Integrated adsorption and photocatalytic degradation of volatile organic compounds (VOCs) using carbon-based nanocomposites: A critical review

Volatile organic compounds (VOCs) are harmful for human and surrounding ecosystem, and a great number of VOC abatement technologies have been developed during the past few decades. However, the single method has some problems such as high energy consumption, unfriendly environment, and low removal e...

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Published inChemosphere (Oxford) Vol. 218; pp. 845 - 859
Main Authors Zou, Weixin, Gao, Bin, Ok, Yong Sik, Dong, Lin
Format Journal Article
LanguageEnglish
Published England Elsevier Ltd 01.03.2019
Subjects
Adsorption
carbon
Carbon-based nanocomposite
ecosystems
electron transfer
energy
humans
Modeling
nanocomposites
photocatalysis
Photocatalytic degradation
surface area
VOC abatement
volatile organic compounds
VOC abatement
Photocatalytic degradation
Adsorption
Modeling
Carbon-based nanocomposite
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Abstract Volatile organic compounds (VOCs) are harmful for human and surrounding ecosystem, and a great number of VOC abatement technologies have been developed during the past few decades. However, the single method has some problems such as high energy consumption, unfriendly environment, and low removal efficiency. Recently, the integration of adsorption and photocatalytic degradation of VOCs is considered as a promising one. Carbon material, with large surface area, high adsorption capacity, and fast electron transfer ability, is widely used in integrated adsorptive-photocatalytic removal of VOCs. It is thus crucial to digest and summarize recent research advances in carbon-based nanocomposites as the adsorbent-photocatalyst for VOC removal. To satisfy this need, this work provides a critical review of the related literature with focuses on: (1) the advantages and disadvantages of various carbon-based nanocomposites for the applications of VOC adsorption and photocatalytic degradation; (2) models and mechanisms of adsorptive-photocatalytic removal of VOCs according to the material properties; and (3) major factors controlling adsorption-photocatalysis processes of VOCs. The review is aimed to establish the “structure-property-application” relationships for the development of innovative carbon-supported nanocomposites and to promote future research on the integrated adsorptive and photocatalytic removal of VOCs. •The advantages and disadvantages of carbon-supported hybrids were discussed.•Adsorption and photocatalytic models of VOC removal were reviewed.•The reaction processes and intermediates were proposed.•Major factors controlling adsorptive-photocatalytic reactions were discussed.
AbstractList Volatile organic compounds (VOCs) are harmful for human and surrounding ecosystem, and a great number of VOC abatement technologies have been developed during the past few decades. However, the single method has some problems such as high energy consumption, unfriendly environment, and low removal efficiency. Recently, the integration of adsorption and photocatalytic degradation of VOCs is considered as a promising one. Carbon material, with large surface area, high adsorption capacity, and fast electron transfer ability, is widely used in integrated adsorptive-photocatalytic removal of VOCs. It is thus crucial to digest and summarize recent research advances in carbon-based nanocomposites as the adsorbent-photocatalyst for VOC removal. To satisfy this need, this work provides a critical review of the related literature with focuses on: (1) the advantages and disadvantages of various carbon-based nanocomposites for the applications of VOC adsorption and photocatalytic degradation; (2) models and mechanisms of adsorptive-photocatalytic removal of VOCs according to the material properties; and (3) major factors controlling adsorption-photocatalysis processes of VOCs. The review is aimed to establish the "structure-property-application" relationships for the development of innovative carbon-supported nanocomposites and to promote future research on the integrated adsorptive and photocatalytic removal of VOCs.
Volatile organic compounds (VOCs) are harmful for human and surrounding ecosystem, and a great number of VOC abatement technologies have been developed during the past few decades. However, the single method has some problems such as high energy consumption, unfriendly environment, and low removal efficiency. Recently, the integration of adsorption and photocatalytic degradation of VOCs is considered as a promising one. Carbon material, with large surface area, high adsorption capacity, and fast electron transfer ability, is widely used in integrated adsorptive-photocatalytic removal of VOCs. It is thus crucial to digest and summarize recent research advances in carbon-based nanocomposites as the adsorbent-photocatalyst for VOC removal. To satisfy this need, this work provides a critical review of the related literature with focuses on: (1) the advantages and disadvantages of various carbon-based nanocomposites for the applications of VOC adsorption and photocatalytic degradation; (2) models and mechanisms of adsorptive-photocatalytic removal of VOCs according to the material properties; and (3) major factors controlling adsorption-photocatalysis processes of VOCs. The review is aimed to establish the “structure-property-application” relationships for the development of innovative carbon-supported nanocomposites and to promote future research on the integrated adsorptive and photocatalytic removal of VOCs. •The advantages and disadvantages of carbon-supported hybrids were discussed.•Adsorption and photocatalytic models of VOC removal were reviewed.•The reaction processes and intermediates were proposed.•Major factors controlling adsorptive-photocatalytic reactions were discussed.
Volatile organic compounds (VOCs) are harmful for human and surrounding ecosystem, and a great number of VOC abatement technologies have been developed during the past few decades. However, the single method has some problems such as high energy consumption, unfriendly environment, and low removal efficiency. Recently, the integration of adsorption and photocatalytic degradation of VOCs is considered as a promising one. Carbon material, with large surface area, high adsorption capacity, and fast electron transfer ability, is widely used in integrated adsorptive-photocatalytic removal of VOCs. It is thus crucial to digest and summarize recent research advances in carbon-based nanocomposites as the adsorbent-photocatalyst for VOC removal. To satisfy this need, this work provides a critical review of the related literature with focuses on: (1) the advantages and disadvantages of various carbon-based nanocomposites for the applications of VOC adsorption and photocatalytic degradation; (2) models and mechanisms of adsorptive-photocatalytic removal of VOCs according to the material properties; and (3) major factors controlling adsorption-photocatalysis processes of VOCs. The review is aimed to establish the "structure-property-application" relationships for the development of innovative carbon-supported nanocomposites and to promote future research on the integrated adsorptive and photocatalytic removal of VOCs.Volatile organic compounds (VOCs) are harmful for human and surrounding ecosystem, and a great number of VOC abatement technologies have been developed during the past few decades. However, the single method has some problems such as high energy consumption, unfriendly environment, and low removal efficiency. Recently, the integration of adsorption and photocatalytic degradation of VOCs is considered as a promising one. Carbon material, with large surface area, high adsorption capacity, and fast electron transfer ability, is widely used in integrated adsorptive-photocatalytic removal of VOCs. It is thus crucial to digest and summarize recent research advances in carbon-based nanocomposites as the adsorbent-photocatalyst for VOC removal. To satisfy this need, this work provides a critical review of the related literature with focuses on: (1) the advantages and disadvantages of various carbon-based nanocomposites for the applications of VOC adsorption and photocatalytic degradation; (2) models and mechanisms of adsorptive-photocatalytic removal of VOCs according to the material properties; and (3) major factors controlling adsorption-photocatalysis processes of VOCs. The review is aimed to establish the "structure-property-application" relationships for the development of innovative carbon-supported nanocomposites and to promote future research on the integrated adsorptive and photocatalytic removal of VOCs.
Author Zou, Weixin
Gao, Bin
Dong, Lin
Ok, Yong Sik
Author_xml – sequence: 1
  givenname: Weixin
  surname: Zou
  fullname: Zou, Weixin
  organization: School of the Environment, Nanjing University, Nanjing 210093, PR China
– sequence: 2
  givenname: Bin
  orcidid: 0000-0003-3769-0191
  surname: Gao
  fullname: Gao, Bin
  email: bg55@ufl.edu
  organization: Department of Agricultural and Biological Engineering, University of Florida, Gainesville, FL, 32611, USA
– sequence: 3
  givenname: Yong Sik
  orcidid: 0000-0003-3401-0912
  surname: Ok
  fullname: Ok, Yong Sik
  organization: Division of Environmental Science and Ecological Engineering, Korea University, Seoul 02841, Republic of Korea
– sequence: 4
  givenname: Lin
  orcidid: 0000-0001-8626-5509
  surname: Dong
  fullname: Dong, Lin
  email: donglin@nju.edu.cn
  organization: School of the Environment, Nanjing University, Nanjing 210093, PR China
BackLink https://www.ncbi.nlm.nih.gov/pubmed/30508803$$D View this record in MEDLINE/PubMed
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Snippet Volatile organic compounds (VOCs) are harmful for human and surrounding ecosystem, and a great number of VOC abatement technologies have been developed during...
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SubjectTerms Adsorption
carbon
Carbon-based nanocomposite
ecosystems
electron transfer
energy
humans
Modeling
nanocomposites
photocatalysis
Photocatalytic degradation
surface area
VOC abatement
volatile organic compounds
Title Integrated adsorption and photocatalytic degradation of volatile organic compounds (VOCs) using carbon-based nanocomposites: A critical review
URI https://dx.doi.org/10.1016/j.chemosphere.2018.11.175
https://www.ncbi.nlm.nih.gov/pubmed/30508803
https://www.proquest.com/docview/2149854607
https://www.proquest.com/docview/2220840098
Volume 218
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