Photo‐Iniferter RAFT Polymerization

Light‐mediated polymerization techniques offer distinct advantages over polymerization reactions fueled by thermal energy, such as high spatial and temporal control as well as the possibility to work under mild reaction conditions. Reversible addition‐fragmentation chain‐transfer (RAFT) polymerizati...

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Published inMacromolecular rapid communications. Vol. 43; no. 1; pp. e2100514 - n/a
Main Author Hartlieb, Matthias
Format Journal Article
LanguageEnglish
Published Germany Wiley Subscription Services, Inc 01.01.2022
Subjects
Addition polymerization
Catalysis
Catalysts
Chain transfer
light
Macromolecules
Molecular Structure
Monomers
photo‐iniferter reversible addition‐fragmentation chain‐transfer
photo‐mediated polymerization
Polyimide resins
Polymerization
radical polymerization
reversible addition‐fragmentation chain‐transfer polymerization
Thermal energy
reversible addition-fragmentation chain-transfer polymerization
photo-mediated polymerization
photo-iniferter reversible addition-fragmentation chain-transfer
light
radical polymerization
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Abstract Light‐mediated polymerization techniques offer distinct advantages over polymerization reactions fueled by thermal energy, such as high spatial and temporal control as well as the possibility to work under mild reaction conditions. Reversible addition‐fragmentation chain‐transfer (RAFT) polymerization is a highly versatile radical polymerization method that can be utilized to control a variety of monomers and produce a vast number of complex macromolecular structures. The use of light to drive a RAFT‐polymerization is possible via multiple routes. Besides the use of photo‐initiators, or photo‐catalysts, the direct activation of the chain transfer agent controlling the RAFT process in a photo‐iniferter (PI) process is an elegant way to initiate and control polymerization reactions. Within this review, PI‐RAFT polymerization and its advantages over the conventional RAFT process are discussed in detail. The direct activation of chain transfer agents controlling a radical polymerization process by light is called a photo‐iniferter reversible addition‐fragmentation chain‐transfer (RAFT) polymerization. This method possesses a number of advantages compared to the conventional RAFT methodology. The origin, mechanistic, and applications of this technique are discussed in this review.
AbstractList Light-mediated polymerization techniques offer distinct advantages over polymerization reactions fueled by thermal energy, such as high spatial and temporal control as well as the possibility to work under mild reaction conditions. Reversible addition-fragmentation chain-transfer (RAFT) polymerization is a highly versatile radical polymerization method that can be utilized to control a variety of monomers and produce a vast number of complex macromolecular structures. The use of light to drive a RAFT-polymerization is possible via multiple routes. Besides the use of photo-initiators, or photo-catalysts, the direct activation of the chain transfer agent controlling the RAFT process in a photo-iniferter (PI) process is an elegant way to initiate and control polymerization reactions. Within this review, PI-RAFT polymerization and its advantages over the conventional RAFT process are discussed in detail.Light-mediated polymerization techniques offer distinct advantages over polymerization reactions fueled by thermal energy, such as high spatial and temporal control as well as the possibility to work under mild reaction conditions. Reversible addition-fragmentation chain-transfer (RAFT) polymerization is a highly versatile radical polymerization method that can be utilized to control a variety of monomers and produce a vast number of complex macromolecular structures. The use of light to drive a RAFT-polymerization is possible via multiple routes. Besides the use of photo-initiators, or photo-catalysts, the direct activation of the chain transfer agent controlling the RAFT process in a photo-iniferter (PI) process is an elegant way to initiate and control polymerization reactions. Within this review, PI-RAFT polymerization and its advantages over the conventional RAFT process are discussed in detail.
Light-mediated polymerization techniques offer distinct advantages over polymerization reactions fueled by thermal energy, such as high spatial and temporal control as well as the possibility to work under mild reaction conditions. Reversible addition-fragmentation chain-transfer (RAFT) polymerization is a highly versatile radical polymerization method that can be utilized to control a variety of monomers and produce a vast number of complex macromolecular structures. The use of light to drive a RAFT-polymerization is possible via multiple routes. Besides the use of photo-initiators, or photo-catalysts, the direct activation of the chain transfer agent controlling the RAFT process in a photo-iniferter (PI) process is an elegant way to initiate and control polymerization reactions. Within this review, PI-RAFT polymerization and its advantages over the conventional RAFT process are discussed in detail.
Light‐mediated polymerization techniques offer distinct advantages over polymerization reactions fueled by thermal energy, such as high spatial and temporal control as well as the possibility to work under mild reaction conditions. Reversible addition‐fragmentation chain‐transfer (RAFT) polymerization is a highly versatile radical polymerization method that can be utilized to control a variety of monomers and produce a vast number of complex macromolecular structures. The use of light to drive a RAFT‐polymerization is possible via multiple routes. Besides the use of photo‐initiators, or photo‐catalysts, the direct activation of the chain transfer agent controlling the RAFT process in a photo‐iniferter (PI) process is an elegant way to initiate and control polymerization reactions. Within this review, PI‐RAFT polymerization and its advantages over the conventional RAFT process are discussed in detail. The direct activation of chain transfer agents controlling a radical polymerization process by light is called a photo‐iniferter reversible addition‐fragmentation chain‐transfer (RAFT) polymerization. This method possesses a number of advantages compared to the conventional RAFT methodology. The origin, mechanistic, and applications of this technique are discussed in this review.
Author Hartlieb, Matthias
Author_xml – sequence: 1
  givenname: Matthias
  orcidid: 0000-0001-5330-7186
  surname: Hartlieb
  fullname: Hartlieb, Matthias
  email: mhartlieb@uni-potsdam.de
  organization: Fraunhofer Institute for Applied Polymer Research (IAP)
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Sun Jul 13 04:31:47 EDT 2025
Wed Feb 19 02:28:26 EST 2025
Tue Jul 01 03:31:45 EDT 2025
Thu Apr 24 22:55:55 EDT 2025
Wed Jan 22 16:26:28 EST 2025
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Issue 1
Keywords reversible addition-fragmentation chain-transfer polymerization
photo-mediated polymerization
photo-iniferter reversible addition-fragmentation chain-transfer
light
radical polymerization
Language English
License Attribution-NonCommercial
2021 The Authors. Macromolecular Rapid Communications published by Wiley-VCH GmbH.
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34994488 - Macromol Rapid Commun. 2022 Jan;43(1):e2100856
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Snippet Light‐mediated polymerization techniques offer distinct advantages over polymerization reactions fueled by thermal energy, such as high spatial and temporal...
Light-mediated polymerization techniques offer distinct advantages over polymerization reactions fueled by thermal energy, such as high spatial and temporal...
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SubjectTerms Addition polymerization
Catalysis
Catalysts
Chain transfer
light
Macromolecules
Molecular Structure
Monomers
photo‐iniferter reversible addition‐fragmentation chain‐transfer
photo‐mediated polymerization
Polyimide resins
Polymerization
radical polymerization
reversible addition‐fragmentation chain‐transfer polymerization
Thermal energy
Title Photo‐Iniferter RAFT Polymerization
URI https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fmarc.202100514
https://www.ncbi.nlm.nih.gov/pubmed/34750911
https://www.proquest.com/docview/2617222613
https://www.proquest.com/docview/2595564744
Volume 43
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