Transition‐Metal‐Based Electrocatalysts as Cocatalysts for Photoelectrochemical Water Splitting: A Mini Review
Converting solar energy into hydrogen via photoelectrochemical (PEC) water splitting is one of the most promising approaches for a sustainable energy supply. Highly active, cost‐effective, and robust photoelectrodes are undoubtedly crucial for the PEC technology. To achieve this goal, transition‐met...
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| Published in | Small (Weinheim an der Bergstrasse, Germany) Vol. 14; no. 23; pp. e1704179 - n/a |
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| Main Authors | , , |
| Format | Journal Article |
| Language | English |
| Published |
Germany
Wiley Subscription Services, Inc
01.06.2018
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Converting solar energy into hydrogen via photoelectrochemical (PEC) water splitting is one of the most promising approaches for a sustainable energy supply. Highly active, cost‐effective, and robust photoelectrodes are undoubtedly crucial for the PEC technology. To achieve this goal, transition‐metal‐based electrocatalysts have been widely used as cocatalysts to improve the performance of PEC cells for water splitting. Herein, this Review summarizes the recent progresses of the design, synthesis, and application of transition‐metal‐based electrocatalysts as cocatalysts for PEC water splitting. Mo, Ni, Co‐based electrocatalysts for the hydrogen evolution reaction (HER) and Co, Ni, Fe‐based electrocatalysts for the oxygen evolution reaction (OER) are emphasized as cocatalysts for efficient PEC HER and OER, respectively. Particularly, some most efficient and robust photoelectrode systems with record photocurrent density or durability for the half reactions of HER and OER are highlighted and discussed. In addition, the self‐biased PEC devices with high solar‐to‐hydrogen efficiency based on earth‐abundant materials are also addressed. Finally, this Review is concluded with a summary and remarks on some challenges and opportunities for the further development of transition‐metal‐based electrocatalysts as cocatalysts for PEC water splitting.
Photoelectrochemical water splitting for hydrogen production is regarded as a promising way to harvest and store the intermittent solar energy. Highly efficient photoelectrodes require integrating of electrocatalysts onto the light absorbers. In this Review, the recent applications of transition‐metal‐based hydrogen evolution reaction and oxygen evolution reaction electrocatalysts as cocatalyst to be incorporated into photoelectrochemical systems for solar water splitting are summarized. |
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| AbstractList | Converting solar energy into hydrogen via photoelectrochemical (PEC) water splitting is one of the most promising approaches for a sustainable energy supply. Highly active, cost‐effective, and robust photoelectrodes are undoubtedly crucial for the PEC technology. To achieve this goal, transition‐metal‐based electrocatalysts have been widely used as cocatalysts to improve the performance of PEC cells for water splitting. Herein, this Review summarizes the recent progresses of the design, synthesis, and application of transition‐metal‐based electrocatalysts as cocatalysts for PEC water splitting. Mo, Ni, Co‐based electrocatalysts for the hydrogen evolution reaction (HER) and Co, Ni, Fe‐based electrocatalysts for the oxygen evolution reaction (OER) are emphasized as cocatalysts for efficient PEC HER and OER, respectively. Particularly, some most efficient and robust photoelectrode systems with record photocurrent density or durability for the half reactions of HER and OER are highlighted and discussed. In addition, the self‐biased PEC devices with high solar‐to‐hydrogen efficiency based on earth‐abundant materials are also addressed. Finally, this Review is concluded with a summary and remarks on some challenges and opportunities for the further development of transition‐metal‐based electrocatalysts as cocatalysts for PEC water splitting. Converting solar energy into hydrogen via photoelectrochemical (PEC) water splitting is one of the most promising approaches for a sustainable energy supply. Highly active, cost-effective, and robust photoelectrodes are undoubtedly crucial for the PEC technology. To achieve this goal, transition-metal-based electrocatalysts have been widely used as cocatalysts to improve the performance of PEC cells for water splitting. Herein, this Review summarizes the recent progresses of the design, synthesis, and application of transition-metal-based electrocatalysts as cocatalysts for PEC water splitting. Mo, Ni, Co-based electrocatalysts for the hydrogen evolution reaction (HER) and Co, Ni, Fe-based electrocatalysts for the oxygen evolution reaction (OER) are emphasized as cocatalysts for efficient PEC HER and OER, respectively. Particularly, some most efficient and robust photoelectrode systems with record photocurrent density or durability for the half reactions of HER and OER are highlighted and discussed. In addition, the self-biased PEC devices with high solar-to-hydrogen efficiency based on earth-abundant materials are also addressed. Finally, this Review is concluded with a summary and remarks on some challenges and opportunities for the further development of transition-metal-based electrocatalysts as cocatalysts for PEC water splitting.Converting solar energy into hydrogen via photoelectrochemical (PEC) water splitting is one of the most promising approaches for a sustainable energy supply. Highly active, cost-effective, and robust photoelectrodes are undoubtedly crucial for the PEC technology. To achieve this goal, transition-metal-based electrocatalysts have been widely used as cocatalysts to improve the performance of PEC cells for water splitting. Herein, this Review summarizes the recent progresses of the design, synthesis, and application of transition-metal-based electrocatalysts as cocatalysts for PEC water splitting. Mo, Ni, Co-based electrocatalysts for the hydrogen evolution reaction (HER) and Co, Ni, Fe-based electrocatalysts for the oxygen evolution reaction (OER) are emphasized as cocatalysts for efficient PEC HER and OER, respectively. Particularly, some most efficient and robust photoelectrode systems with record photocurrent density or durability for the half reactions of HER and OER are highlighted and discussed. In addition, the self-biased PEC devices with high solar-to-hydrogen efficiency based on earth-abundant materials are also addressed. Finally, this Review is concluded with a summary and remarks on some challenges and opportunities for the further development of transition-metal-based electrocatalysts as cocatalysts for PEC water splitting. Converting solar energy into hydrogen via photoelectrochemical (PEC) water splitting is one of the most promising approaches for a sustainable energy supply. Highly active, cost‐effective, and robust photoelectrodes are undoubtedly crucial for the PEC technology. To achieve this goal, transition‐metal‐based electrocatalysts have been widely used as cocatalysts to improve the performance of PEC cells for water splitting. Herein, this Review summarizes the recent progresses of the design, synthesis, and application of transition‐metal‐based electrocatalysts as cocatalysts for PEC water splitting. Mo, Ni, Co‐based electrocatalysts for the hydrogen evolution reaction (HER) and Co, Ni, Fe‐based electrocatalysts for the oxygen evolution reaction (OER) are emphasized as cocatalysts for efficient PEC HER and OER, respectively. Particularly, some most efficient and robust photoelectrode systems with record photocurrent density or durability for the half reactions of HER and OER are highlighted and discussed. In addition, the self‐biased PEC devices with high solar‐to‐hydrogen efficiency based on earth‐abundant materials are also addressed. Finally, this Review is concluded with a summary and remarks on some challenges and opportunities for the further development of transition‐metal‐based electrocatalysts as cocatalysts for PEC water splitting. Photoelectrochemical water splitting for hydrogen production is regarded as a promising way to harvest and store the intermittent solar energy. Highly efficient photoelectrodes require integrating of electrocatalysts onto the light absorbers. In this Review, the recent applications of transition‐metal‐based hydrogen evolution reaction and oxygen evolution reaction electrocatalysts as cocatalyst to be incorporated into photoelectrochemical systems for solar water splitting are summarized. |
| Author | Li, Can Shi, Jingying Li, Deng |
| Author_xml | – sequence: 1 givenname: Deng surname: Li fullname: Li, Deng organization: University of Chinese Academy of Sciences – sequence: 2 givenname: Jingying orcidid: 0000-0002-8493-8172 surname: Shi fullname: Shi, Jingying email: jingyingshi@dicp.ac.cn organization: Dalian National Laboratory for Clean Energy – sequence: 3 givenname: Can surname: Li fullname: Li, Can organization: Dalian National Laboratory for Clean Energy |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/29575653$$D View this record in MEDLINE/PubMed |
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| Copyright | 2018 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim 2018 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim. |
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| Keywords | transition-metal-based electrocatalysts oxygen evolution reaction photoelectrochemistry water splitting hydrogen evolution reaction |
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| Snippet | Converting solar energy into hydrogen via photoelectrochemical (PEC) water splitting is one of the most promising approaches for a sustainable energy supply.... |
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| SubjectTerms | Electrocatalysts hydrogen evolution reaction Hydrogen evolution reactions Hydrogen-based energy Molybdenum Nanotechnology Nickel oxygen evolution reaction Oxygen evolution reactions Performance enhancement Photoelectric effect Photoelectric emission photoelectrochemistry Solar energy conversion transition‐metal‐based electrocatalysts Water splitting |
| Title | Transition‐Metal‐Based Electrocatalysts as Cocatalysts for Photoelectrochemical Water Splitting: A Mini Review |
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