Renewable Castor‐Oil‐based Waterborne Polyurethane Networks: Simultaneously Showing High Strength, Self‐Healing, Processability and Tunable Multishape Memory
Materials with multifunctionality or multiresponsiveness, especially polymers derived from green, renewable precursors, have recently attracted significant attention resulting from their technological impact. Nowadays, vegetable‐oil‐based waterborne polyurethanes (WPUs) are widely used in various fi...
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| Published in | Angewandte Chemie International Edition Vol. 60; no. 8; pp. 4289 - 4299 |
|---|---|
| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Germany
Wiley Subscription Services, Inc
19.02.2021
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| Edition | International ed. in English |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Materials with multifunctionality or multiresponsiveness, especially polymers derived from green, renewable precursors, have recently attracted significant attention resulting from their technological impact. Nowadays, vegetable‐oil‐based waterborne polyurethanes (WPUs) are widely used in various fields, while strategies for simultaneous realization of their self‐healing, reprocessing, shape memory as well as high mechanical properties are still highly anticipated. We report development of a multifunctional castor‐oil‐based waterborne polyurethane with high strength using controlled amounts of dithiodiphenylamine. The polymer networks possessed high tensile strength up to 38 MPa as well as excellent self‐healing efficiency. Moreover, the WPU film exhibited a maximum recovery of 100 % of the original mechanical properties after reprocessing four times. The broad glass‐transition temperature of the samples endowed the films with a versatile shape‐memory effect, including a dual‐to‐quadruple shape‐memory effect.
A castor‐oil‐based waterborne polyurethane (WPU) with high strength was developed. The PU networks demonstrated high tensile strength up to 38 MPa, excellent self‐healing with a tensile strength of 100 %, and a maximum recovery of 100 % of the original mechanical strength after reprocessing four times. The broad glass‐transition temperature of the samples endows the films with shape‐memory effects. |
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| AbstractList | Materials with multifunctionality or multiresponsiveness, especially polymers derived from green, renewable precursors, have recently attracted significant attention resulting from their technological impact. Nowadays, vegetable-oil-based waterborne polyurethanes (WPUs) are widely used in various fields, while strategies for simultaneous realization of their self-healing, reprocessing, shape memory as well as high mechanical properties are still highly anticipated. We report development of a multifunctional castor-oil-based waterborne polyurethane with high strength using controlled amounts of dithiodiphenylamine. The polymer networks possessed high tensile strength up to 38 MPa as well as excellent self-healing efficiency. Moreover, the WPU film exhibited a maximum recovery of 100 % of the original mechanical properties after reprocessing four times. The broad glass-transition temperature of the samples endowed the films with a versatile shape-memory effect, including a dual-to-quadruple shape-memory effect.Materials with multifunctionality or multiresponsiveness, especially polymers derived from green, renewable precursors, have recently attracted significant attention resulting from their technological impact. Nowadays, vegetable-oil-based waterborne polyurethanes (WPUs) are widely used in various fields, while strategies for simultaneous realization of their self-healing, reprocessing, shape memory as well as high mechanical properties are still highly anticipated. We report development of a multifunctional castor-oil-based waterborne polyurethane with high strength using controlled amounts of dithiodiphenylamine. The polymer networks possessed high tensile strength up to 38 MPa as well as excellent self-healing efficiency. Moreover, the WPU film exhibited a maximum recovery of 100 % of the original mechanical properties after reprocessing four times. The broad glass-transition temperature of the samples endowed the films with a versatile shape-memory effect, including a dual-to-quadruple shape-memory effect. Materials with multifunctionality or multiresponsiveness, especially polymers derived from green, renewable precursors, have recently attracted significant attention resulting from their technological impact. Nowadays, vegetable‐oil‐based waterborne polyurethanes (WPUs) are widely used in various fields, while strategies for simultaneous realization of their self‐healing, reprocessing, shape memory as well as high mechanical properties are still highly anticipated. We report development of a multifunctional castor‐oil‐based waterborne polyurethane with high strength using controlled amounts of dithiodiphenylamine. The polymer networks possessed high tensile strength up to 38 MPa as well as excellent self‐healing efficiency. Moreover, the WPU film exhibited a maximum recovery of 100 % of the original mechanical properties after reprocessing four times. The broad glass‐transition temperature of the samples endowed the films with a versatile shape‐memory effect, including a dual‐to‐quadruple shape‐memory effect. Materials with multifunctionality or multiresponsiveness, especially polymers derived from green, renewable precursors, have recently attracted significant attention resulting from their technological impact. Nowadays, vegetable‐oil‐based waterborne polyurethanes (WPUs) are widely used in various fields, while strategies for simultaneous realization of their self‐healing, reprocessing, shape memory as well as high mechanical properties are still highly anticipated. We report development of a multifunctional castor‐oil‐based waterborne polyurethane with high strength using controlled amounts of dithiodiphenylamine. The polymer networks possessed high tensile strength up to 38 MPa as well as excellent self‐healing efficiency. Moreover, the WPU film exhibited a maximum recovery of 100 % of the original mechanical properties after reprocessing four times. The broad glass‐transition temperature of the samples endowed the films with a versatile shape‐memory effect, including a dual‐to‐quadruple shape‐memory effect. A castor‐oil‐based waterborne polyurethane (WPU) with high strength was developed. The PU networks demonstrated high tensile strength up to 38 MPa, excellent self‐healing with a tensile strength of 100 %, and a maximum recovery of 100 % of the original mechanical strength after reprocessing four times. The broad glass‐transition temperature of the samples endows the films with shape‐memory effects. |
| Author | Feng, Pengju Lin, Zirun Liang, Haiyan Zhang, Chaoqun Liang, Dunsheng Wang, Qingwen Chen, Qian |
| Author_xml | – sequence: 1 givenname: Chaoqun surname: Zhang fullname: Zhang, Chaoqun email: zhangcq@scau.edu.cn, nwpuzcq@gmail.com organization: Guangdong Laboratory for Lingnan Modern Agriculture – sequence: 2 givenname: Haiyan surname: Liang fullname: Liang, Haiyan organization: Guangdong Laboratory for Lingnan Modern Agriculture – sequence: 3 givenname: Dunsheng surname: Liang fullname: Liang, Dunsheng organization: Guangdong Laboratory for Lingnan Modern Agriculture – sequence: 4 givenname: Zirun surname: Lin fullname: Lin, Zirun organization: Jinan University and Guangdong Provincial Key Laboratory of Functional Supramolecular Coordination Materials and Applications – sequence: 5 givenname: Qian surname: Chen fullname: Chen, Qian organization: South China Agricultural University, National Engineering Research Center for Breeding Swine Industry and Guangdong Provincial Key Laboratory of Agro-Animal Genomics – sequence: 6 givenname: Pengju orcidid: 0000-0002-5470-0403 surname: Feng fullname: Feng, Pengju email: pfeng@jnu.edu.cn organization: Jinan University and Guangdong Provincial Key Laboratory of Functional Supramolecular Coordination Materials and Applications – sequence: 7 givenname: Qingwen surname: Wang fullname: Wang, Qingwen organization: Guangdong Laboratory for Lingnan Modern Agriculture |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/33140558$$D View this record in MEDLINE/PubMed |
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| Copyright | 2020 Wiley‐VCH GmbH 2020 Wiley-VCH GmbH. 2021 Wiley‐VCH GmbH |
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| SubjectTerms | Healing High strength Mechanical properties multishape memory plant oil Polymers Polyurethane Polyurethane resins processability Reprocessing Shape effects Shape memory simultaneous self-healing Tensile strength Transition temperature Transition temperatures Vegetable oils waterborne polyurethane |
| Title | Renewable Castor‐Oil‐based Waterborne Polyurethane Networks: Simultaneously Showing High Strength, Self‐Healing, Processability and Tunable Multishape Memory |
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