Surface-Anchored MOF-Based Photonic Antennae
The loading of a metal‐organic framework (MOF), [Cu3(btc)2xH2O] HKUST‐1, with europium β‐diketonate complexes is studied with the goal to using the porous molecular framework as a photonic antenna. Whereas loading of HKUST‐1 powder particles produced via the conventional solvothermal synthesis metho...
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| Published in | Chemphyschem Vol. 13; no. 11; pp. 2699 - 2702 |
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| Main Authors | , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
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Weinheim
WILEY-VCH Verlag
06.08.2012
WILEY‐VCH Verlag Wiley |
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| Abstract | The loading of a metal‐organic framework (MOF), [Cu3(btc)2xH2O] HKUST‐1, with europium β‐diketonate complexes is studied with the goal to using the porous molecular framework as a photonic antenna. Whereas loading of HKUST‐1 powder particles produced via the conventional solvothermal synthesis method was strongly hindered, for HKUST‐1 SURMOFs, thin MOF films fabricated using the liquid phase epitaxy method, a high filling factor can be achieved. The optical properties of the HKUST‐1‐MOFs before and after loading were analysed with the aid of luminescence spectroscopy. Careful analysis of the absorption spectra reveals the presence of an effective energy transfer between the HKUST‐1 framework and the Eu3+ centers.
The optical properties of HKUST‐1 MOFs before and after loading a Eu3+ complex are analysed with the aid of luminescence spectroscopy (see graphic). The presence of an effective energy transfer between the HKUST‐1 framework and the Eu3+ centers was found as is described herein. |
|---|---|
| AbstractList | Abstract
The loading of a metal‐organic framework (MOF), [Cu
3
(btc)
2
x
H
2
O] HKUST‐1, with europium β‐diketonate complexes is studied with the goal to using the porous molecular framework as a photonic antenna. Whereas loading of HKUST‐1 powder particles produced via the conventional solvothermal synthesis method was strongly hindered, for HKUST‐1 SURMOFs, thin MOF films fabricated using the liquid phase epitaxy method, a high filling factor can be achieved. The optical properties of the HKUST‐1‐MOFs before and after loading were analysed with the aid of luminescence spectroscopy. Careful analysis of the absorption spectra reveals the presence of an effective energy transfer between the HKUST‐1 framework and the Eu
3+
centers. The loading of a metal-organic framework (MOF), [Cu(3)(btc)(2)xH(2)O] HKUST-1, with europium β-diketonate complexes is studied with the goal to using the porous molecular framework as a photonic antenna. Whereas loading of HKUST-1 powder particles produced via the conventional solvothermal synthesis method was strongly hindered, for HKUST-1 SURMOFs, thin MOF films fabricated using the liquid phase epitaxy method, a high filling factor can be achieved. The optical properties of the HKUST-1-MOFs before and after loading were analysed with the aid of luminescence spectroscopy. Careful analysis of the absorption spectra reveals the presence of an effective energy transfer between the HKUST-1 framework and the Eu(3+) centers. The loading of a metal‐organic framework (MOF), [Cu3(btc)2xH2O] HKUST‐1, with europium β‐diketonate complexes is studied with the goal to using the porous molecular framework as a photonic antenna. Whereas loading of HKUST‐1 powder particles produced via the conventional solvothermal synthesis method was strongly hindered, for HKUST‐1 SURMOFs, thin MOF films fabricated using the liquid phase epitaxy method, a high filling factor can be achieved. The optical properties of the HKUST‐1‐MOFs before and after loading were analysed with the aid of luminescence spectroscopy. Careful analysis of the absorption spectra reveals the presence of an effective energy transfer between the HKUST‐1 framework and the Eu3+ centers. The optical properties of HKUST‐1 MOFs before and after loading a Eu3+ complex are analysed with the aid of luminescence spectroscopy (see graphic). The presence of an effective energy transfer between the HKUST‐1 framework and the Eu3+ centers was found as is described herein. |
| Author | Arslan, Hasan Kemal Ladnorg, Tatjana Shekhah, Osama Adlung, Matthias Franzreb, Matthias Stammer, Xia Gliemann, Hartmut Wöll, Christof Zybaylo, Olexandra Wickleder, Claudia Streit, Huayna Cerqueira |
| Author_xml | – sequence: 1 givenname: Huayna Cerqueira surname: Streit fullname: Streit, Huayna Cerqueira organization: Inorganic Chemistry, Science and Engineering, University of Siegen, Adolf-Reichwein-Straße 2, 57076 Siegen (Germany) – sequence: 2 givenname: Matthias surname: Adlung fullname: Adlung, Matthias organization: Inorganic Chemistry, Science and Engineering, University of Siegen, Adolf-Reichwein-Straße 2, 57076 Siegen (Germany) – sequence: 3 givenname: Osama surname: Shekhah fullname: Shekhah, Osama organization: Institute of Functional Interfaces (IFG), Karlsruhe Institute of Technology (KIT), 76021 Karlsruhe (Germany) – sequence: 4 givenname: Xia surname: Stammer fullname: Stammer, Xia organization: Institute of Functional Interfaces (IFG), Karlsruhe Institute of Technology (KIT), 76021 Karlsruhe (Germany) – sequence: 5 givenname: Hasan Kemal surname: Arslan fullname: Arslan, Hasan Kemal organization: Institute of Functional Interfaces (IFG), Karlsruhe Institute of Technology (KIT), 76021 Karlsruhe (Germany) – sequence: 6 givenname: Olexandra surname: Zybaylo fullname: Zybaylo, Olexandra organization: Institute of Functional Interfaces (IFG), Karlsruhe Institute of Technology (KIT), 76021 Karlsruhe (Germany) – sequence: 7 givenname: Tatjana surname: Ladnorg fullname: Ladnorg, Tatjana organization: Institute of Functional Interfaces (IFG), Karlsruhe Institute of Technology (KIT), 76021 Karlsruhe (Germany) – sequence: 8 givenname: Hartmut surname: Gliemann fullname: Gliemann, Hartmut organization: Institute of Functional Interfaces (IFG), Karlsruhe Institute of Technology (KIT), 76021 Karlsruhe (Germany) – sequence: 9 givenname: Matthias surname: Franzreb fullname: Franzreb, Matthias organization: Institute of Functional Interfaces (IFG), Karlsruhe Institute of Technology (KIT), 76021 Karlsruhe (Germany) – sequence: 10 givenname: Christof surname: Wöll fullname: Wöll, Christof email: Christof.woell@kit.edu organization: Institute of Functional Interfaces (IFG), Karlsruhe Institute of Technology (KIT), 76021 Karlsruhe (Germany) – sequence: 11 givenname: Claudia surname: Wickleder fullname: Wickleder, Claudia email: wickleder@chemie.uni-siegen.de organization: Inorganic Chemistry, Science and Engineering, University of Siegen, Adolf-Reichwein-Straße 2, 57076 Siegen (Germany) |
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| Keywords | Metal organic framework photonic antenna europium complexes Rare earth metal complex Luminescence Organic ligand Europium complex Energy transfer surface-anchored metalorganic frameworks |
| Language | English |
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| Snippet | The loading of a metal‐organic framework (MOF), [Cu3(btc)2xH2O] HKUST‐1, with europium β‐diketonate complexes is studied with the goal to using the porous... The loading of a metal-organic framework (MOF), [Cu(3)(btc)(2)xH(2)O] HKUST-1, with europium β-diketonate complexes is studied with the goal to using the... Abstract The loading of a metal‐organic framework (MOF), [Cu 3 (btc) 2 x H 2 O] HKUST‐1, with europium β‐diketonate complexes is studied with the goal to using... |
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| SubjectTerms | Chemistry energy transfer europium complexes Exact sciences and technology General and physical chemistry luminescence photonic antennae Surface physical chemistry surface-anchored metal-organic frameworks |
| Title | Surface-Anchored MOF-Based Photonic Antennae |
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