Light-driven water oxidation for solar fuels

. [Display omitted] ► Anodes for light-driven water oxidation. ► Design includes semiconductor, light-harvesting molecule, and catalyst. ► Integration of components is greatest challenge. Light-driven water oxidation is an essential step for conversion of sunlight into storable chemical fuels. Fujis...

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Published in	Coordination chemistry reviews Vol. 256; no. 21-22; pp. 2503 - 2520
Main Authors	Young, Karin J., Martini, Lauren A., Milot, Rebecca L., Snoeberger, Robert C., Batista, Victor S., Schmuttenmaer, Charles A., Crabtree, Robert H., Brudvig, Gary W.
Format	Journal Article
Language	English
Published	Switzerland Elsevier B.V 01.11.2012
Subjects	Artificial photosynthesis Solar fuels Water splitting FTO BODIPY TW ITO salen EPR PSII PCET VCS HOMO LUMO NHE D-π-A PVP XRD Cp FITC DFT Solar fuels t-tpy bpy-Mebim2py bpmp UV GC–MS Water splitting bpp bpy IPCE OEC tacn MLCT Artificial photosynthesis Acac tpy DC DSSC
Online Access	Get full text
ISSN	0010-8545 1873-3840
DOI	10.1016/j.ccr.2012.03.031

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Abstract	. [Display omitted] ► Anodes for light-driven water oxidation. ► Design includes semiconductor, light-harvesting molecule, and catalyst. ► Integration of components is greatest challenge. Light-driven water oxidation is an essential step for conversion of sunlight into storable chemical fuels. Fujishima and Honda reported the first example of photoelectrochemical water oxidation in 1972. In their system, TiO2 was irradiated with ultraviolet light, producing oxygen at the anode and hydrogen at a platinum cathode. Inspired by this system, more recent work has focused on functionalizing nanoporous TiO2 or other semiconductor surfaces with molecular adsorbates, including chromophores and catalysts that absorb visible light and generate electricity (i.e., dye-sensitized solar cells) or trigger water oxidation at low overpotentials (i.e., photocatalytic cells). The physics involved in harnessing multiple photochemical events for multi-electron reactions, as required in the four-electron water-oxidation process, has been the subject of much experimental and computational study. In spite of significant advances with regard to individual components, the development of highly efficient photocatalytic cells for solar water splitting remains an outstanding challenge. This article reviews recent progress in the field with emphasis on water-oxidation photoanodes inspired by the design of functionalized thin-film semiconductors of typical dye-sensitized solar cells.
AbstractList	Light-driven water oxidation is an essential step for conversion of sunlight into storable chemical fuels. Fujishima and Honda reported the first example of photoelectrochemical water oxidation in 1972. In their system, TiO2 was irradiated with ultraviolet light, producing oxygen at the anode and hydrogen at a platinum cathode. Inspired by this system, more recent work has focused on functionalizing nanoporous TiO2 or other semiconductor surfaces with molecular adsorbates, including chromophores and catalysts that absorb visible light and generate electricity (i.e., dye-sensitized solar cells) or trigger water oxidation at low overpotentials (i.e., photocatalytic cells). The physics involved in harnessing multiple photochemical events for multielectron reactions, as required in the four-electron water oxidation process, has been the subject of much experimental and computational study. In spite of significant advances with regard to individual components, the development of highly efficient photocatalytic cells for solar water splitting remains an outstanding challenge. This article reviews recent progress in the field with emphasis on water-oxidation photoanodes inspired by the design of functionalized thin film semiconductors of typical dye-sensitized solar cells.Light-driven water oxidation is an essential step for conversion of sunlight into storable chemical fuels. Fujishima and Honda reported the first example of photoelectrochemical water oxidation in 1972. In their system, TiO2 was irradiated with ultraviolet light, producing oxygen at the anode and hydrogen at a platinum cathode. Inspired by this system, more recent work has focused on functionalizing nanoporous TiO2 or other semiconductor surfaces with molecular adsorbates, including chromophores and catalysts that absorb visible light and generate electricity (i.e., dye-sensitized solar cells) or trigger water oxidation at low overpotentials (i.e., photocatalytic cells). The physics involved in harnessing multiple photochemical events for multielectron reactions, as required in the four-electron water oxidation process, has been the subject of much experimental and computational study. In spite of significant advances with regard to individual components, the development of highly efficient photocatalytic cells for solar water splitting remains an outstanding challenge. This article reviews recent progress in the field with emphasis on water-oxidation photoanodes inspired by the design of functionalized thin film semiconductors of typical dye-sensitized solar cells. Light-driven water oxidation is an essential step for conversion of sunlight into storable chemical fuels. Fujishima and Honda reported the first example of photoelectrochemical water oxidation in 1972. In their system, TiO was irradiated with ultraviolet light, producing oxygen at the anode and hydrogen at a platinum cathode. Inspired by this system, more recent work has focused on functionalizing nanoporous TiO or other semiconductor surfaces with molecular adsorbates, including chromophores and catalysts that absorb visible light and generate electricity ( , dye-sensitized solar cells) or trigger water oxidation at low overpotentials ( , photocatalytic cells). The physics involved in harnessing multiple photochemical events for multielectron reactions, as required in the four-electron water oxidation process, has been the subject of much experimental and computational study. In spite of significant advances with regard to individual components, the development of highly efficient photocatalytic cells for solar water splitting remains an outstanding challenge. This article reviews recent progress in the field with emphasis on water-oxidation photoanodes inspired by the design of functionalized thin film semiconductors of typical dye-sensitized solar cells. . [Display omitted] ► Anodes for light-driven water oxidation. ► Design includes semiconductor, light-harvesting molecule, and catalyst. ► Integration of components is greatest challenge. Light-driven water oxidation is an essential step for conversion of sunlight into storable chemical fuels. Fujishima and Honda reported the first example of photoelectrochemical water oxidation in 1972. In their system, TiO2 was irradiated with ultraviolet light, producing oxygen at the anode and hydrogen at a platinum cathode. Inspired by this system, more recent work has focused on functionalizing nanoporous TiO2 or other semiconductor surfaces with molecular adsorbates, including chromophores and catalysts that absorb visible light and generate electricity (i.e., dye-sensitized solar cells) or trigger water oxidation at low overpotentials (i.e., photocatalytic cells). The physics involved in harnessing multiple photochemical events for multi-electron reactions, as required in the four-electron water-oxidation process, has been the subject of much experimental and computational study. In spite of significant advances with regard to individual components, the development of highly efficient photocatalytic cells for solar water splitting remains an outstanding challenge. This article reviews recent progress in the field with emphasis on water-oxidation photoanodes inspired by the design of functionalized thin-film semiconductors of typical dye-sensitized solar cells. Light-driven water oxidation is an essential step for conversion of sunlight into storable chemical fuels. Fujishima and Honda reported the first example of photoelectrochemical water oxidation in 1972. In their system, TiO 2 was irradiated with ultraviolet light, producing oxygen at the anode and hydrogen at a platinum cathode. Inspired by this system, more recent work has focused on functionalizing nanoporous TiO 2 or other semiconductor surfaces with molecular adsorbates, including chromophores and catalysts that absorb visible light and generate electricity ( i.e. , dye-sensitized solar cells) or trigger water oxidation at low overpotentials ( i.e. , photocatalytic cells). The physics involved in harnessing multiple photochemical events for multielectron reactions, as required in the four-electron water oxidation process, has been the subject of much experimental and computational study. In spite of significant advances with regard to individual components, the development of highly efficient photocatalytic cells for solar water splitting remains an outstanding challenge. This article reviews recent progress in the field with emphasis on water-oxidation photoanodes inspired by the design of functionalized thin film semiconductors of typical dye-sensitized solar cells.
Author	Milot, Rebecca L. Brudvig, Gary W. Martini, Lauren A. Batista, Victor S. Snoeberger, Robert C. Schmuttenmaer, Charles A. Young, Karin J. Crabtree, Robert H.
Author_xml	– sequence: 1 givenname: Karin J. surname: Young fullname: Young, Karin J. – sequence: 2 givenname: Lauren A. surname: Martini fullname: Martini, Lauren A. – sequence: 3 givenname: Rebecca L. surname: Milot fullname: Milot, Rebecca L. – sequence: 4 givenname: Robert C. surname: Snoeberger fullname: Snoeberger, Robert C. – sequence: 5 givenname: Victor S. surname: Batista fullname: Batista, Victor S. email: victor.batista@yale.edu – sequence: 6 givenname: Charles A. surname: Schmuttenmaer fullname: Schmuttenmaer, Charles A. email: charles.schmuttenmaer@yale.edu – sequence: 7 givenname: Robert H. surname: Crabtree fullname: Crabtree, Robert H. email: robert.crabtree@yale.edu – sequence: 8 givenname: Gary W. surname: Brudvig fullname: Brudvig, Gary W. email: gary.brudvig@yale.edu
BackLink	https://www.ncbi.nlm.nih.gov/pubmed/25364029$$D View this record in MEDLINE/PubMed
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Snippet	. [Display omitted] ► Anodes for light-driven water oxidation. ► Design includes semiconductor, light-harvesting molecule, and catalyst. ► Integration of... Light-driven water oxidation is an essential step for conversion of sunlight into storable chemical fuels. Fujishima and Honda reported the first example of...
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SubjectTerms	Artificial photosynthesis Solar fuels Water splitting
Title	Light-driven water oxidation for solar fuels
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