Review on Li Deposition in Working Batteries: From Nucleation to Early Growth

Lithium (Li) metal is one of the most promising alternative anode materials of next‐generation high‐energy‐density batteries demanded for advanced energy storage in the coming fourth industrial revolution. Nevertheless, disordered Li deposition easily causes short lifespan and safety concerns and th...

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Published inAdvanced materials (Weinheim) Vol. 33; no. 8; pp. e2004128 - n/a
Main Authors Chen, Xiao‐Ru, Zhao, Bo‐Chen, Yan, Chong, Zhang, Qiang
Format Journal Article
LanguageEnglish
Published Germany Wiley Subscription Services, Inc 01.02.2021
Subjects
Anodes
Crystallography
dendrite inhibition
Dendritic structure
Deposition
Electrochemical analysis
Electrode materials
Energy storage
Lithium
lithium dendrite growth
lithium deposition
lithium metal batteries
Materials science
Morphology
Nucleation
Space charge
Storage batteries
Surface diffusion
nucleation
lithium deposition
lithium dendrite growth
dendrite inhibition
lithium metal batteries
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Abstract Lithium (Li) metal is one of the most promising alternative anode materials of next‐generation high‐energy‐density batteries demanded for advanced energy storage in the coming fourth industrial revolution. Nevertheless, disordered Li deposition easily causes short lifespan and safety concerns and thus severely hinders the practical applications of Li metal batteries. Tremendous efforts are devoted to understanding the mechanism for Li deposition, while the final deposition morphology tightly relies on the Li nucleation and early growth. Here, the recent progress in insightful and influential models proposed to understand the process of Li deposition from nucleation to early growth, including the heterogeneous model, surface diffusion model, crystallography model, space charge model, and Li‐SEI model, are highlighted. Inspired by the abovementioned understanding on Li nucleation and early growth, diverse anode‐design strategies, which contribute to better batteries with superior electrochemical performance and dendrite‐free deposition behavior, are also summarized. This work broadens the horizon for practical Li metal batteries and also sheds light on more understanding of other important metal‐based batteries involving the metal deposition process. Lithium (Li) nucleation and early growth processes significantly determine the final deposition behavior. The recent progress in influential models proposed to understand the process of Li nucleation and early growth is highlighted. Inspired by the abovementioned understanding, diverse anode‐design strategies, which contribute to better batteries with superior electrochemical performance and dendrite‐free deposition behavior, are also summarized.
AbstractList Lithium (Li) metal is one of the most promising alternative anode materials of next-generation high-energy-density batteries demanded for advanced energy storage in the coming fourth industrial revolution. Nevertheless, disordered Li deposition easily causes short lifespan and safety concerns and thus severely hinders the practical applications of Li metal batteries. Tremendous efforts are devoted to understanding the mechanism for Li deposition, while the final deposition morphology tightly relies on the Li nucleation and early growth. Here, the recent progress in insightful and influential models proposed to understand the process of Li deposition from nucleation to early growth, including the heterogeneous model, surface diffusion model, crystallography model, space charge model, and Li-SEI model, are highlighted. Inspired by the abovementioned understanding on Li nucleation and early growth, diverse anode-design strategies, which contribute to better batteries with superior electrochemical performance and dendrite-free deposition behavior, are also summarized. This work broadens the horizon for practical Li metal batteries and also sheds light on more understanding of other important metal-based batteries involving the metal deposition process.Lithium (Li) metal is one of the most promising alternative anode materials of next-generation high-energy-density batteries demanded for advanced energy storage in the coming fourth industrial revolution. Nevertheless, disordered Li deposition easily causes short lifespan and safety concerns and thus severely hinders the practical applications of Li metal batteries. Tremendous efforts are devoted to understanding the mechanism for Li deposition, while the final deposition morphology tightly relies on the Li nucleation and early growth. Here, the recent progress in insightful and influential models proposed to understand the process of Li deposition from nucleation to early growth, including the heterogeneous model, surface diffusion model, crystallography model, space charge model, and Li-SEI model, are highlighted. Inspired by the abovementioned understanding on Li nucleation and early growth, diverse anode-design strategies, which contribute to better batteries with superior electrochemical performance and dendrite-free deposition behavior, are also summarized. This work broadens the horizon for practical Li metal batteries and also sheds light on more understanding of other important metal-based batteries involving the metal deposition process.
Lithium (Li) metal is one of the most promising alternative anode materials of next-generation high-energy-density batteries demanded for advanced energy storage in the coming fourth industrial revolution. Nevertheless, disordered Li deposition easily causes short lifespan and safety concerns and thus severely hinders the practical applications of Li metal batteries. Tremendous efforts are devoted to understanding the mechanism for Li deposition, while the final deposition morphology tightly relies on the Li nucleation and early growth. Here, the recent progress in insightful and influential models proposed to understand the process of Li deposition from nucleation to early growth, including the heterogeneous model, surface diffusion model, crystallography model, space charge model, and Li-SEI model, are highlighted. Inspired by the abovementioned understanding on Li nucleation and early growth, diverse anode-design strategies, which contribute to better batteries with superior electrochemical performance and dendrite-free deposition behavior, are also summarized. This work broadens the horizon for practical Li metal batteries and also sheds light on more understanding of other important metal-based batteries involving the metal deposition process.
Lithium (Li) metal is one of the most promising alternative anode materials of next‐generation high‐energy‐density batteries demanded for advanced energy storage in the coming fourth industrial revolution. Nevertheless, disordered Li deposition easily causes short lifespan and safety concerns and thus severely hinders the practical applications of Li metal batteries. Tremendous efforts are devoted to understanding the mechanism for Li deposition, while the final deposition morphology tightly relies on the Li nucleation and early growth. Here, the recent progress in insightful and influential models proposed to understand the process of Li deposition from nucleation to early growth, including the heterogeneous model, surface diffusion model, crystallography model, space charge model, and Li‐SEI model, are highlighted. Inspired by the abovementioned understanding on Li nucleation and early growth, diverse anode‐design strategies, which contribute to better batteries with superior electrochemical performance and dendrite‐free deposition behavior, are also summarized. This work broadens the horizon for practical Li metal batteries and also sheds light on more understanding of other important metal‐based batteries involving the metal deposition process. Lithium (Li) nucleation and early growth processes significantly determine the final deposition behavior. The recent progress in influential models proposed to understand the process of Li nucleation and early growth is highlighted. Inspired by the abovementioned understanding, diverse anode‐design strategies, which contribute to better batteries with superior electrochemical performance and dendrite‐free deposition behavior, are also summarized.
Author Chen, Xiao‐Ru
Zhao, Bo‐Chen
Zhang, Qiang
Yan, Chong
Author_xml – sequence: 1
  givenname: Xiao‐Ru
  surname: Chen
  fullname: Chen, Xiao‐Ru
  organization: Tsinghua University
– sequence: 2
  givenname: Bo‐Chen
  surname: Zhao
  fullname: Zhao, Bo‐Chen
  organization: Tsinghua University
– sequence: 3
  givenname: Chong
  surname: Yan
  fullname: Yan, Chong
  organization: Tsinghua University
– sequence: 4
  givenname: Qiang
  orcidid: 0000-0002-3929-1541
  surname: Zhang
  fullname: Zhang, Qiang
  email: zhang-qiang@mails.tsinghua.edu.cn
  organization: Tsinghua University
BackLink https://www.ncbi.nlm.nih.gov/pubmed/33432664$$D View this record in MEDLINE/PubMed
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Keywords nucleation
lithium deposition
lithium dendrite growth
dendrite inhibition
lithium metal batteries
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Snippet Lithium (Li) metal is one of the most promising alternative anode materials of next‐generation high‐energy‐density batteries demanded for advanced energy...
Lithium (Li) metal is one of the most promising alternative anode materials of next-generation high-energy-density batteries demanded for advanced energy...
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SubjectTerms Anodes
Crystallography
dendrite inhibition
Dendritic structure
Deposition
Electrochemical analysis
Electrode materials
Energy storage
Lithium
lithium dendrite growth
lithium deposition
lithium metal batteries
Materials science
Morphology
Nucleation
Space charge
Storage batteries
Surface diffusion
Title Review on Li Deposition in Working Batteries: From Nucleation to Early Growth
URI https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fadma.202004128
https://www.ncbi.nlm.nih.gov/pubmed/33432664
https://www.proquest.com/docview/2491837062
https://www.proquest.com/docview/2477265011
Volume 33
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