Effect of peroxydisulfate on the degradation of phenol under dielectric barrier discharge plasma treatment

The activation of peroxydisulfate (PDS) by gas/liquid dielectric barrier discharge (DBD) plasma in a flat plate configuration was assessed through phenol removal. The results indicated that PDS addition exhibited a significantly promoting effect on phenol removal and mineralization. In the reaction...

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Published inChemosphere (Oxford) Vol. 232; pp. 462 - 470
Main Authors Wang, Xiaojing, Zhang, Guangshan, Liu, Xiaomeng, Hu, Limin, Wang, Qiao, Wang, Peng
Format Journal Article
LanguageEnglish
Published England Elsevier Ltd 01.10.2019
Subjects
aqueous solutions
Dielectric barrier discharge plasma
electric potential difference
hydroxyl radicals
liquids
mineralization
Peroxydisulfate activation
phenol
Phenol degradation
Sulfate radical
total organic carbon
wastewater treatment
Peroxydisulfate activation
Sulfate radical
Phenol degradation
Dielectric barrier discharge plasma
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Abstract The activation of peroxydisulfate (PDS) by gas/liquid dielectric barrier discharge (DBD) plasma in a flat plate configuration was assessed through phenol removal. The results indicated that PDS addition exhibited a significantly promoting effect on phenol removal and mineralization. In the reaction lacking PDS, phenol in aqueous solution was removed from the initial 10 mg L−1 to 4.75 mg L−1 (by 52.5%), whereas the addition of 1770 mg L−1 PDS increased the overall removal to 78.7%, as indicated by a one-fold increase in the pseudo-first-order kinetic constant. In addition, the corresponding total organic carbon (TOC) removal was increased from 27.5% to 48.4%. Furthermore, an increased input voltage was favourable for increases in phenol removal, the kinetic constant and PDS utilization, which were also influenced by the PDS dose, initial solution pH and water matrix. In addition, through the analysis of radical quenching experiments, the enhancement could be mainly attributed to the production of SO4•- and •OH by PDS activation by discharge plasma. The DBD system coupled with PDS exhibited a high removal efficiency for phenol, and thus, the overall findings could provide new insight into wastewater treatment. [Display omitted] •Addition of PDS in discharge plasma can improve phenol degradation and TOC removal.•Enhanced phenol removal was attributed to increment of •OH and SO4•-.•Phenol removal was simultaneously attributed to •OH, SO4•- and other chemical and physical effects.•The activation of PDS by UV generated with discharge plasma likely occurred.
AbstractList The activation of peroxydisulfate (PDS) by gas/liquid dielectric barrier discharge (DBD) plasma in a flat plate configuration was assessed through phenol removal. The results indicated that PDS addition exhibited a significantly promoting effect on phenol removal and mineralization. In the reaction lacking PDS, phenol in aqueous solution was removed from the initial 10 mg L-1 to 4.75 mg L-1 (by 52.5%), whereas the addition of 1770 mg L-1 PDS increased the overall removal to 78.7%, as indicated by a one-fold increase in the pseudo-first-order kinetic constant. In addition, the corresponding total organic carbon (TOC) removal was increased from 27.5% to 48.4%. Furthermore, an increased input voltage was favourable for increases in phenol removal, the kinetic constant and PDS utilization, which were also influenced by the PDS dose, initial solution pH and water matrix. In addition, through the analysis of radical quenching experiments, the enhancement could be mainly attributed to the production of SO4•- and •OH by PDS activation by discharge plasma. The DBD system coupled with PDS exhibited a high removal efficiency for phenol, and thus, the overall findings could provide new insight into wastewater treatment.The activation of peroxydisulfate (PDS) by gas/liquid dielectric barrier discharge (DBD) plasma in a flat plate configuration was assessed through phenol removal. The results indicated that PDS addition exhibited a significantly promoting effect on phenol removal and mineralization. In the reaction lacking PDS, phenol in aqueous solution was removed from the initial 10 mg L-1 to 4.75 mg L-1 (by 52.5%), whereas the addition of 1770 mg L-1 PDS increased the overall removal to 78.7%, as indicated by a one-fold increase in the pseudo-first-order kinetic constant. In addition, the corresponding total organic carbon (TOC) removal was increased from 27.5% to 48.4%. Furthermore, an increased input voltage was favourable for increases in phenol removal, the kinetic constant and PDS utilization, which were also influenced by the PDS dose, initial solution pH and water matrix. In addition, through the analysis of radical quenching experiments, the enhancement could be mainly attributed to the production of SO4•- and •OH by PDS activation by discharge plasma. The DBD system coupled with PDS exhibited a high removal efficiency for phenol, and thus, the overall findings could provide new insight into wastewater treatment.
The activation of peroxydisulfate (PDS) by gas/liquid dielectric barrier discharge (DBD) plasma in a flat plate configuration was assessed through phenol removal. The results indicated that PDS addition exhibited a significantly promoting effect on phenol removal and mineralization. In the reaction lacking PDS, phenol in aqueous solution was removed from the initial 10 mg L⁻¹ to 4.75 mg L⁻¹ (by 52.5%), whereas the addition of 1770 mg L⁻¹ PDS increased the overall removal to 78.7%, as indicated by a one-fold increase in the pseudo-first-order kinetic constant. In addition, the corresponding total organic carbon (TOC) removal was increased from 27.5% to 48.4%. Furthermore, an increased input voltage was favourable for increases in phenol removal, the kinetic constant and PDS utilization, which were also influenced by the PDS dose, initial solution pH and water matrix. In addition, through the analysis of radical quenching experiments, the enhancement could be mainly attributed to the production of SO₄•⁻ and •OH by PDS activation by discharge plasma. The DBD system coupled with PDS exhibited a high removal efficiency for phenol, and thus, the overall findings could provide new insight into wastewater treatment.
The activation of peroxydisulfate (PDS) by gas/liquid dielectric barrier discharge (DBD) plasma in a flat plate configuration was assessed through phenol removal. The results indicated that PDS addition exhibited a significantly promoting effect on phenol removal and mineralization. In the reaction lacking PDS, phenol in aqueous solution was removed from the initial 10 mg L to 4.75 mg L (by 52.5%), whereas the addition of 1770 mg L PDS increased the overall removal to 78.7%, as indicated by a one-fold increase in the pseudo-first-order kinetic constant. In addition, the corresponding total organic carbon (TOC) removal was increased from 27.5% to 48.4%. Furthermore, an increased input voltage was favourable for increases in phenol removal, the kinetic constant and PDS utilization, which were also influenced by the PDS dose, initial solution pH and water matrix. In addition, through the analysis of radical quenching experiments, the enhancement could be mainly attributed to the production of SO and •OH by PDS activation by discharge plasma. The DBD system coupled with PDS exhibited a high removal efficiency for phenol, and thus, the overall findings could provide new insight into wastewater treatment.
The activation of peroxydisulfate (PDS) by gas/liquid dielectric barrier discharge (DBD) plasma in a flat plate configuration was assessed through phenol removal. The results indicated that PDS addition exhibited a significantly promoting effect on phenol removal and mineralization. In the reaction lacking PDS, phenol in aqueous solution was removed from the initial 10 mg L−1 to 4.75 mg L−1 (by 52.5%), whereas the addition of 1770 mg L−1 PDS increased the overall removal to 78.7%, as indicated by a one-fold increase in the pseudo-first-order kinetic constant. In addition, the corresponding total organic carbon (TOC) removal was increased from 27.5% to 48.4%. Furthermore, an increased input voltage was favourable for increases in phenol removal, the kinetic constant and PDS utilization, which were also influenced by the PDS dose, initial solution pH and water matrix. In addition, through the analysis of radical quenching experiments, the enhancement could be mainly attributed to the production of SO4•- and •OH by PDS activation by discharge plasma. The DBD system coupled with PDS exhibited a high removal efficiency for phenol, and thus, the overall findings could provide new insight into wastewater treatment. [Display omitted] •Addition of PDS in discharge plasma can improve phenol degradation and TOC removal.•Enhanced phenol removal was attributed to increment of •OH and SO4•-.•Phenol removal was simultaneously attributed to •OH, SO4•- and other chemical and physical effects.•The activation of PDS by UV generated with discharge plasma likely occurred.
Author Zhang, Guangshan
Wang, Qiao
Wang, Peng
Hu, Limin
Wang, Xiaojing
Liu, Xiaomeng
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BackLink https://www.ncbi.nlm.nih.gov/pubmed/31158641$$D View this record in MEDLINE/PubMed
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Keywords Peroxydisulfate activation
Sulfate radical
Phenol degradation
Dielectric barrier discharge plasma
Language English
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Snippet The activation of peroxydisulfate (PDS) by gas/liquid dielectric barrier discharge (DBD) plasma in a flat plate configuration was assessed through phenol...
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SubjectTerms aqueous solutions
Dielectric barrier discharge plasma
electric potential difference
hydroxyl radicals
liquids
mineralization
Peroxydisulfate activation
phenol
Phenol degradation
Sulfate radical
total organic carbon
wastewater treatment
Title Effect of peroxydisulfate on the degradation of phenol under dielectric barrier discharge plasma treatment
URI https://dx.doi.org/10.1016/j.chemosphere.2019.05.214
https://www.ncbi.nlm.nih.gov/pubmed/31158641
https://www.proquest.com/docview/2235069023
https://www.proquest.com/docview/2271866487
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