Lithiophilic Sites in Doped Graphene Guide Uniform Lithium Nucleation for Dendrite‐Free Lithium Metal Anodes
Lithium (Li) metal is the most promising electrode for next‐generation rechargeable batteries. However, the challenges induced by Li dendrites on a working Li metal anode hinder the practical applications of Li metal batteries. Herein, nitrogen (N) doped graphene was adopted as the Li plating matrix...
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| Published in | Angewandte Chemie International Edition Vol. 56; no. 27; pp. 7764 - 7768 |
|---|---|
| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Germany
Wiley Subscription Services, Inc
26.06.2017
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| Edition | International ed. in English |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Lithium (Li) metal is the most promising electrode for next‐generation rechargeable batteries. However, the challenges induced by Li dendrites on a working Li metal anode hinder the practical applications of Li metal batteries. Herein, nitrogen (N) doped graphene was adopted as the Li plating matrix to regulate Li metal nucleation and suppress dendrite growth. The N‐containing functional groups, such as pyridinic and pyrrolic nitrogen in the N‐doped graphene, are lithiophilic, which guide the metallic Li nucleation causing the metal to distribute uniformly on the anode surface. As a result, the N‐doped graphene modified Li metal anode exhibits a dendrite‐free morphology during repeated Li plating and demonstrates a high Coulombic efficiency of 98 % for near 200 cycles.
The matrix: Nitrogen‐doped graphene is used as the Li plating matrix to regulate Li metal nucleation and suppress dendrite growth. The N‐containing functional groups in the N‐doped graphene are lithiophilic, which guide the Li nucleation and give a uniform distribution of Li on the anode surface. The dendrite‐free lithium‐metal anodes exhibit an impressive electrochemical performance. |
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| AbstractList | Lithium (Li) metal is the most promising electrode for next‐generation rechargeable batteries. However, the challenges induced by Li dendrites on a working Li metal anode hinder the practical applications of Li metal batteries. Herein, nitrogen (N) doped graphene was adopted as the Li plating matrix to regulate Li metal nucleation and suppress dendrite growth. The N‐containing functional groups, such as pyridinic and pyrrolic nitrogen in the N‐doped graphene, are lithiophilic, which guide the metallic Li nucleation causing the metal to distribute uniformly on the anode surface. As a result, the N‐doped graphene modified Li metal anode exhibits a dendrite‐free morphology during repeated Li plating and demonstrates a high Coulombic efficiency of 98 % for near 200 cycles. Lithium (Li) metal is the most promising electrode for next-generation rechargeable batteries. However, the challenges induced by Li dendrites on a working Li metal anode hinder the practical applications of Li metal batteries. Herein, nitrogen (N) doped graphene was adopted as the Li plating matrix to regulate Li metal nucleation and suppress dendrite growth. The N-containing functional groups, such as pyridinic and pyrrolic nitrogen in the N-doped graphene, are lithiophilic, which guide the metallic Li nucleation causing the metal to distribute uniformly on the anode surface. As a result, the N-doped graphene modified Li metal anode exhibits a dendrite-free morphology during repeated Li plating and demonstrates a high Coulombic efficiency of 98% for near 200cycles. Lithium (Li) metal is the most promising electrode for next‐generation rechargeable batteries. However, the challenges induced by Li dendrites on a working Li metal anode hinder the practical applications of Li metal batteries. Herein, nitrogen (N) doped graphene was adopted as the Li plating matrix to regulate Li metal nucleation and suppress dendrite growth. The N‐containing functional groups, such as pyridinic and pyrrolic nitrogen in the N‐doped graphene, are lithiophilic, which guide the metallic Li nucleation causing the metal to distribute uniformly on the anode surface. As a result, the N‐doped graphene modified Li metal anode exhibits a dendrite‐free morphology during repeated Li plating and demonstrates a high Coulombic efficiency of 98 % for near 200 cycles. The matrix: Nitrogen‐doped graphene is used as the Li plating matrix to regulate Li metal nucleation and suppress dendrite growth. The N‐containing functional groups in the N‐doped graphene are lithiophilic, which guide the Li nucleation and give a uniform distribution of Li on the anode surface. The dendrite‐free lithium‐metal anodes exhibit an impressive electrochemical performance. Lithium (Li) metal is the most promising electrode for next-generation rechargeable batteries. However, the challenges induced by Li dendrites on a working Li metal anode hinder the practical applications of Li metal batteries. Herein, nitrogen (N) doped graphene was adopted as the Li plating matrix to regulate Li metal nucleation and suppress dendrite growth. The N-containing functional groups, such as pyridinic and pyrrolic nitrogen in the N-doped graphene, are lithiophilic, which guide the metallic Li nucleation causing the metal to distribute uniformly on the anode surface. As a result, the N-doped graphene modified Li metal anode exhibits a dendrite-free morphology during repeated Li plating and demonstrates a high Coulombic efficiency of 98 % for near 200 cycles.Lithium (Li) metal is the most promising electrode for next-generation rechargeable batteries. However, the challenges induced by Li dendrites on a working Li metal anode hinder the practical applications of Li metal batteries. Herein, nitrogen (N) doped graphene was adopted as the Li plating matrix to regulate Li metal nucleation and suppress dendrite growth. The N-containing functional groups, such as pyridinic and pyrrolic nitrogen in the N-doped graphene, are lithiophilic, which guide the metallic Li nucleation causing the metal to distribute uniformly on the anode surface. As a result, the N-doped graphene modified Li metal anode exhibits a dendrite-free morphology during repeated Li plating and demonstrates a high Coulombic efficiency of 98 % for near 200 cycles. |
| Author | Zhang, Qiang Chen, Xiao‐Ru Cheng, Xin‐Bing Zhang, Rui Zhang, Xue‐Qiang Chen, Xiang Yan, Chong |
| Author_xml | – sequence: 1 givenname: Rui orcidid: 0000-0003-3740-8352 surname: Zhang fullname: Zhang, Rui organization: Tsinghua University – sequence: 2 givenname: Xiao‐Ru surname: Chen fullname: Chen, Xiao‐Ru organization: Tsinghua University – sequence: 3 givenname: Xiang orcidid: 0000-0002-7686-6308 surname: Chen fullname: Chen, Xiang organization: Tsinghua University – sequence: 4 givenname: Xin‐Bing orcidid: 0000-0001-7567-1210 surname: Cheng fullname: Cheng, Xin‐Bing organization: Tsinghua University – sequence: 5 givenname: Xue‐Qiang surname: Zhang fullname: Zhang, Xue‐Qiang organization: Tsinghua University – sequence: 6 givenname: Chong surname: Yan fullname: Yan, Chong organization: Tsinghua University – sequence: 7 givenname: Qiang orcidid: 0000-0002-3929-1541 surname: Zhang fullname: Zhang, Qiang email: zhang-qiang@mails.tsinghua.edu.cn organization: Tsinghua University |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/28466583$$D View this record in MEDLINE/PubMed |
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| Copyright | 2017 Wiley‐VCH Verlag GmbH & Co. KGaA, Weinheim 2017 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim. 2017 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim |
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| DOI | 10.1002/anie.201702099 |
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| Snippet | Lithium (Li) metal is the most promising electrode for next‐generation rechargeable batteries. However, the challenges induced by Li dendrites on a working Li... Lithium (Li) metal is the most promising electrode for next-generation rechargeable batteries. However, the challenges induced by Li dendrites on a working Li... |
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| SubjectTerms | Batteries Dendrites Functional groups Graphene Lithium lithium dendrites lithium metal anode Metals Nitrogen nitrogen-doped graphene Nucleation nucleation and growth Rechargeable batteries |
| Title | Lithiophilic Sites in Doped Graphene Guide Uniform Lithium Nucleation for Dendrite‐Free Lithium Metal Anodes |
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