High‐Performance Thermally Conductive Phase Change Composites by Large‐Size Oriented Graphite Sheets for Scalable Thermal Energy Harvesting
Efficient thermal energy harvesting using phase‐change materials (PCMs) has great potential for cost‐effective thermal management and energy storage applications. However, the low thermal conductivity of PCMs (KPCM) is a long‐standing bottleneck for high‐power‐density energy harvesting. Although PCM...
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| Published in | Advanced materials (Weinheim) Vol. 31; no. 49; pp. e1905099 - n/a |
|---|---|
| Main Authors | , , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Germany
Wiley Subscription Services, Inc
01.12.2019
|
| Subjects | |
| Online Access | Get full text |
| ISSN | 0935-9648 1521-4095 1521-4095 |
| DOI | 10.1002/adma.201905099 |
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| Abstract | Efficient thermal energy harvesting using phase‐change materials (PCMs) has great potential for cost‐effective thermal management and energy storage applications. However, the low thermal conductivity of PCMs (KPCM) is a long‐standing bottleneck for high‐power‐density energy harvesting. Although PCM‐based nanocomposites with an enhanced thermal conductivity can address this issue, achieving a higher K (>10 W m−1 K−1) at filler loadings below 50 wt% remains challenging. A strategy for synthesizing highly thermally conductive phase‐change composites (PCCs) by compression‐induced construction of large aligned graphite sheets inside PCCs is demonstrated. The millimeter‐sized graphite sheet consists of lateral van‐der‐Waals‐bonded and oriented graphite nanoplatelets at the micro/nanoscale, which together with a thin PCM layer between the sheets synergistically enhance KPCM in the range of 4.4–35.0 W m−1 K−1 at graphite loadings below 40.0 wt%. The resulting PCCs also demonstrate homogeneity, no leakage, and superior phase change behavior, which can be easily engineered into devices for efficient thermal energy harvesting by coordinating the sheet orientation with the thermal transport direction. This method offers a promising route to high‐power‐density and low‐cost applications of PCMs in large‐scale thermal energy storage, thermal management of electronics, etc.
A method for synthesizing high‐performance thermally conductive phase‐ change composites is demonstrated. Large aligned graphite sheets inside the composite are generated from worm‐like expanded graphite. The aligned and interconnected graphite framework enhances KPCM up to 4.4–35.0 W m−1 K−1 at graphite loadings below 40.0 wt%, which may accelerate the high‐power‐density, low‐cost, and large‐scale applications of phase‐change materials. |
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| AbstractList | Efficient thermal energy harvesting using phase‐change materials (PCMs) has great potential for cost‐effective thermal management and energy storage applications. However, the low thermal conductivity of PCMs (
K
PCM
) is a long‐standing bottleneck for high‐power‐density energy harvesting. Although PCM‐based nanocomposites with an enhanced thermal conductivity can address this issue, achieving a higher
K
(>10 W m
−1
K
−1
) at filler loadings below 50 wt% remains challenging. A strategy for synthesizing highly thermally conductive phase‐change composites (PCCs) by compression‐induced construction of large aligned graphite sheets inside PCCs is demonstrated. The millimeter‐sized graphite sheet consists of lateral van‐der‐Waals‐bonded and oriented graphite nanoplatelets at the micro/nanoscale, which together with a thin PCM layer between the sheets synergistically enhance
K
PCM
in the range of 4.4–35.0 W m
−1
K
−1
at graphite loadings below 40.0 wt%. The resulting PCCs also demonstrate homogeneity, no leakage, and superior phase change behavior, which can be easily engineered into devices for efficient thermal energy harvesting by coordinating the sheet orientation with the thermal transport direction. This method offers a promising route to high‐power‐density and low‐cost applications of PCMs in large‐scale thermal energy storage, thermal management of electronics, etc. Efficient thermal energy harvesting using phase‐change materials (PCMs) has great potential for cost‐effective thermal management and energy storage applications. However, the low thermal conductivity of PCMs (KPCM) is a long‐standing bottleneck for high‐power‐density energy harvesting. Although PCM‐based nanocomposites with an enhanced thermal conductivity can address this issue, achieving a higher K (>10 W m−1 K−1) at filler loadings below 50 wt% remains challenging. A strategy for synthesizing highly thermally conductive phase‐change composites (PCCs) by compression‐induced construction of large aligned graphite sheets inside PCCs is demonstrated. The millimeter‐sized graphite sheet consists of lateral van‐der‐Waals‐bonded and oriented graphite nanoplatelets at the micro/nanoscale, which together with a thin PCM layer between the sheets synergistically enhance KPCM in the range of 4.4–35.0 W m−1 K−1 at graphite loadings below 40.0 wt%. The resulting PCCs also demonstrate homogeneity, no leakage, and superior phase change behavior, which can be easily engineered into devices for efficient thermal energy harvesting by coordinating the sheet orientation with the thermal transport direction. This method offers a promising route to high‐power‐density and low‐cost applications of PCMs in large‐scale thermal energy storage, thermal management of electronics, etc. Efficient thermal energy harvesting using phase-change materials (PCMs) has great potential for cost-effective thermal management and energy storage applications. However, the low thermal conductivity of PCMs (K ) is a long-standing bottleneck for high-power-density energy harvesting. Although PCM-based nanocomposites with an enhanced thermal conductivity can address this issue, achieving a higher K (>10 W m K ) at filler loadings below 50 wt% remains challenging. A strategy for synthesizing highly thermally conductive phase-change composites (PCCs) by compression-induced construction of large aligned graphite sheets inside PCCs is demonstrated. The millimeter-sized graphite sheet consists of lateral van-der-Waals-bonded and oriented graphite nanoplatelets at the micro/nanoscale, which together with a thin PCM layer between the sheets synergistically enhance K in the range of 4.4-35.0 W m K at graphite loadings below 40.0 wt%. The resulting PCCs also demonstrate homogeneity, no leakage, and superior phase change behavior, which can be easily engineered into devices for efficient thermal energy harvesting by coordinating the sheet orientation with the thermal transport direction. This method offers a promising route to high-power-density and low-cost applications of PCMs in large-scale thermal energy storage, thermal management of electronics, etc. Efficient thermal energy harvesting using phase‐change materials (PCMs) has great potential for cost‐effective thermal management and energy storage applications. However, the low thermal conductivity of PCMs (KPCM) is a long‐standing bottleneck for high‐power‐density energy harvesting. Although PCM‐based nanocomposites with an enhanced thermal conductivity can address this issue, achieving a higher K (>10 W m−1 K−1) at filler loadings below 50 wt% remains challenging. A strategy for synthesizing highly thermally conductive phase‐change composites (PCCs) by compression‐induced construction of large aligned graphite sheets inside PCCs is demonstrated. The millimeter‐sized graphite sheet consists of lateral van‐der‐Waals‐bonded and oriented graphite nanoplatelets at the micro/nanoscale, which together with a thin PCM layer between the sheets synergistically enhance KPCM in the range of 4.4–35.0 W m−1 K−1 at graphite loadings below 40.0 wt%. The resulting PCCs also demonstrate homogeneity, no leakage, and superior phase change behavior, which can be easily engineered into devices for efficient thermal energy harvesting by coordinating the sheet orientation with the thermal transport direction. This method offers a promising route to high‐power‐density and low‐cost applications of PCMs in large‐scale thermal energy storage, thermal management of electronics, etc. A method for synthesizing high‐performance thermally conductive phase‐ change composites is demonstrated. Large aligned graphite sheets inside the composite are generated from worm‐like expanded graphite. The aligned and interconnected graphite framework enhances KPCM up to 4.4–35.0 W m−1 K−1 at graphite loadings below 40.0 wt%, which may accelerate the high‐power‐density, low‐cost, and large‐scale applications of phase‐change materials. Efficient thermal energy harvesting using phase-change materials (PCMs) has great potential for cost-effective thermal management and energy storage applications. However, the low thermal conductivity of PCMs (KPCM ) is a long-standing bottleneck for high-power-density energy harvesting. Although PCM-based nanocomposites with an enhanced thermal conductivity can address this issue, achieving a higher K (>10 W m-1 K-1 ) at filler loadings below 50 wt% remains challenging. A strategy for synthesizing highly thermally conductive phase-change composites (PCCs) by compression-induced construction of large aligned graphite sheets inside PCCs is demonstrated. The millimeter-sized graphite sheet consists of lateral van-der-Waals-bonded and oriented graphite nanoplatelets at the micro/nanoscale, which together with a thin PCM layer between the sheets synergistically enhance KPCM in the range of 4.4-35.0 W m-1 K-1 at graphite loadings below 40.0 wt%. The resulting PCCs also demonstrate homogeneity, no leakage, and superior phase change behavior, which can be easily engineered into devices for efficient thermal energy harvesting by coordinating the sheet orientation with the thermal transport direction. This method offers a promising route to high-power-density and low-cost applications of PCMs in large-scale thermal energy storage, thermal management of electronics, etc.Efficient thermal energy harvesting using phase-change materials (PCMs) has great potential for cost-effective thermal management and energy storage applications. However, the low thermal conductivity of PCMs (KPCM ) is a long-standing bottleneck for high-power-density energy harvesting. Although PCM-based nanocomposites with an enhanced thermal conductivity can address this issue, achieving a higher K (>10 W m-1 K-1 ) at filler loadings below 50 wt% remains challenging. A strategy for synthesizing highly thermally conductive phase-change composites (PCCs) by compression-induced construction of large aligned graphite sheets inside PCCs is demonstrated. The millimeter-sized graphite sheet consists of lateral van-der-Waals-bonded and oriented graphite nanoplatelets at the micro/nanoscale, which together with a thin PCM layer between the sheets synergistically enhance KPCM in the range of 4.4-35.0 W m-1 K-1 at graphite loadings below 40.0 wt%. The resulting PCCs also demonstrate homogeneity, no leakage, and superior phase change behavior, which can be easily engineered into devices for efficient thermal energy harvesting by coordinating the sheet orientation with the thermal transport direction. This method offers a promising route to high-power-density and low-cost applications of PCMs in large-scale thermal energy storage, thermal management of electronics, etc. |
| Author | Wu, Si Yan, Taisen Tong, Zhen Xu, Jiaxing Deng, Tao Zhai, Tianyao Xu, Zhenyuan Wang, Ruzhu Chao, Jingwei Wu, Minqiang Li, Tingxian Bao, Hua |
| Author_xml | – sequence: 1 givenname: Si surname: Wu fullname: Wu, Si organization: Shanghai Jiao Tong University – sequence: 2 givenname: Tingxian orcidid: 0000-0003-4618-8144 surname: Li fullname: Li, Tingxian email: Litx@sjtu.edu.cn organization: Shanghai Jiao Tong University – sequence: 3 givenname: Zhen surname: Tong fullname: Tong, Zhen organization: Shanghai Jiao Tong University – sequence: 4 givenname: Jingwei surname: Chao fullname: Chao, Jingwei organization: Shanghai Jiao Tong University – sequence: 5 givenname: Tianyao surname: Zhai fullname: Zhai, Tianyao organization: Shanghai Jiao Tong University – sequence: 6 givenname: Jiaxing surname: Xu fullname: Xu, Jiaxing organization: Shanghai Jiao Tong University – sequence: 7 givenname: Taisen surname: Yan fullname: Yan, Taisen organization: Shanghai Jiao Tong University – sequence: 8 givenname: Minqiang surname: Wu fullname: Wu, Minqiang organization: Shanghai Jiao Tong University – sequence: 9 givenname: Zhenyuan surname: Xu fullname: Xu, Zhenyuan organization: Shanghai Jiao Tong University – sequence: 10 givenname: Hua surname: Bao fullname: Bao, Hua organization: Shanghai Jiao Tong University – sequence: 11 givenname: Tao surname: Deng fullname: Deng, Tao email: Dengtao@sjtu.edu.cn organization: Shanghai Jiao Tong University – sequence: 12 givenname: Ruzhu surname: Wang fullname: Wang, Ruzhu email: Rzwang@sjtu.edu.cn organization: Shanghai Jiao Tong University |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/31621971$$D View this record in MEDLINE/PubMed |
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| Snippet | Efficient thermal energy harvesting using phase‐change materials (PCMs) has great potential for cost‐effective thermal management and energy storage... Efficient thermal energy harvesting using phase-change materials (PCMs) has great potential for cost-effective thermal management and energy storage... |
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| SubjectTerms | Density Energy harvesting Energy management Energy storage expanded graphite Graphite graphite sheets Heat conductivity Heat transfer Materials science Nanocomposites Phase change phase change composites Sheets Thermal conductivity Thermal energy thermal energy harvesting Thermal management |
| Title | High‐Performance Thermally Conductive Phase Change Composites by Large‐Size Oriented Graphite Sheets for Scalable Thermal Energy Harvesting |
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