Transport and Retention of Poly(Acrylic Acid-co-Maleic Acid) Coated Magnetite Nanoparticles in Porous Media: Effect of Input Concentration, Ionic Strength and Grain Size
Understanding the physicochemical factors affecting nanoparticle transport in porous media is critical for their environmental application. Water-saturated column experiments were conducted to investigate the effects of input concentration (Co), ionic strength (IS), and sand grain size on the transp...
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| Published in | Nanomaterials (Basel, Switzerland) Vol. 12; no. 9; p. 1536 |
|---|---|
| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Switzerland
MDPI AG
02.05.2022
MDPI |
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| Online Access | Get full text |
| ISSN | 2079-4991 2079-4991 |
| DOI | 10.3390/nano12091536 |
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| Abstract | Understanding the physicochemical factors affecting nanoparticle transport in porous media is critical for their environmental application. Water-saturated column experiments were conducted to investigate the effects of input concentration (Co), ionic strength (IS), and sand grain size on the transport of poly(acrylic acid-co-maleic acid) coated magnetite nanoparticles (PAM@MNP). Mass recoveries in the column effluent ranged from 45.2 to 99.3%. The highest relative retention of PAM@MNP was observed for the lowest Co. Smaller Co also resulted in higher relative retention (39.8%) when IS increased to 10 mM. However, relative retention became much less sensitive to solution IS as Co increased. The high mobility is attributed to the PAM coating provoking steric stability of PAM@MNP against homoaggregation. PAM@MNP retention was about 10-fold higher for smaller grain sizes, i.e., 240 µm and 350 µm versus 607 µm. The simulated maximum retained concentration on the solid phase (Smax) and retention rate coefficient (k1) increased with decreasing Co and grain sizes, reflecting higher retention rates at these parameters. The study revealed under various IS for the first time the high mobility premise of polymer-coated magnetite nanoparticles at realistic (<10 mg L−1) environmental concentrations, thereby highlighting an untapped potential for novel environmental PAM@MNP application usage. |
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| AbstractList | Understanding the physicochemical factors affecting nanoparticle transport in porous media is critical for their environmental application. Water-saturated column experiments were conducted to investigate the effects of input concentration (Co), ionic strength (IS), and sand grain size on the transport of poly(acrylic acid-co-maleic acid) coated magnetite nanoparticles (PAM@MNP). Mass recoveries in the column effluent ranged from 45.2 to 99.3%. The highest relative retention of PAM@MNP was observed for the lowest Co. Smaller Co also resulted in higher relative retention (39.8%) when IS increased to 10 mM. However, relative retention became much less sensitive to solution IS as Co increased. The high mobility is attributed to the PAM coating provoking steric stability of PAM@MNP against homoaggregation. PAM@MNP retention was about 10-fold higher for smaller grain sizes, i.e., 240 µm and 350 µm versus 607 µm. The simulated maximum retained concentration on the solid phase (Smax) and retention rate coefficient (k1) increased with decreasing Co and grain sizes, reflecting higher retention rates at these parameters. The study revealed under various IS for the first time the high mobility premise of polymer-coated magnetite nanoparticles at realistic (<10 mg L−1) environmental concentrations, thereby highlighting an untapped potential for novel environmental PAM@MNP application usage. Understanding the physicochemical factors affecting nanoparticle transport in porous media is critical for their environmental application. Water-saturated column experiments were conducted to investigate the effects of input concentration (Co), ionic strength (IS), and sand grain size on the transport of poly(acrylic acid-co-maleic acid) coated magnetite nanoparticles (PAM@MNP). Mass recoveries in the column effluent ranged from 45.2 to 99.3%. The highest relative retention of PAM@MNP was observed for the lowest Co. Smaller Co also resulted in higher relative retention (39.8%) when IS increased to 10 mM. However, relative retention became much less sensitive to solution IS as Co increased. The high mobility is attributed to the PAM coating provoking steric stability of PAM@MNP against homoaggregation. PAM@MNP retention was about 10-fold higher for smaller grain sizes, i.e., 240 µm and 350 µm versus 607 µm. The simulated maximum retained concentration on the solid phase (Smax) and retention rate coefficient (k1) increased with decreasing Co and grain sizes, reflecting higher retention rates at these parameters. The study revealed under various IS for the first time the high mobility premise of polymer-coated magnetite nanoparticles at realistic (<10 mg L−1) environmental concentrations, thereby highlighting an untapped potential for novel environmental PAM@MNP application usage.Understanding the physicochemical factors affecting nanoparticle transport in porous media is critical for their environmental application. Water-saturated column experiments were conducted to investigate the effects of input concentration (Co), ionic strength (IS), and sand grain size on the transport of poly(acrylic acid-co-maleic acid) coated magnetite nanoparticles (PAM@MNP). Mass recoveries in the column effluent ranged from 45.2 to 99.3%. The highest relative retention of PAM@MNP was observed for the lowest Co. Smaller Co also resulted in higher relative retention (39.8%) when IS increased to 10 mM. However, relative retention became much less sensitive to solution IS as Co increased. The high mobility is attributed to the PAM coating provoking steric stability of PAM@MNP against homoaggregation. PAM@MNP retention was about 10-fold higher for smaller grain sizes, i.e., 240 µm and 350 µm versus 607 µm. The simulated maximum retained concentration on the solid phase (Smax) and retention rate coefficient (k1) increased with decreasing Co and grain sizes, reflecting higher retention rates at these parameters. The study revealed under various IS for the first time the high mobility premise of polymer-coated magnetite nanoparticles at realistic (<10 mg L−1) environmental concentrations, thereby highlighting an untapped potential for novel environmental PAM@MNP application usage. Understanding the physicochemical factors affecting nanoparticle transport in porous media is critical for their environmental application. Water-saturated column experiments were conducted to investigate the effects of input concentration (Co), ionic strength (IS), and sand grain size on the transport of poly(acrylic acid-co-maleic acid) coated magnetite nanoparticles (PAM@MNP). Mass recoveries in the column effluent ranged from 45.2 to 99.3%. The highest relative retention of PAM@MNP was observed for the lowest Co. Smaller Co also resulted in higher relative retention (39.8%) when IS increased to 10 mM. However, relative retention became much less sensitive to solution IS as Co increased. The high mobility is attributed to the PAM coating provoking steric stability of PAM@MNP against homoaggregation. PAM@MNP retention was about 10-fold higher for smaller grain sizes, i.e., 240 µm and 350 µm versus 607 µm. The simulated maximum retained concentration on the solid phase (Smax) and retention rate coefficient (k1) increased with decreasing Co and grain sizes, reflecting higher retention rates at these parameters. The study revealed under various IS for the first time the high mobility premise of polymer-coated magnetite nanoparticles at realistic (<10 mg L −1 ) environmental concentrations, thereby highlighting an untapped potential for novel environmental PAM@MNP application usage. |
| Author | Klumpp, Erwin Liang, Yan Zhang, Miaoyue Mlih, Rawan Tombácz, Etelka Bol, Roland |
| AuthorAffiliation | 5 Soós Ernő Water Technology Research and Development Center, University of Pannonia, H-8800 Nagykanizsa, Hungary; e.tombacz@chem.u-szeged.hu 1 Institute of Bio- and Geosciences, Agrosphere (IBG–3), Research Centre Juelich (FZJ), 52425 Juelich, Germany; r.bol@fz-juelich.de (R.B.); e.klumpp@fz-juelich.de (E.K.) 2 Institute for Environmental Research, Biology 5, RWTH Aachen University, 52074 Aachen, Germany 4 School of Environmental Science and Engineering, Sun Yat-sen University, Guangzhou 510006, China; zhangmy53@mail.sysu.edu.cn 6 School of Natural Sciences, Environment Centre Wales, Bangor University, Bangor LL57 2DG, UK 3 School of Resources, Environment and Materials, Guangxi University, Nanning 530004, China; liangyan@gxu.edu.cn |
| AuthorAffiliation_xml | – name: 2 Institute for Environmental Research, Biology 5, RWTH Aachen University, 52074 Aachen, Germany – name: 4 School of Environmental Science and Engineering, Sun Yat-sen University, Guangzhou 510006, China; zhangmy53@mail.sysu.edu.cn – name: 5 Soós Ernő Water Technology Research and Development Center, University of Pannonia, H-8800 Nagykanizsa, Hungary; e.tombacz@chem.u-szeged.hu – name: 3 School of Resources, Environment and Materials, Guangxi University, Nanning 530004, China; liangyan@gxu.edu.cn – name: 6 School of Natural Sciences, Environment Centre Wales, Bangor University, Bangor LL57 2DG, UK – name: 1 Institute of Bio- and Geosciences, Agrosphere (IBG–3), Research Centre Juelich (FZJ), 52425 Juelich, Germany; r.bol@fz-juelich.de (R.B.); e.klumpp@fz-juelich.de (E.K.) |
| Author_xml | – sequence: 1 givenname: Rawan surname: Mlih fullname: Mlih, Rawan – sequence: 2 givenname: Yan surname: Liang fullname: Liang, Yan – sequence: 3 givenname: Miaoyue orcidid: 0000-0002-2939-6665 surname: Zhang fullname: Zhang, Miaoyue – sequence: 4 givenname: Etelka orcidid: 0000-0002-2068-0459 surname: Tombácz fullname: Tombácz, Etelka – sequence: 5 givenname: Roland orcidid: 0000-0003-3015-7706 surname: Bol fullname: Bol, Roland – sequence: 6 givenname: Erwin surname: Klumpp fullname: Klumpp, Erwin |
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| CitedBy_id | crossref_primary_10_3389_fenvs_2022_1114940 crossref_primary_10_1016_j_chemosphere_2024_143259 |
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| Title | Transport and Retention of Poly(Acrylic Acid-co-Maleic Acid) Coated Magnetite Nanoparticles in Porous Media: Effect of Input Concentration, Ionic Strength and Grain Size |
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