Photocatalytic degradation of sulfamethazine using a direct Z-Scheme AgI/Bi4V2O11 photocatalyst: Mineralization activity, degradation pathways and promoted charge separation mechanism
[Display omitted] •Novel direct Z-scheme AgI/Bi4V2O11 photocatalysts were prepared.•A superior photocatalytic activity for the degradation of SMZ refractory pollutants.•A plausible degradation pathway for SMZ was proposed.•The fabrication Z-scheme heterostructure play a central role in promoting cha...
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| Published in | Journal of hazardous materials Vol. 385; p. 121508 |
|---|---|
| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
05.03.2020
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| Subjects | |
| Online Access | Get full text |
| ISSN | 0304-3894 1873-3336 1873-3336 |
| DOI | 10.1016/j.jhazmat.2019.121508 |
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| Abstract | [Display omitted]
•Novel direct Z-scheme AgI/Bi4V2O11 photocatalysts were prepared.•A superior photocatalytic activity for the degradation of SMZ refractory pollutants.•A plausible degradation pathway for SMZ was proposed.•The fabrication Z-scheme heterostructure play a central role in promoting charge separation and active radical generation.
Z-scheme heterojunction can not only promote the separation of photogenerated carriers, but also retain the strong redox potential of the system, which would greatly improve the photocatalytic performance of catalyst. Herein, a Z-scheme AgI/Bi4V2O11 heterojunction photocatalyst was prepared by a hydrothermal process combined with in situ coprecipitation process. Multiple techniques were employed to investigate the morphology, composition, chemical and electronic properties of the as-prepared samples. The obtained Z-scheme AgI/Bi4V2O11 heterojunction photocatalyst exhibited remarkably enhanced photocatalytic performance towards sulfamethazine (SMZ) degradation under visible light irradiation. Especially, the 20 wt% AgI/Bi4V2O11 composites exhibited the highest photocatalytic activity for sulfamethazine (SMZ) degradation and 91.47% SMZ would be eliminated within 60 min. In comparison with NO3− and SO42−, the presence of Cl− and HCO3− presented more obviously inhibition effects on SMZ degradation. The possible degradation pathways of SMZ were speculated by identifying degradation intermediates. O2−, h+ and OH all involved in the photocatalytic degradation SMZ. The highly enhanced photocatalytic performance might be attributed to form Z-scheme junction between AgI and BVO, which are conducive to the efficient charges separation and maintain high redox potential. This work enriches Bi4V2O11-based Z-scheme heterojunction photocatalytic system and provides a reference for the preparation of effective Z-scheme junction photocatalysts. |
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| AbstractList | Z-scheme heterojunction can not only promote the separation of photogenerated carriers, but also retain the strong redox potential of the system, which would greatly improve the photocatalytic performance of catalyst. Herein, a Z-scheme AgI/Bi4V2O11 heterojunction photocatalyst was prepared by a hydrothermal process combined with in situ coprecipitation process. Multiple techniques were employed to investigate the morphology, composition, chemical and electronic properties of the as-prepared samples. The obtained Z-scheme AgI/Bi4V2O11 heterojunction photocatalyst exhibited remarkably enhanced photocatalytic performance towards sulfamethazine (SMZ) degradation under visible light irradiation. Especially, the 20 wt% AgI/Bi4V2O11 composites exhibited the highest photocatalytic activity for sulfamethazine (SMZ) degradation and 91.47% SMZ would be eliminated within 60 min. In comparison with NO3- and SO42-, the presence of Cl- and HCO3- presented more obviously inhibition effects on SMZ degradation. The possible degradation pathways of SMZ were speculated by identifying degradation intermediates. O2-, h+ and OH all involved in the photocatalytic degradation SMZ. The highly enhanced photocatalytic performance might be attributed to form Z-scheme junction between AgI and BVO, which are conducive to the efficient charges separation and maintain high redox potential. This work enriches Bi4V2O11-based Z-scheme heterojunction photocatalytic system and provides a reference for the preparation of effective Z-scheme junction photocatalysts.Z-scheme heterojunction can not only promote the separation of photogenerated carriers, but also retain the strong redox potential of the system, which would greatly improve the photocatalytic performance of catalyst. Herein, a Z-scheme AgI/Bi4V2O11 heterojunction photocatalyst was prepared by a hydrothermal process combined with in situ coprecipitation process. Multiple techniques were employed to investigate the morphology, composition, chemical and electronic properties of the as-prepared samples. The obtained Z-scheme AgI/Bi4V2O11 heterojunction photocatalyst exhibited remarkably enhanced photocatalytic performance towards sulfamethazine (SMZ) degradation under visible light irradiation. Especially, the 20 wt% AgI/Bi4V2O11 composites exhibited the highest photocatalytic activity for sulfamethazine (SMZ) degradation and 91.47% SMZ would be eliminated within 60 min. In comparison with NO3- and SO42-, the presence of Cl- and HCO3- presented more obviously inhibition effects on SMZ degradation. The possible degradation pathways of SMZ were speculated by identifying degradation intermediates. O2-, h+ and OH all involved in the photocatalytic degradation SMZ. The highly enhanced photocatalytic performance might be attributed to form Z-scheme junction between AgI and BVO, which are conducive to the efficient charges separation and maintain high redox potential. This work enriches Bi4V2O11-based Z-scheme heterojunction photocatalytic system and provides a reference for the preparation of effective Z-scheme junction photocatalysts. Z-scheme heterojunction can not only promote the separation of photogenerated carriers, but also retain the strong redox potential of the system, which would greatly improve the photocatalytic performance of catalyst. Herein, a Z-scheme AgI/Bi₄V₂O₁₁ heterojunction photocatalyst was prepared by a hydrothermal process combined with in situ coprecipitation process. Multiple techniques were employed to investigate the morphology, composition, chemical and electronic properties of the as-prepared samples. The obtained Z-scheme AgI/Bi₄V₂O₁₁ heterojunction photocatalyst exhibited remarkably enhanced photocatalytic performance towards sulfamethazine (SMZ) degradation under visible light irradiation. Especially, the 20 wt% AgI/Bi₄V₂O₁₁ composites exhibited the highest photocatalytic activity for sulfamethazine (SMZ) degradation and 91.47% SMZ would be eliminated within 60 min. In comparison with NO₃⁻ and SO₄²⁻, the presence of Cl⁻ and HCO₃⁻ presented more obviously inhibition effects on SMZ degradation. The possible degradation pathways of SMZ were speculated by identifying degradation intermediates. O₂⁻, h⁺ and OH all involved in the photocatalytic degradation SMZ. The highly enhanced photocatalytic performance might be attributed to form Z-scheme junction between AgI and BVO, which are conducive to the efficient charges separation and maintain high redox potential. This work enriches Bi₄V₂O₁₁-based Z-scheme heterojunction photocatalytic system and provides a reference for the preparation of effective Z-scheme junction photocatalysts. [Display omitted] •Novel direct Z-scheme AgI/Bi4V2O11 photocatalysts were prepared.•A superior photocatalytic activity for the degradation of SMZ refractory pollutants.•A plausible degradation pathway for SMZ was proposed.•The fabrication Z-scheme heterostructure play a central role in promoting charge separation and active radical generation. Z-scheme heterojunction can not only promote the separation of photogenerated carriers, but also retain the strong redox potential of the system, which would greatly improve the photocatalytic performance of catalyst. Herein, a Z-scheme AgI/Bi4V2O11 heterojunction photocatalyst was prepared by a hydrothermal process combined with in situ coprecipitation process. Multiple techniques were employed to investigate the morphology, composition, chemical and electronic properties of the as-prepared samples. The obtained Z-scheme AgI/Bi4V2O11 heterojunction photocatalyst exhibited remarkably enhanced photocatalytic performance towards sulfamethazine (SMZ) degradation under visible light irradiation. Especially, the 20 wt% AgI/Bi4V2O11 composites exhibited the highest photocatalytic activity for sulfamethazine (SMZ) degradation and 91.47% SMZ would be eliminated within 60 min. In comparison with NO3− and SO42−, the presence of Cl− and HCO3− presented more obviously inhibition effects on SMZ degradation. The possible degradation pathways of SMZ were speculated by identifying degradation intermediates. O2−, h+ and OH all involved in the photocatalytic degradation SMZ. The highly enhanced photocatalytic performance might be attributed to form Z-scheme junction between AgI and BVO, which are conducive to the efficient charges separation and maintain high redox potential. This work enriches Bi4V2O11-based Z-scheme heterojunction photocatalytic system and provides a reference for the preparation of effective Z-scheme junction photocatalysts. |
| ArticleNumber | 121508 |
| Author | Guo, Jie Wen, Xiao-Ju Sun, Jie Qian-Lu Fei, Zheng-Hao Niu, Cheng-Gang Lv, Xiao-Xiao |
| Author_xml | – sequence: 1 givenname: Xiao-Ju orcidid: 0000-0002-6450-7244 surname: Wen fullname: Wen, Xiao-Ju email: wenxiaoju1990@126.com organization: School of Chemistry and Environmental Engineering, Yancheng Teachers University, Yancheng, Jiangsu Province, 224051, China – sequence: 2 surname: Qian-Lu fullname: Qian-Lu organization: School of Chemistry and Environmental Engineering, Yancheng Teachers University, Yancheng, Jiangsu Province, 224051, China – sequence: 3 givenname: Xiao-Xiao surname: Lv fullname: Lv, Xiao-Xiao email: lvxiaoxiao0120@163.com organization: Department of Transportation and Environment, Shenzhen Institute of Information Technology, Shenzhen, Guangdong Province, 518172, China – sequence: 4 givenname: Jie surname: Sun fullname: Sun, Jie organization: School of Chemistry and Environmental Engineering, Yancheng Teachers University, Yancheng, Jiangsu Province, 224051, China – sequence: 5 givenname: Jie surname: Guo fullname: Guo, Jie organization: School of Chemistry and Environmental Engineering, Yancheng Teachers University, Yancheng, Jiangsu Province, 224051, China – sequence: 6 givenname: Zheng-Hao surname: Fei fullname: Fei, Zheng-Hao organization: School of Chemistry and Environmental Engineering, Yancheng Teachers University, Yancheng, Jiangsu Province, 224051, China – sequence: 7 givenname: Cheng-Gang orcidid: 0000-0002-5904-9111 surname: Niu fullname: Niu, Cheng-Gang organization: College of Environmental Science Engineering, Hunan University, Changsha, Hunan province, 410082, China |
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•Novel direct Z-scheme AgI/Bi4V2O11 photocatalysts were prepared.•A superior photocatalytic activity for the degradation of SMZ refractory... Z-scheme heterojunction can not only promote the separation of photogenerated carriers, but also retain the strong redox potential of the system, which would... |
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| SubjectTerms | AgI/Bi4V2O11 bicarbonates chlorides coprecipitation irradiation light mineralization nitrates photocatalysis photocatalysts Photocatalytic redox potential Sulfamethazine sulfates superoxide anion Visible light Z-scheme |
| Title | Photocatalytic degradation of sulfamethazine using a direct Z-Scheme AgI/Bi4V2O11 photocatalyst: Mineralization activity, degradation pathways and promoted charge separation mechanism |
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