Atomically Dispersed Metal Sites in MOF‐Based Materials for Electrocatalytic and Photocatalytic Energy Conversion

Metal sites play an essential role in both electrocatalytic and photocatalytic energy conversion. The highly ordered arrangements of the organic linkers and metal nodes as well as the well‐defined pore structures of metal‐organic frameworks (MOFs) make them ideal substrates to support atomically dis...

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Published inAngewandte Chemie International Edition Vol. 57; no. 31; pp. 9604 - 9633
Main Authors Liang, Zibin, Qu, Chong, Xia, Dingguo, Zou, Ruqiang, Xu, Qiang
Format Journal Article
LanguageEnglish
Published Germany Wiley Subscription Services, Inc 26.07.2018
EditionInternational ed. in English
Subjects
Carbon
Catalysis
Catalysts
Dispersion
Energy
Energy conversion
heterogeneous catalysis
metal centers
Metal-organic frameworks
Metals
Molecular chains
Porous materials
single-atom catalysts
Substrates
single-atom catalysts
energy conversion
heterogeneous catalysis
metal centers
metal-organic frameworks
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Abstract Metal sites play an essential role in both electrocatalytic and photocatalytic energy conversion. The highly ordered arrangements of the organic linkers and metal nodes as well as the well‐defined pore structures of metal‐organic frameworks (MOFs) make them ideal substrates to support atomically dispersed metal sites (ADMSs) located in their metal nodes, linkers, and pores. Porous carbon materials doped with ADMSs can be derived from these ADMS‐incorporating MOF precursors through controlled treatments. These ADMSs incorporated in pristine MOFs and MOF‐derived carbon materials possess unique advantages over molecular or bulk metal‐based catalysts and bridge the gap between homogeneous and heterogeneous catalysts for energy‐conversion applications. This Review presents recent progress in the design and incorporation of ADMSs in MOFs and MOF‐derived materials for energy‐conversion applications. A site to behold: Atomically dispersed metal sites in MOFs and MOF‐derived materials offer great potential for the design and modification of advanced catalysts for applications in photocatalytic and electrocatalytic energy conversion. Recent breakthroughs and future perspectives are presented in this Review.
AbstractList Metal sites play an essential role in both electrocatalytic and photocatalytic energy conversion. The highly ordered arrangements of the organic linkers and metal nodes as well as the well-defined pore structures of metal-organic frameworks (MOFs) make them ideal substrates to support atomically dispersed metal sites (ADMSs) located in their metal nodes, linkers, and pores. Porous carbon materials doped with ADMSs can be derived from these ADMS-incorporating MOF precursors through controlled treatments. These ADMSs incorporated in pristine MOFs and MOF-derived carbon materials possess unique advantages over molecular or bulk metal-based catalysts and bridge the gap between homogeneous and heterogeneous catalysts for energy-conversion applications. This Review presents recent progress in the design and incorporation of ADMSs in MOFs and MOF-derived materials for energy-conversion applications.Metal sites play an essential role in both electrocatalytic and photocatalytic energy conversion. The highly ordered arrangements of the organic linkers and metal nodes as well as the well-defined pore structures of metal-organic frameworks (MOFs) make them ideal substrates to support atomically dispersed metal sites (ADMSs) located in their metal nodes, linkers, and pores. Porous carbon materials doped with ADMSs can be derived from these ADMS-incorporating MOF precursors through controlled treatments. These ADMSs incorporated in pristine MOFs and MOF-derived carbon materials possess unique advantages over molecular or bulk metal-based catalysts and bridge the gap between homogeneous and heterogeneous catalysts for energy-conversion applications. This Review presents recent progress in the design and incorporation of ADMSs in MOFs and MOF-derived materials for energy-conversion applications.
Metal sites play an essential role in both electrocatalytic and photocatalytic energy conversion. The highly ordered arrangements of the organic linkers and metal nodes as well as the well‐defined pore structures of metal‐organic frameworks (MOFs) make them ideal substrates to support atomically dispersed metal sites (ADMSs) located in their metal nodes, linkers, and pores. Porous carbon materials doped with ADMSs can be derived from these ADMS‐incorporating MOF precursors through controlled treatments. These ADMSs incorporated in pristine MOFs and MOF‐derived carbon materials possess unique advantages over molecular or bulk metal‐based catalysts and bridge the gap between homogeneous and heterogeneous catalysts for energy‐conversion applications. This Review presents recent progress in the design and incorporation of ADMSs in MOFs and MOF‐derived materials for energy‐conversion applications.
Metal sites play an essential role in both electrocatalytic and photocatalytic energy conversion. The highly ordered arrangements of the organic linkers and metal nodes as well as the well‐defined pore structures of metal‐organic frameworks (MOFs) make them ideal substrates to support atomically dispersed metal sites (ADMSs) located in their metal nodes, linkers, and pores. Porous carbon materials doped with ADMSs can be derived from these ADMS‐incorporating MOF precursors through controlled treatments. These ADMSs incorporated in pristine MOFs and MOF‐derived carbon materials possess unique advantages over molecular or bulk metal‐based catalysts and bridge the gap between homogeneous and heterogeneous catalysts for energy‐conversion applications. This Review presents recent progress in the design and incorporation of ADMSs in MOFs and MOF‐derived materials for energy‐conversion applications. A site to behold: Atomically dispersed metal sites in MOFs and MOF‐derived materials offer great potential for the design and modification of advanced catalysts for applications in photocatalytic and electrocatalytic energy conversion. Recent breakthroughs and future perspectives are presented in this Review.
Author Xia, Dingguo
Xu, Qiang
Qu, Chong
Zou, Ruqiang
Liang, Zibin
Author_xml – sequence: 1
  givenname: Zibin
  surname: Liang
  fullname: Liang, Zibin
  organization: Peking University
– sequence: 2
  givenname: Chong
  surname: Qu
  fullname: Qu, Chong
  organization: Peking University
– sequence: 3
  givenname: Dingguo
  surname: Xia
  fullname: Xia, Dingguo
  organization: Peking University
– sequence: 4
  givenname: Ruqiang
  surname: Zou
  fullname: Zou, Ruqiang
  email: rzou@pku.edu.cn
  organization: Peking University
– sequence: 5
  givenname: Qiang
  orcidid: 0000-0001-5385-9650
  surname: Xu
  fullname: Xu, Qiang
  email: q.xu@aist.go.jp
  organization: Yangzhou University
BackLink https://www.ncbi.nlm.nih.gov/pubmed/29460497$$D View this record in MEDLINE/PubMed
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Snippet Metal sites play an essential role in both electrocatalytic and photocatalytic energy conversion. The highly ordered arrangements of the organic linkers and...
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SubjectTerms Carbon
Catalysis
Catalysts
Dispersion
Energy
Energy conversion
heterogeneous catalysis
metal centers
Metal-organic frameworks
Metals
Molecular chains
Porous materials
single-atom catalysts
Substrates
Title Atomically Dispersed Metal Sites in MOF‐Based Materials for Electrocatalytic and Photocatalytic Energy Conversion
URI https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fanie.201800269
https://www.ncbi.nlm.nih.gov/pubmed/29460497
https://www.proquest.com/docview/2073941081
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Volume 57
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