Challenges and Perspectives for NASICON‐Type Electrode Materials for Advanced Sodium‐Ion Batteries
Sodium‐ion batteries (SIBs) have attracted increasing attention in the past decades, because of high overall abundance of precursors, their even geographical distribution, and low cost. Apart from inherent thermodynamic disadvantages, SIBs have to overcome multiple kinetic problems, such as fast cap...
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| Published in | Advanced materials (Weinheim) Vol. 29; no. 48 |
|---|---|
| Main Authors | , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Germany
Wiley Subscription Services, Inc
01.12.2017
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Sodium‐ion batteries (SIBs) have attracted increasing attention in the past decades, because of high overall abundance of precursors, their even geographical distribution, and low cost. Apart from inherent thermodynamic disadvantages, SIBs have to overcome multiple kinetic problems, such as fast capacity decay, low rate capacities and low Coulombic efficiencies. A special case is sodium super ion conductor (NASICON)‐based electrode materials as they exhibit – besides pronounced structural stability – exceptionally high ion conductivity, rendering them most promising for sodium storage. Owing to the limiting, comparatively low electronic conductivity, nano‐structuring is a prerequisite for achieving satisfactory rate‐capability. In this review, we analyze advantages and disadvantages of NASICON‐type electrode materials and highlight electrode structure design principles for obtaining the desired electrochemical performance. Moreover, we give an overview of recent approaches to enhance electrical conductivity and structural stability of cathode and anode materials based on NASICON structure. We believe that this review provides a pertinent insight into relevant design principles and inspires further research in this respect.
Sodium super ion conductor (NASICON)‐based electrode materials, exhibiting pronounced structural stability and exceptionally high ion conductivity are promising materials for sodium storage. Challenges and perspectives of NASICON‐type electrode materials are discussed, and electrode structure design principles for obtaining the desired electrochemical performance are highlighted. Recent progress in enhancing electrical conductivity and structural stability of NASICON materials is summarized. |
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| AbstractList | Sodium‐ion batteries (SIBs) have attracted increasing attention in the past decades, because of high overall abundance of precursors, their even geographical distribution, and low cost. Apart from inherent thermodynamic disadvantages, SIBs have to overcome multiple kinetic problems, such as fast capacity decay, low rate capacities and low Coulombic efficiencies. A special case is sodium super ion conductor (NASICON)‐based electrode materials as they exhibit – besides pronounced structural stability – exceptionally high ion conductivity, rendering them most promising for sodium storage. Owing to the limiting, comparatively low electronic conductivity, nano‐structuring is a prerequisite for achieving satisfactory rate‐capability. In this review, we analyze advantages and disadvantages of NASICON‐type electrode materials and highlight electrode structure design principles for obtaining the desired electrochemical performance. Moreover, we give an overview of recent approaches to enhance electrical conductivity and structural stability of cathode and anode materials based on NASICON structure. We believe that this review provides a pertinent insight into relevant design principles and inspires further research in this respect.
Sodium super ion conductor (NASICON)‐based electrode materials, exhibiting pronounced structural stability and exceptionally high ion conductivity are promising materials for sodium storage. Challenges and perspectives of NASICON‐type electrode materials are discussed, and electrode structure design principles for obtaining the desired electrochemical performance are highlighted. Recent progress in enhancing electrical conductivity and structural stability of NASICON materials is summarized. Sodium-ion batteries (SIBs) have attracted increasing attention in the past decades, because of high overall abundance of precursors, their even geographical distribution, and low cost. Apart from inherent thermodynamic disadvantages, SIBs have to overcome multiple kinetic problems, such as fast capacity decay, low rate capacities and low Coulombic efficiencies. A special case is sodium super ion conductor (NASICON)-based electrode materials as they exhibit - besides pronounced structural stability - exceptionally high ion conductivity, rendering them most promising for sodium storage. Owing to the limiting, comparatively low electronic conductivity, nano-structuring is a prerequisite for achieving satisfactory rate-capability. In this review, we analyze advantages and disadvantages of NASICON-type electrode materials and highlight electrode structure design principles for obtaining the desired electrochemical performance. Moreover, we give an overview of recent approaches to enhance electrical conductivity and structural stability of cathode and anode materials based on NASICON structure. We believe that this review provides a pertinent insight into relevant design principles and inspires further research in this respect. Sodium-ion batteries (SIBs) have attracted increasing attention in the past decades, because of high overall abundance of precursors, their even geographical distribution, and low cost. Apart from inherent thermodynamic disadvantages, SIBs have to overcome multiple kinetic problems, such as fast capacity decay, low rate capacities and low Coulombic efficiencies. A special case is sodium super ion conductor (NASICON)-based electrode materials as they exhibit - besides pronounced structural stability - exceptionally high ion conductivity, rendering them most promising for sodium storage. Owing to the limiting, comparatively low electronic conductivity, nano-structuring is a prerequisite for achieving satisfactory rate-capability. In this review, we analyze advantages and disadvantages of NASICON-type electrode materials and highlight electrode structure design principles for obtaining the desired electrochemical performance. Moreover, we give an overview of recent approaches to enhance electrical conductivity and structural stability of cathode and anode materials based on NASICON structure. We believe that this review provides a pertinent insight into relevant design principles and inspires further research in this respect.Sodium-ion batteries (SIBs) have attracted increasing attention in the past decades, because of high overall abundance of precursors, their even geographical distribution, and low cost. Apart from inherent thermodynamic disadvantages, SIBs have to overcome multiple kinetic problems, such as fast capacity decay, low rate capacities and low Coulombic efficiencies. A special case is sodium super ion conductor (NASICON)-based electrode materials as they exhibit - besides pronounced structural stability - exceptionally high ion conductivity, rendering them most promising for sodium storage. Owing to the limiting, comparatively low electronic conductivity, nano-structuring is a prerequisite for achieving satisfactory rate-capability. In this review, we analyze advantages and disadvantages of NASICON-type electrode materials and highlight electrode structure design principles for obtaining the desired electrochemical performance. Moreover, we give an overview of recent approaches to enhance electrical conductivity and structural stability of cathode and anode materials based on NASICON structure. We believe that this review provides a pertinent insight into relevant design principles and inspires further research in this respect. |
| Author | Wu, Chao Xi, Kai Maier, Joachim Huang, Yuanye Chen, Shuangqiang Shen, Laifa Yu, Yan Zhu, Changbao |
| Author_xml | – sequence: 1 givenname: Shuangqiang surname: Chen fullname: Chen, Shuangqiang organization: Max Planck Institute for Solid State Research – sequence: 2 givenname: Chao surname: Wu fullname: Wu, Chao organization: Max Planck Institute for Solid State Research – sequence: 3 givenname: Laifa surname: Shen fullname: Shen, Laifa organization: Max Planck Institute for Solid State Research – sequence: 4 givenname: Changbao surname: Zhu fullname: Zhu, Changbao organization: Max Planck Institute for Solid State Research – sequence: 5 givenname: Yuanye surname: Huang fullname: Huang, Yuanye organization: Max Planck Institute for Solid State Research – sequence: 6 givenname: Kai surname: Xi fullname: Xi, Kai organization: University of Cambridge – sequence: 7 givenname: Joachim surname: Maier fullname: Maier, Joachim organization: Max Planck Institute for Solid State Research – sequence: 8 givenname: Yan orcidid: 0000-0002-3685-7773 surname: Yu fullname: Yu, Yan email: yanyumse@ustc.edu.cn organization: Max Planck Institute for Solid State Research |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/28626908$$D View this record in MEDLINE/PubMed |
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| Keywords | NASICON-type materials electrode materials sodium-ion batteries |
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| Snippet | Sodium‐ion batteries (SIBs) have attracted increasing attention in the past decades, because of high overall abundance of precursors, their even geographical... Sodium-ion batteries (SIBs) have attracted increasing attention in the past decades, because of high overall abundance of precursors, their even geographical... |
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| SubjectTerms | Conductors Decay rate Electrical resistivity Electrochemical analysis Electrode materials Electrodes Geographical distribution Lithium Materials science NASICON‐type materials Rechargeable batteries Sodium Sodium-ion batteries Structural stability |
| Title | Challenges and Perspectives for NASICON‐Type Electrode Materials for Advanced Sodium‐Ion Batteries |
| URI | https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fadma.201700431 https://www.ncbi.nlm.nih.gov/pubmed/28626908 https://www.proquest.com/docview/1978281860 https://www.proquest.com/docview/1911202169 |
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