Hydrophobic, Flexible, and Lightweight MXene Foams for High‐Performance Electromagnetic‐Interference Shielding
Ultrathin, lightweight, and flexible electromagnetic‐interference (EMI) shielding materials are urgently required to manage increasingly serious radiation pollution. 2D transition‐metal carbides (MXenes) are considered promising alternatives to graphene for providing excellent EMI‐shielding performa...
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| Published in | Advanced materials (Weinheim) Vol. 29; no. 38 |
|---|---|
| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Germany
Wiley Subscription Services, Inc
01.10.2017
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Ultrathin, lightweight, and flexible electromagnetic‐interference (EMI) shielding materials are urgently required to manage increasingly serious radiation pollution. 2D transition‐metal carbides (MXenes) are considered promising alternatives to graphene for providing excellent EMI‐shielding performance due to their outstanding metallic electrical conductivity. However, the hydrophilicity of MXene films may affect their stability and reliability when applied in moist or wet environments. Herein, for the first time, an efficient and facile approach is reported to fabricate freestanding, flexible, and hydrophobic MXene foam with reasonable strength by assembling MXene sheets into films followed by a hydrazine‐induced foaming process. In striking contrast to well‐known hydrophilic MXene materials, the MXene foams surprisingly exhibit hydrophobic surfaces and outstanding water resistance and durability. More interestingly, a much enhanced EMI‐shielding effectiveness of ≈70 dB is achieved for the lightweight MXene foam as compared to its unfoamed film counterpart (53 dB) due to the highly efficient wave attenuation in the favorable porous structure. Therefore, the hydrophobic, flexible, and lightweight MXene foam with an excellent EMI‐shielding performance is highly promising for applications in aerospace and portable and wearable smart electronics.
A hydrophobic, lightweight, and flexible MXene foam is fabricated for the first time by a hydrazine‐induced foaming process. The hydrophobic porous structure affords an extraordinary water tolerance, good durability, and strong absorption capacity. A much enhanced electromagnetic‐interference shielding effectiveness of 70 dB is achieved for the MXene foam as compared to the corresponding unfoamed film, due to the favorable porous structure. |
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| AbstractList | Ultrathin, lightweight, and flexible electromagnetic-interference (EMI) shielding materials are urgently required to manage increasingly serious radiation pollution. 2D transition-metal carbides (MXenes) are considered promising alternatives to graphene for providing excellent EMI-shielding performance due to their outstanding metallic electrical conductivity. However, the hydrophilicity of MXene films may affect their stability and reliability when applied in moist or wet environments. Herein, for the first time, an efficient and facile approach is reported to fabricate freestanding, flexible, and hydrophobic MXene foam with reasonable strength by assembling MXene sheets into films followed by a hydrazine-induced foaming process. In striking contrast to well-known hydrophilic MXene materials, the MXene foams surprisingly exhibit hydrophobic surfaces and outstanding water resistance and durability. More interestingly, a much enhanced EMI-shielding effectiveness of ≈70 dB is achieved for the lightweight MXene foam as compared to its unfoamed film counterpart (53 dB) due to the highly efficient wave attenuation in the favorable porous structure. Therefore, the hydrophobic, flexible, and lightweight MXene foam with an excellent EMI-shielding performance is highly promising for applications in aerospace and portable and wearable smart electronics.Ultrathin, lightweight, and flexible electromagnetic-interference (EMI) shielding materials are urgently required to manage increasingly serious radiation pollution. 2D transition-metal carbides (MXenes) are considered promising alternatives to graphene for providing excellent EMI-shielding performance due to their outstanding metallic electrical conductivity. However, the hydrophilicity of MXene films may affect their stability and reliability when applied in moist or wet environments. Herein, for the first time, an efficient and facile approach is reported to fabricate freestanding, flexible, and hydrophobic MXene foam with reasonable strength by assembling MXene sheets into films followed by a hydrazine-induced foaming process. In striking contrast to well-known hydrophilic MXene materials, the MXene foams surprisingly exhibit hydrophobic surfaces and outstanding water resistance and durability. More interestingly, a much enhanced EMI-shielding effectiveness of ≈70 dB is achieved for the lightweight MXene foam as compared to its unfoamed film counterpart (53 dB) due to the highly efficient wave attenuation in the favorable porous structure. Therefore, the hydrophobic, flexible, and lightweight MXene foam with an excellent EMI-shielding performance is highly promising for applications in aerospace and portable and wearable smart electronics. Ultrathin, lightweight, and flexible electromagnetic‐interference (EMI) shielding materials are urgently required to manage increasingly serious radiation pollution. 2D transition‐metal carbides (MXenes) are considered promising alternatives to graphene for providing excellent EMI‐shielding performance due to their outstanding metallic electrical conductivity. However, the hydrophilicity of MXene films may affect their stability and reliability when applied in moist or wet environments. Herein, for the first time, an efficient and facile approach is reported to fabricate freestanding, flexible, and hydrophobic MXene foam with reasonable strength by assembling MXene sheets into films followed by a hydrazine‐induced foaming process. In striking contrast to well‐known hydrophilic MXene materials, the MXene foams surprisingly exhibit hydrophobic surfaces and outstanding water resistance and durability. More interestingly, a much enhanced EMI‐shielding effectiveness of ≈70 dB is achieved for the lightweight MXene foam as compared to its unfoamed film counterpart (53 dB) due to the highly efficient wave attenuation in the favorable porous structure. Therefore, the hydrophobic, flexible, and lightweight MXene foam with an excellent EMI‐shielding performance is highly promising for applications in aerospace and portable and wearable smart electronics. Ultrathin, lightweight, and flexible electromagnetic‐interference (EMI) shielding materials are urgently required to manage increasingly serious radiation pollution. 2D transition‐metal carbides (MXenes) are considered promising alternatives to graphene for providing excellent EMI‐shielding performance due to their outstanding metallic electrical conductivity. However, the hydrophilicity of MXene films may affect their stability and reliability when applied in moist or wet environments. Herein, for the first time, an efficient and facile approach is reported to fabricate freestanding, flexible, and hydrophobic MXene foam with reasonable strength by assembling MXene sheets into films followed by a hydrazine‐induced foaming process. In striking contrast to well‐known hydrophilic MXene materials, the MXene foams surprisingly exhibit hydrophobic surfaces and outstanding water resistance and durability. More interestingly, a much enhanced EMI‐shielding effectiveness of ≈70 dB is achieved for the lightweight MXene foam as compared to its unfoamed film counterpart (53 dB) due to the highly efficient wave attenuation in the favorable porous structure. Therefore, the hydrophobic, flexible, and lightweight MXene foam with an excellent EMI‐shielding performance is highly promising for applications in aerospace and portable and wearable smart electronics. A hydrophobic, lightweight, and flexible MXene foam is fabricated for the first time by a hydrazine‐induced foaming process. The hydrophobic porous structure affords an extraordinary water tolerance, good durability, and strong absorption capacity. A much enhanced electromagnetic‐interference shielding effectiveness of 70 dB is achieved for the MXene foam as compared to the corresponding unfoamed film, due to the favorable porous structure. Ultrathin, lightweight, and flexible electromagnetic-interference (EMI) shielding materials are urgently required to manage increasingly serious radiation pollution. 2D transition-metal carbides (MXenes) are considered promising alternatives to graphene for providing excellent EMI-shielding performance due to their outstanding metallic electrical conductivity. However, the hydrophilicity of MXene films may affect their stability and reliability when applied in moist or wet environments. Herein, for the first time, an efficient and facile approach is reported to fabricate freestanding, flexible, and hydrophobic MXene foam with reasonable strength by assembling MXene sheets into films followed by a hydrazine-induced foaming process. In striking contrast to well-known hydrophilic MXene materials, the MXene foams surprisingly exhibit hydrophobic surfaces and outstanding water resistance and durability. More interestingly, a much enhanced EMI-shielding effectiveness of [asymp]70 dB is achieved for the lightweight MXene foam as compared to its unfoamed film counterpart (53 dB) due to the highly efficient wave attenuation in the favorable porous structure. Therefore, the hydrophobic, flexible, and lightweight MXene foam with an excellent EMI-shielding performance is highly promising for applications in aerospace and portable and wearable smart electronics. |
| Author | Liu, Ji Liu, Yafeng Liu, Zhangshuo Yu, Zhong‐Zhen Zhou, Aiguo Sun, Renhui Zhang, Hao‐Bin |
| Author_xml | – sequence: 1 givenname: Ji surname: Liu fullname: Liu, Ji organization: Beijing University of Chemical Technology – sequence: 2 givenname: Hao‐Bin surname: Zhang fullname: Zhang, Hao‐Bin email: zhanghaobin@mail.buct.edu.cn organization: Beijing University of Chemical Technology – sequence: 3 givenname: Renhui surname: Sun fullname: Sun, Renhui organization: Beijing University of Chemical Technology – sequence: 4 givenname: Yafeng surname: Liu fullname: Liu, Yafeng organization: Beijing University of Chemical Technology – sequence: 5 givenname: Zhangshuo surname: Liu fullname: Liu, Zhangshuo organization: Beijing University of Chemical Technology – sequence: 6 givenname: Aiguo surname: Zhou fullname: Zhou, Aiguo organization: Henan Polytechnic University – sequence: 7 givenname: Zhong‐Zhen surname: Yu fullname: Yu, Zhong‐Zhen email: yuzz@mail.buct.edu.cn organization: Beijing University of Chemical Technology |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/28799671$$D View this record in MEDLINE/PubMed |
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| Snippet | Ultrathin, lightweight, and flexible electromagnetic‐interference (EMI) shielding materials are urgently required to manage increasingly serious radiation... Ultrathin, lightweight, and flexible electromagnetic-interference (EMI) shielding materials are urgently required to manage increasingly serious radiation... |
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| SubjectTerms | Avionics Electrical resistivity Electromagnetic interference electromagnetic‐interference shielding Foaming Foams hydrophobicity Lightweight Metal carbides MXene foam MXenes Water pollution Water resistance Wave attenuation Wearable technology Weight reduction |
| Title | Hydrophobic, Flexible, and Lightweight MXene Foams for High‐Performance Electromagnetic‐Interference Shielding |
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