellulose. During the formation of the 3D complex CNF@NG, the graphene species was tethered to CNF via carbon–carbon bonds. Such an interconnected 3D network facilitates both the electron transfer and mass diffusion for electrochemical reactions. “Green” leaves: A novel “vein‐leaf”‐type 3D complex of carbon nanofibers with nitrogen‐doped graphene (CNF@NG) was prepared through thermolysis of biomass materials. The interconnected 3D network of CNF@NG facilitates both the electron transfer and mass diffusion for electrochemical reactions. As a result, the CNF@NG complexes demonstrate remarkable electrocatalytic activities toward the oxygen reduction reaction (ORR). Effective integration of one-dimensional carbon nanofibers (CNF) and two-dimensional carbon sheets into three-dimensional (3D) conductive frameworks is essential for their practical applications as electrode materials. Herein, a novel "vein-leaf"-type 3D complex of carbon nanofibers with nitrogen-doped graphene (NG) was prepared through a simple thermal condensation of urea and bacterial cellulose. During the formation of the 3D complex CNF[at]NG, the graphene species was tethered to CNF via carbon-carbon bonds. Such an interconnected 3D network facilitates both the electron transfer and mass diffusion for electrochemical reactions. "Green" leaves: A novel "vein-leaf"-type 3D complex of carbon nanofibers with nitrogen-doped graphene (CNF[at]NG) was prepared through thermolysis of biomass materials. The interconnected 3D network of CNF[at]NG facilitates both the electron transfer and mass diffusion for electrochemical reactions. As a result, the CNF[at]NG complexes demonstrate remarkable electrocatalytic activities toward the oxygen reduction reaction (ORR). Effective integration of one-dimensional carbon nanofibers (CNF) and two-dimensional carbon sheets into three-dimensional (3D) conductive frameworks is essential for their practical applications as electrode materials. Herein, a novel "vein-leaf"-type 3D complex of carbon nanofibers with nitrogen-doped graphene (NG) was prepared through a simple thermal condensation of urea and bacterial cellulose. During the formation of the 3D complex CNF@NG, the graphene species was tethered to CNF via carbon-carbon bonds. Such an interconnected 3D network facilitates both the electron transfer and mass diffusion for electrochemical reactions. |
| Author | Lv, Li-Bing Ye, Tian-Nan Xu, Miao Li, Xin-Hao Chen, Jie-Sheng |
| Author_xml | – sequence: 1 givenname: Tian-Nan surname: Ye fullname: Ye, Tian-Nan organization: School of Chemistry and Chemical Engineering, Shanghai Jiao Tong University, Shanghai 200240 (P. R. China) – sequence: 2 givenname: Li-Bing surname: Lv fullname: Lv, Li-Bing organization: School of Chemistry and Chemical Engineering, Shanghai Jiao Tong University, Shanghai 200240 (P. R. China) – sequence: 3 givenname: Xin-Hao surname: Li fullname: Li, Xin-Hao email: xinhaoli@sjtu.edu.cn organization: School of Chemistry and Chemical Engineering, Shanghai Jiao Tong University, Shanghai 200240 (P. R. China) – sequence: 4 givenname: Miao surname: Xu fullname: Xu, Miao organization: School of Chemistry and Chemical Engineering, Shanghai Jiao Tong University, Shanghai 200240 (P. R. China) – sequence: 5 givenname: Jie-Sheng surname: Chen fullname: Chen, Jie-Sheng email: chemcj@sjtu.edu.cn organization: School of Chemistry and Chemical Engineering, Shanghai Jiao Tong University, Shanghai 200240 (P. R. China) |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/24854797$$D View this record in MEDLINE/PubMed |
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| Keywords | biomass electrocatalysts carbon nanofibers graphene leaf nanostructures |
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| Snippet | Effective integration of one‐dimensional carbon nanofibers (CNF) and two‐dimensional carbon sheets into three‐dimensional (3D) conductive frameworks is... Effective integration of one-dimensional carbon nanofibers (CNF) and two-dimensional carbon sheets into three-dimensional (3D) conductive frameworks is... Abstract Effective integration of one‐dimensional carbon nanofibers (CNF) and two‐dimensional carbon sheets into three‐dimensional (3D) conductive frameworks... |
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| SubjectTerms | Bacteria biomass Carbon Carbon fibers carbon nanofibers Diffusion electrocatalysts Electron transfer Graphene leaf nanostructures Nanofibers Networks Three dimensional |
| Title | Strongly Veined Carbon Nanoleaves as a Highly Efficient Metal-Free Electrocatalyst |
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