Photodegradation of Rhodamine B over unexcited semiconductor compounds of BiOCl and BiOBr
[Display omitted] ► Photosensitized degradation of Rodamine B was investigated on BiOX (X=Cl, Br). ► Methylene Blue could not be degraded on BiOX under visible light irradiation. ► The relationship between LOMO of dye molecules and degradation rate was established. This study reported, for the first...
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| Published in | Journal of colloid and interface science Vol. 377; no. 1; pp. 291 - 298 |
|---|---|
| Main Authors | , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Amsterdam
Elsevier Inc
01.07.2012
Elsevier |
| Subjects | |
| Online Access | Get full text |
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| Abstract | [Display omitted]
► Photosensitized degradation of Rodamine B was investigated on BiOX (X=Cl, Br). ► Methylene Blue could not be degraded on BiOX under visible light irradiation. ► The relationship between LOMO of dye molecules and degradation rate was established.
This study reported, for the first time systematically, photodegradation of Rhodamine B (RhB) in aqueous solution over BiOCl and BiOBr semiconductors. Under visible light irradiation (λ>400nm, λ>420nm and λ=550±15nm), RhB adsorbed on the surface of BiOCl and BiOBr was photosensitized and decomposed effectively over unexcited BiOCl and BiOBr. The degradation of Methyl Orange (MO) and Methylene Blue (MB) over BiOCl and BiOBr was investigated as well, and the results were compared with RhB photodegradation. It was found that MB molecules having the lowest LUMO could not be degraded by this process. Utilizing the quantum chemical calculation (Gaussian 03 program), the relationship between frontier orbital energy of selected dye molecules and photodegradation rate was established for the first time in this study. |
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| AbstractList | This study reported, for the first time systematically, photodegradation of Rhodamine B (RhB) in aqueous solution over BiOCl and BiOBr semiconductors. Under visible light irradiation (λ>400nm, λ>420nm and λ=550±15nm), RhB adsorbed on the surface of BiOCl and BiOBr was photosensitized and decomposed effectively over unexcited BiOCl and BiOBr. The degradation of Methyl Orange (MO) and Methylene Blue (MB) over BiOCl and BiOBr was investigated as well, and the results were compared with RhB photodegradation. It was found that MB molecules having the lowest LUMO could not be degraded by this process. Utilizing the quantum chemical calculation (Gaussian 03 program), the relationship between frontier orbital energy of selected dye molecules and photodegradation rate was established for the first time in this study. This study reported, for the first time systematically, photodegradation of Rhodamine B (RhB) in aqueous solution over BiOCl and BiOBr semiconductors. Under visible light irradiation (λ>400 nm, λ>420 nm and λ=550±15 nm), RhB adsorbed on the surface of BiOCl and BiOBr was photosensitized and decomposed effectively over unexcited BiOCl and BiOBr. The degradation of Methyl Orange (MO) and Methylene Blue (MB) over BiOCl and BiOBr was investigated as well, and the results were compared with RhB photodegradation. It was found that MB molecules having the lowest LUMO could not be degraded by this process. Utilizing the quantum chemical calculation (Gaussian 03 program), the relationship between frontier orbital energy of selected dye molecules and photodegradation rate was established for the first time in this study.This study reported, for the first time systematically, photodegradation of Rhodamine B (RhB) in aqueous solution over BiOCl and BiOBr semiconductors. Under visible light irradiation (λ>400 nm, λ>420 nm and λ=550±15 nm), RhB adsorbed on the surface of BiOCl and BiOBr was photosensitized and decomposed effectively over unexcited BiOCl and BiOBr. The degradation of Methyl Orange (MO) and Methylene Blue (MB) over BiOCl and BiOBr was investigated as well, and the results were compared with RhB photodegradation. It was found that MB molecules having the lowest LUMO could not be degraded by this process. Utilizing the quantum chemical calculation (Gaussian 03 program), the relationship between frontier orbital energy of selected dye molecules and photodegradation rate was established for the first time in this study. This study reported, for the first time systematically, photodegradation of Rhodamine B (RhB) in aqueous solution over BiOCl and BiOBr semiconductors. Under visible light irradiation (λ>400 nm, λ>420 nm and λ=550±15 nm), RhB adsorbed on the surface of BiOCl and BiOBr was photosensitized and decomposed effectively over unexcited BiOCl and BiOBr. The degradation of Methyl Orange (MO) and Methylene Blue (MB) over BiOCl and BiOBr was investigated as well, and the results were compared with RhB photodegradation. It was found that MB molecules having the lowest LUMO could not be degraded by this process. Utilizing the quantum chemical calculation (Gaussian 03 program), the relationship between frontier orbital energy of selected dye molecules and photodegradation rate was established for the first time in this study. [Display omitted] ► Photosensitized degradation of Rodamine B was investigated on BiOX (X=Cl, Br). ► Methylene Blue could not be degraded on BiOX under visible light irradiation. ► The relationship between LOMO of dye molecules and degradation rate was established. This study reported, for the first time systematically, photodegradation of Rhodamine B (RhB) in aqueous solution over BiOCl and BiOBr semiconductors. Under visible light irradiation (λ>400nm, λ>420nm and λ=550±15nm), RhB adsorbed on the surface of BiOCl and BiOBr was photosensitized and decomposed effectively over unexcited BiOCl and BiOBr. The degradation of Methyl Orange (MO) and Methylene Blue (MB) over BiOCl and BiOBr was investigated as well, and the results were compared with RhB photodegradation. It was found that MB molecules having the lowest LUMO could not be degraded by this process. Utilizing the quantum chemical calculation (Gaussian 03 program), the relationship between frontier orbital energy of selected dye molecules and photodegradation rate was established for the first time in this study. This study reported, for the first time systematically, photodegradation of Rhodamine B (RhB) in aqueous solution over BiOCl and BiOBr semiconductors. Under visible light irradiation (I> > 400 nm, I> > 420 nm and I> = 550-15 nm), RhB adsorbed on the surface of BiOCl and BiOBr was photosensitized and decomposed effectively over unexcited BiOCl and BiOBr. The degradation of Methyl Orange (MO) and Methylene Blue (MB) over BiOCl and BiOBr was investigated as well, and the results were compared with RhB photodegradation. It was found that MB molecules having the lowest LUMO could not be degraded by this process. Utilizing the quantum chemical calculation (Gaussian 03 program), the relationship between frontier orbital energy of selected dye molecules and photodegradation rate was established for the first time in this study. |
| Author | Zhou, Qin Al-Saadi, A.A. Liu, Yousong Ali, M.A. Chang, Xiaofeng Shen, Hefei Ji, Guangbin Gondal, M.A. Zhang, Jun Du, Mengping |
| Author_xml | – sequence: 1 givenname: Xiaofeng surname: Chang fullname: Chang, Xiaofeng organization: Department of Applied Chemistry, College of Materials Science and Technology, Nanjing University of Aeronautics and Astronautics, Nanjing 211100, China – sequence: 2 givenname: M.A. surname: Gondal fullname: Gondal, M.A. organization: Laser Research Group, Physics Department, King Fahd University of Petroleum and Minerals, Dhahran 31261, Saudi Arabia – sequence: 3 givenname: A.A. surname: Al-Saadi fullname: Al-Saadi, A.A. organization: Department of Chemistry, King Fahd University of Petroleum and Minerals, Dhahran 31261, Saudi Arabia – sequence: 4 givenname: M.A. surname: Ali fullname: Ali, M.A. organization: Center for Refining and Petrochemicals, Research Institute, King Fahd University of Petroleum and Minerals, Dhahran 31261, Saudi Arabia – sequence: 5 givenname: Hefei surname: Shen fullname: Shen, Hefei organization: Department of Applied Chemistry, College of Materials Science and Technology, Nanjing University of Aeronautics and Astronautics, Nanjing 211100, China – sequence: 6 givenname: Qin surname: Zhou fullname: Zhou, Qin organization: State Key Laboratory of Environmental Aquatic Chemistry, Research Center for Eco-environmental Sciences, Chinese Academy of Sciences, Beijing 100085, China – sequence: 7 givenname: Jun surname: Zhang fullname: Zhang, Jun organization: Department of Applied Chemistry, College of Materials Science and Technology, Nanjing University of Aeronautics and Astronautics, Nanjing 211100, China – sequence: 8 givenname: Mengping surname: Du fullname: Du, Mengping organization: Department of Applied Chemistry, College of Materials Science and Technology, Nanjing University of Aeronautics and Astronautics, Nanjing 211100, China – sequence: 9 givenname: Yousong surname: Liu fullname: Liu, Yousong organization: Department of Applied Chemistry, College of Materials Science and Technology, Nanjing University of Aeronautics and Astronautics, Nanjing 211100, China – sequence: 10 givenname: Guangbin surname: Ji fullname: Ji, Guangbin email: gbji@nuaa.edu.cn organization: Department of Applied Chemistry, College of Materials Science and Technology, Nanjing University of Aeronautics and Astronautics, Nanjing 211100, China |
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| Keywords | Methylene Blue BiOBr BiOCl Photosensitized degradation Rhodamine B Methyl Orange Rhodamine Dyes Semiconductor materials Frontier orbital Methylene blue Energy Calculation Aqueous solution Photochemical degradation |
| Language | English |
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► Photosensitized degradation of Rodamine B was investigated on BiOX (X=Cl, Br). ► Methylene Blue could not be degraded on BiOX under visible... This study reported, for the first time systematically, photodegradation of Rhodamine B (RhB) in aqueous solution over BiOCl and BiOBr semiconductors. Under... |
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| SubjectTerms | aqueous solutions BiOBr BiOCl Bismuth - chemistry Chemistry Degradation Dyes energy Exact sciences and technology Gaussian General and physical chemistry irradiation Light Mathematical analysis Methyl Orange Methylene Blue Photochemical Processes Photochemistry Photodegradation photolysis Photosensitized degradation Physical chemistry of induced reactions (with radiations, particles and ultrasonics) Quantum chemistry Rhodamine Rhodamine B Rhodamines - chemistry Semiconductors |
| Title | Photodegradation of Rhodamine B over unexcited semiconductor compounds of BiOCl and BiOBr |
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