High‐Capacity Cathode Material with High Voltage for Li‐Ion Batteries
Electrochemical energy storage devices with a high energy density are an important technology in modern society, especially for electric vehicles. The most effective approach to improve the energy density of batteries is to search for high‐capacity electrode materials. According to the concept of en...
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| Published in | Advanced materials (Weinheim) Vol. 30; no. 9 |
|---|---|
| Main Authors | , , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Germany
Wiley Subscription Services, Inc
01.03.2018
Wiley |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Electrochemical energy storage devices with a high energy density are an important technology in modern society, especially for electric vehicles. The most effective approach to improve the energy density of batteries is to search for high‐capacity electrode materials. According to the concept of energy quality, a high‐voltage battery delivers a highly useful energy, thus providing a new insight to improve energy density. Based on this concept, a novel and successful strategy to increase the energy density and energy quality by increasing the discharge voltage of cathode materials and preserving high capacity is proposed. The proposal is realized in high‐capacity Li‐rich cathode materials. The average discharge voltage is increased from 3.5 to 3.8 V by increasing the nickel content and applying a simple after‐treatment, and the specific energy is improved from 912 to 1033 Wh kg−1. The current work provides an insightful universal principle for developing, designing, and screening electrode materials for high energy density and energy quality.
Li‐ion batteries with high energy quality require a high capacity coupled with high operating voltage. This requires the electrode materials to not only have a high specific capacity but also a high discharge voltage for cathode materials and low charge voltage for anode materials. |
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| AbstractList | Electrochemical energy storage devices with a high energy density are an important technology in modern society, especially for electric vehicles. The most effective approach to improve the energy density of batteries is to search for high‐capacity electrode materials. According to the concept of energy quality, a high‐voltage battery delivers a highly useful energy, thus providing a new insight to improve energy density. Based on this concept, a novel and successful strategy to increase the energy density and energy quality by increasing the discharge voltage of cathode materials and preserving high capacity is proposed. The proposal is realized in high‐capacity Li‐rich cathode materials. The average discharge voltage is increased from 3.5 to 3.8 V by increasing the nickel content and applying a simple after‐treatment, and the specific energy is improved from 912 to 1033 Wh kg−1. The current work provides an insightful universal principle for developing, designing, and screening electrode materials for high energy density and energy quality.
Li‐ion batteries with high energy quality require a high capacity coupled with high operating voltage. This requires the electrode materials to not only have a high specific capacity but also a high discharge voltage for cathode materials and low charge voltage for anode materials. Electrochemical energy storage devices with a high energy density are an important technology in modern society, especially for electric vehicles. The most effective approach to improve the energy density of batteries is to search for high-capacity electrode materials. According to the concept of energy quality, a high-voltage battery delivers a highly useful energy, thus providing a new insight to improve energy density. Based on this concept, a novel and successful strategy to increase the energy density and energy quality by increasing the discharge voltage of cathode materials and preserving high capacity is proposed. The proposal is realized in high-capacity Li-rich cathode materials. The average discharge voltage is increased from 3.5 to 3.8 V by increasing the nickel content and applying a simple after-treatment, and the specific energy is improved from 912 to 1033 Wh kg-1. The current work provides an insightful universal principle for developing, designing, and screening electrode materials for high energy density and energy quality. Electrochemical energy storage devices with a high energy density are an important technology in modern society, especially for electric vehicles. The most effective approach to improve the energy density of batteries is to search for high‐capacity electrode materials. According to the concept of energy quality, a high‐voltage battery delivers a highly useful energy, thus providing a new insight to improve energy density. Based on this concept, a novel and successful strategy to increase the energy density and energy quality by increasing the discharge voltage of cathode materials and preserving high capacity is proposed. The proposal is realized in high‐capacity Li‐rich cathode materials. The average discharge voltage is increased from 3.5 to 3.8 V by increasing the nickel content and applying a simple after‐treatment, and the specific energy is improved from 912 to 1033 Wh kg −1 . The current work provides an insightful universal principle for developing, designing, and screening electrode materials for high energy density and energy quality. Electrochemical energy storage devices with a high energy density are an important technology in modern society, especially for electric vehicles. The most effective approach to improve the energy density of batteries is to search for high-capacity electrode materials. According to the concept of energy quality, a high-voltage battery delivers a highly useful energy, thus providing a new insight to improve energy density. Based on this concept, a novel and successful strategy to increase the energy density and energy quality by increasing the discharge voltage of cathode materials and preserving high capacity is proposed. The proposal is realized in high-capacity Li-rich cathode materials. The average discharge voltage is increased from 3.5 to 3.8 V by increasing the nickel content and applying a simple after-treatment, and the specific energy is improved from 912 to 1033 Wh kg . The current work provides an insightful universal principle for developing, designing, and screening electrode materials for high energy density and energy quality. Electrochemical energy storage devices with a high energy density are an important technology in modern society, especially for electric vehicles. The most effective approach to improve the energy density of batteries is to search for high‐capacity electrode materials. According to the concept of energy quality, a high‐voltage battery delivers a highly useful energy, thus providing a new insight to improve energy density. Based on this concept, a novel and successful strategy to increase the energy density and energy quality by increasing the discharge voltage of cathode materials and preserving high capacity is proposed. The proposal is realized in high‐capacity Li‐rich cathode materials. The average discharge voltage is increased from 3.5 to 3.8 V by increasing the nickel content and applying a simple after‐treatment, and the specific energy is improved from 912 to 1033 Wh kg−1. The current work provides an insightful universal principle for developing, designing, and screening electrode materials for high energy density and energy quality. Electrochemical energy storage devices with a high energy density are an important technology in modern society, especially for electric vehicles. The most effective approach to improve the energy density of batteries is to search for high-capacity electrode materials. According to the concept of energy quality, a high-voltage battery delivers a highly useful energy, thus providing a new insight to improve energy density. Based on this concept, a novel and successful strategy to increase the energy density and energy quality by increasing the discharge voltage of cathode materials and preserving high capacity is proposed. The proposal is realized in high-capacity Li-rich cathode materials. The average discharge voltage is increased from 3.5 to 3.8 V by increasing the nickel content and applying a simple after-treatment, and the specific energy is improved from 912 to 1033 Wh kg-1 . The current work provides an insightful universal principle for developing, designing, and screening electrode materials for high energy density and energy quality.Electrochemical energy storage devices with a high energy density are an important technology in modern society, especially for electric vehicles. The most effective approach to improve the energy density of batteries is to search for high-capacity electrode materials. According to the concept of energy quality, a high-voltage battery delivers a highly useful energy, thus providing a new insight to improve energy density. Based on this concept, a novel and successful strategy to increase the energy density and energy quality by increasing the discharge voltage of cathode materials and preserving high capacity is proposed. The proposal is realized in high-capacity Li-rich cathode materials. The average discharge voltage is increased from 3.5 to 3.8 V by increasing the nickel content and applying a simple after-treatment, and the specific energy is improved from 912 to 1033 Wh kg-1 . The current work provides an insightful universal principle for developing, designing, and screening electrode materials for high energy density and energy quality. |
| Author | Huang, Xiaojing Xiao, Dong‐Dong Gu, Lin Wan, Li‐Jun Yin, Ya‐Xia Yu, Xiqian Yang, Xiao‐Qing Guo, Yu‐Guo Shi, Ji‐Lei Chu, Yong Zhang, Xu‐Dong Ge, Mingyuan |
| Author_xml | – sequence: 1 givenname: Ji‐Lei surname: Shi fullname: Shi, Ji‐Lei organization: University of Chinese Academy of Sciences – sequence: 2 givenname: Dong‐Dong surname: Xiao fullname: Xiao, Dong‐Dong organization: Chinese Academy of Sciences (CAS) – sequence: 3 givenname: Mingyuan surname: Ge fullname: Ge, Mingyuan organization: Brookhaven National Laboratory – sequence: 4 givenname: Xiqian surname: Yu fullname: Yu, Xiqian organization: Chinese Academy of Sciences (CAS) – sequence: 5 givenname: Yong surname: Chu fullname: Chu, Yong organization: Brookhaven National Laboratory – sequence: 6 givenname: Xiaojing surname: Huang fullname: Huang, Xiaojing organization: Brookhaven National Laboratory – sequence: 7 givenname: Xu‐Dong surname: Zhang fullname: Zhang, Xu‐Dong organization: University of Chinese Academy of Sciences – sequence: 8 givenname: Ya‐Xia surname: Yin fullname: Yin, Ya‐Xia organization: University of Chinese Academy of Sciences – sequence: 9 givenname: Xiao‐Qing surname: Yang fullname: Yang, Xiao‐Qing organization: Brookhaven National Laboratory – sequence: 10 givenname: Yu‐Guo orcidid: 0000-0003-0322-8476 surname: Guo fullname: Guo, Yu‐Guo email: ygguo@iccas.ac.cn organization: University of Chinese Academy of Sciences – sequence: 11 givenname: Lin surname: Gu fullname: Gu, Lin email: l.gu@iphy.ac.cn organization: Chinese Academy of Sciences (CAS) – sequence: 12 givenname: Li‐Jun surname: Wan fullname: Wan, Li‐Jun email: wanlijun@iccas.ac.cn organization: Chinese Academy of Sciences (CAS) |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/29333690$$D View this record in MEDLINE/PubMed https://www.osti.gov/servlets/purl/1436262$$D View this record in Osti.gov |
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| SubjectTerms | cathode materials Cathodes Density Electric potential Electric vehicles Electrode materials Electrodes Energy energy quality Energy storage Flux density high capacity batteries Lithium MATERIALS SCIENCE Storage batteries voltage decay |
| Title | High‐Capacity Cathode Material with High Voltage for Li‐Ion Batteries |
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