An abundant porous biochar material derived from wakame (Undaria pinnatifida) with high adsorption performance for three organic dyes
[Display omitted] •A one-step pyrolysis/activation method was used to prepare wakame biochar (AWBM).•AWBM has abundant mesopores with a high specific surface area (1156.25 m2/g).•At 293 K, the adsorption of MG using AWBM can reach 4066.96 mg/g.•The adsorption of dyes using AWBM contain physical and...
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| Published in | Bioresource technology Vol. 318; no. C; p. 124082 |
|---|---|
| Main Authors | , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
England
Elsevier Ltd
01.12.2020
Elsevier |
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| Online Access | Get full text |
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| Abstract | [Display omitted]
•A one-step pyrolysis/activation method was used to prepare wakame biochar (AWBM).•AWBM has abundant mesopores with a high specific surface area (1156.25 m2/g).•At 293 K, the adsorption of MG using AWBM can reach 4066.96 mg/g.•The adsorption of dyes using AWBM contain physical and chemical adsorption.
In this study, an activated wakame biochar material (AWBM) was prepared by a one-step calcination and activation method, whose adsorption performances for methylene blue (MB), Rhodamine B (RB) and malachite green (MG) were also analyzed. The results showed AWBM was a mesoporous fluffy structure material with a higher specific surface (1156.25 m2/g), exhibiting superior adsorption capacities for MB (841.64 mg/g), RB (533.77 mg/g) and MG (4066.96 mg/g), respectively. In addition, FT-IR analysis showed that AWBM possessed abundant active groups (such as –OH, –CO and –CH), further enhancing the adsorption efficiencies. The Langmuir model could better fit the three dyes adsorption isotherms process using AWBM, and the Pseudo-second-order model could better describe the adsorption kinetic experimental data. The thermodynamic analysis showed that the three dyes adsorption using AWBM was spontaneous endothermic reaction. This study suggests AWBM has enormous potential in the application of removing organic dyes from wastewater. |
|---|---|
| AbstractList | In this study, an activated wakame biochar material (AWBM) was prepared by a one-step calcination and activation method, whose adsorption performances for methylene blue (MB), Rhodamine B (RB) and malachite green (MG) were also analyzed. The results showed AWBM was a mesoporous fluffy structure material with a higher specific surface (1156.25 m2/g), exhibiting superior adsorption capacities for MB (841.64 mg/g), RB (533.77 mg/g) and MG (4066.96 mg/g), respectively. In addition, FT-IR analysis showed that AWBM possessed abundant active groups (such as -OH, -CO and -CH), further enhancing the adsorption efficiencies. The Langmuir model could better fit the three dyes adsorption isotherms process using AWBM, and the Pseudo-second-order model could better describe the adsorption kinetic experimental data. The thermodynamic analysis showed that the three dyes adsorption using AWBM was spontaneous endothermic reaction. This study suggests AWBM has enormous potential in the application of removing organic dyes from wastewater.In this study, an activated wakame biochar material (AWBM) was prepared by a one-step calcination and activation method, whose adsorption performances for methylene blue (MB), Rhodamine B (RB) and malachite green (MG) were also analyzed. The results showed AWBM was a mesoporous fluffy structure material with a higher specific surface (1156.25 m2/g), exhibiting superior adsorption capacities for MB (841.64 mg/g), RB (533.77 mg/g) and MG (4066.96 mg/g), respectively. In addition, FT-IR analysis showed that AWBM possessed abundant active groups (such as -OH, -CO and -CH), further enhancing the adsorption efficiencies. The Langmuir model could better fit the three dyes adsorption isotherms process using AWBM, and the Pseudo-second-order model could better describe the adsorption kinetic experimental data. The thermodynamic analysis showed that the three dyes adsorption using AWBM was spontaneous endothermic reaction. This study suggests AWBM has enormous potential in the application of removing organic dyes from wastewater. In this study, an activated wakame biochar material (AWBM) was prepared by a one-step calcination and activation method, whose adsorption performances for methylene blue (MB), Rhodamine B (RB) and malachite green (MG) were also analyzed. The results showed AWBM was a mesoporous fluffy structure material with a higher specific surface (1156.25 m /g), exhibiting superior adsorption capacities for MB (841.64 mg/g), RB (533.77 mg/g) and MG (4066.96 mg/g), respectively. In addition, FT-IR analysis showed that AWBM possessed abundant active groups (such as -OH, -CO and -CH), further enhancing the adsorption efficiencies. The Langmuir model could better fit the three dyes adsorption isotherms process using AWBM, and the Pseudo-second-order model could better describe the adsorption kinetic experimental data. The thermodynamic analysis showed that the three dyes adsorption using AWBM was spontaneous endothermic reaction. This study suggests AWBM has enormous potential in the application of removing organic dyes from wastewater. [Display omitted] •A one-step pyrolysis/activation method was used to prepare wakame biochar (AWBM).•AWBM has abundant mesopores with a high specific surface area (1156.25 m2/g).•At 293 K, the adsorption of MG using AWBM can reach 4066.96 mg/g.•The adsorption of dyes using AWBM contain physical and chemical adsorption. In this study, an activated wakame biochar material (AWBM) was prepared by a one-step calcination and activation method, whose adsorption performances for methylene blue (MB), Rhodamine B (RB) and malachite green (MG) were also analyzed. The results showed AWBM was a mesoporous fluffy structure material with a higher specific surface (1156.25 m2/g), exhibiting superior adsorption capacities for MB (841.64 mg/g), RB (533.77 mg/g) and MG (4066.96 mg/g), respectively. In addition, FT-IR analysis showed that AWBM possessed abundant active groups (such as –OH, –CO and –CH), further enhancing the adsorption efficiencies. The Langmuir model could better fit the three dyes adsorption isotherms process using AWBM, and the Pseudo-second-order model could better describe the adsorption kinetic experimental data. The thermodynamic analysis showed that the three dyes adsorption using AWBM was spontaneous endothermic reaction. This study suggests AWBM has enormous potential in the application of removing organic dyes from wastewater. In this study, an activated wakame biochar material (AWBM) was prepared by a one-step calcination and activation method, whose adsorption performances for methylene blue (MB), Rhodamine B (RB) and malachite green (MG) were also analyzed. The results showed AWBM was a mesoporous fluffy structure material with a higher specific surface (1156.25 m²/g), exhibiting superior adsorption capacities for MB (841.64 mg/g), RB (533.77 mg/g) and MG (4066.96 mg/g), respectively. In addition, FT-IR analysis showed that AWBM possessed abundant active groups (such as –OH, –CO and –CH), further enhancing the adsorption efficiencies. The Langmuir model could better fit the three dyes adsorption isotherms process using AWBM, and the Pseudo-second-order model could better describe the adsorption kinetic experimental data. The thermodynamic analysis showed that the three dyes adsorption using AWBM was spontaneous endothermic reaction. This study suggests AWBM has enormous potential in the application of removing organic dyes from wastewater. |
| ArticleNumber | 124082 |
| Author | Wang, Yaning Guo, Jian Lu, Wencheng Chen, Yingna Ge, Shaoliang Yao, Xinxin Cai, Lu Song, Wendong Ji, Lili |
| Author_xml | – sequence: 1 givenname: Xinxin surname: Yao fullname: Yao, Xinxin organization: College of Naval Architecture and Mechanical-Electrical Engineering, Zhejiang Ocean University, Zhoushan, Zhejiang 316022, China – sequence: 2 givenname: Lili surname: Ji fullname: Ji, Lili email: jll-gb@163.com organization: Institute of Innovation & Application, Zhejiang Ocean University, Zhoushan, Zhejiang 316022, China – sequence: 3 givenname: Jian surname: Guo fullname: Guo, Jian organization: College of Food and Medical, Zhejiang Ocean University, Zhoushan, Zhejiang 316022, China – sequence: 4 givenname: Shaoliang surname: Ge fullname: Ge, Shaoliang organization: College of Port and Transportation Engineering, Zhejiang Ocean University, Zhoushan, Zhejiang 316022, China – sequence: 5 givenname: Wencheng surname: Lu fullname: Lu, Wencheng organization: College of Naval Architecture and Mechanical-Electrical Engineering, Zhejiang Ocean University, Zhoushan, Zhejiang 316022, China – sequence: 6 givenname: Yingna surname: Chen fullname: Chen, Yingna organization: College of Food and Medical, Zhejiang Ocean University, Zhoushan, Zhejiang 316022, China – sequence: 7 givenname: Lu surname: Cai fullname: Cai, Lu organization: Donghai Science and Technology College, Zhejiang Ocean University, Zhoushan 316000, China – sequence: 8 givenname: Yaning surname: Wang fullname: Wang, Yaning organization: Institute of Innovation & Application, Zhejiang Ocean University, Zhoushan, Zhejiang 316022, China – sequence: 9 givenname: Wendong surname: Song fullname: Song, Wendong organization: College of Petrochemical and Energy Engineering College, Zhejiang Ocean University, Zhoushan, Zhejiang 316022, China |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/32932115$$D View this record in MEDLINE/PubMed https://www.osti.gov/biblio/2279898$$D View this record in Osti.gov |
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| Keywords | Abundant porous structure Organic dyes Adsorption mechanism Wakame biochar |
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•A one-step pyrolysis/activation method was used to prepare wakame biochar (AWBM).•AWBM has abundant mesopores with a high specific surface... In this study, an activated wakame biochar material (AWBM) was prepared by a one-step calcination and activation method, whose adsorption performances for... |
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| SubjectTerms | Abundant porous structure activated carbon Adsorption Adsorption mechanism biochar Charcoal Coloring Agents endothermy heat treatment Kinetics malachite green Methylene Blue Organic dyes Porosity porous media rhodamines sorption isotherms Spectroscopy, Fourier Transform Infrared thermodynamics Undaria Undaria pinnatifida Wakame biochar wastewater treatment Water Pollutants, Chemical |
| Title | An abundant porous biochar material derived from wakame (Undaria pinnatifida) with high adsorption performance for three organic dyes |
| URI | https://dx.doi.org/10.1016/j.biortech.2020.124082 https://www.ncbi.nlm.nih.gov/pubmed/32932115 https://www.proquest.com/docview/2443521717 https://www.proquest.com/docview/2552020899 https://www.osti.gov/biblio/2279898 |
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