Heterogeneous Catalysis in Zeolites, Mesoporous Silica, and Metal–Organic Frameworks

Crystalline porous materials are important in the development of catalytic systems with high scientific and industrial impact. Zeolites, ordered mesoporous silica, and metal–organic frameworks (MOFs) are three types of porous materials that can be used as heterogeneous catalysts. This review focuses...

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Published in	Advanced materials (Weinheim) Vol. 29; no. 30
Main Authors	Liang, Jie, Liang, Zibin, Zou, Ruqiang, Zhao, Yanli
Format	Journal Article
Language	English
Published	Germany Wiley Subscription Services, Inc 01.08.2017
Subjects	Catalysis Crystal structure heterogeneous catalysis Hydrogenation mesoporous silica Metal-organic frameworks Oxidation Porous materials Silica Silicon dioxide Zeolites mesoporous silica porous materials zeolites heterogeneous catalysis metal-organic frameworks
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Abstract	Crystalline porous materials are important in the development of catalytic systems with high scientific and industrial impact. Zeolites, ordered mesoporous silica, and metal–organic frameworks (MOFs) are three types of porous materials that can be used as heterogeneous catalysts. This review focuses on a comparison of the catalytic activities of zeolites, mesoporous silica, and MOFs. In the first part of the review, the distinctive properties of these porous materials relevant to catalysis are discussed, and the corresponding catalytic reactions are highlighted. In the second part, the catalytic behaviors of zeolites, mesoporous silica, and MOFs in four types of general organic reactions (acid, base, oxidation, and hydrogenation) are compared. The advantages and disadvantages of each porous material for catalytic reactions are summarized. Conclusions and prospects for future development of these porous materials in this field are provided in the last section. This review aims to highlight recent research advancements in zeolites, ordered mesoporous silica, and MOFs for heterogeneous catalysis, and inspire further studies in this rapidly developing field. The similarities and differences in catalytic behavior of zeolites, mesoporous silica, and metal–organic frameworks in four types of general organic reactions (acid, base, oxidation, and hydrogenation) are discussed herein. The advantages and disadvantages of each porous material for particular catalytic reactions are highlighted. Future developments of the three types of porous materials in heterogeneous catalysis are also discussed.
AbstractList	Crystalline porous materials are important in the development of catalytic systems with high scientific and industrial impact. Zeolites, ordered mesoporous silica, and metal-organic frameworks (MOFs) are three types of porous materials that can be used as heterogeneous catalysts. This review focuses on a comparison of the catalytic activities of zeolites, mesoporous silica, and MOFs. In the first part of the review, the distinctive properties of these porous materials relevant to catalysis are discussed, and the corresponding catalytic reactions are highlighted. In the second part, the catalytic behaviors of zeolites, mesoporous silica, and MOFs in four types of general organic reactions (acid, base, oxidation, and hydrogenation) are compared. The advantages and disadvantages of each porous material for catalytic reactions are summarized. Conclusions and prospects for future development of these porous materials in this field are provided in the last section. This review aims to highlight recent research advancements in zeolites, ordered mesoporous silica, and MOFs for heterogeneous catalysis, and inspire further studies in this rapidly developing field. Crystalline porous materials are important in the development of catalytic systems with high scientific and industrial impact. Zeolites, ordered mesoporous silica, and metal-organic frameworks (MOFs) are three types of porous materials that can be used as heterogeneous catalysts. This review focuses on a comparison of the catalytic activities of zeolites, mesoporous silica, and MOFs. In the first part of the review, the distinctive properties of these porous materials relevant to catalysis are discussed, and the corresponding catalytic reactions are highlighted. In the second part, the catalytic behaviors of zeolites, mesoporous silica, and MOFs in four types of general organic reactions (acid, base, oxidation, and hydrogenation) are compared. The advantages and disadvantages of each porous material for catalytic reactions are summarized. Conclusions and prospects for future development of these porous materials in this field are provided in the last section. This review aims to highlight recent research advancements in zeolites, ordered mesoporous silica, and MOFs for heterogeneous catalysis, and inspire further studies in this rapidly developing field.Crystalline porous materials are important in the development of catalytic systems with high scientific and industrial impact. Zeolites, ordered mesoporous silica, and metal-organic frameworks (MOFs) are three types of porous materials that can be used as heterogeneous catalysts. This review focuses on a comparison of the catalytic activities of zeolites, mesoporous silica, and MOFs. In the first part of the review, the distinctive properties of these porous materials relevant to catalysis are discussed, and the corresponding catalytic reactions are highlighted. In the second part, the catalytic behaviors of zeolites, mesoporous silica, and MOFs in four types of general organic reactions (acid, base, oxidation, and hydrogenation) are compared. The advantages and disadvantages of each porous material for catalytic reactions are summarized. Conclusions and prospects for future development of these porous materials in this field are provided in the last section. This review aims to highlight recent research advancements in zeolites, ordered mesoporous silica, and MOFs for heterogeneous catalysis, and inspire further studies in this rapidly developing field. Crystalline porous materials are important in the development of catalytic systems with high scientific and industrial impact. Zeolites, ordered mesoporous silica, and metal–organic frameworks (MOFs) are three types of porous materials that can be used as heterogeneous catalysts. This review focuses on a comparison of the catalytic activities of zeolites, mesoporous silica, and MOFs. In the first part of the review, the distinctive properties of these porous materials relevant to catalysis are discussed, and the corresponding catalytic reactions are highlighted. In the second part, the catalytic behaviors of zeolites, mesoporous silica, and MOFs in four types of general organic reactions (acid, base, oxidation, and hydrogenation) are compared. The advantages and disadvantages of each porous material for catalytic reactions are summarized. Conclusions and prospects for future development of these porous materials in this field are provided in the last section. This review aims to highlight recent research advancements in zeolites, ordered mesoporous silica, and MOFs for heterogeneous catalysis, and inspire further studies in this rapidly developing field. The similarities and differences in catalytic behavior of zeolites, mesoporous silica, and metal–organic frameworks in four types of general organic reactions (acid, base, oxidation, and hydrogenation) are discussed herein. The advantages and disadvantages of each porous material for particular catalytic reactions are highlighted. Future developments of the three types of porous materials in heterogeneous catalysis are also discussed.
Author	Liang, Jie Zou, Ruqiang Zhao, Yanli Liang, Zibin
Author_xml	– sequence: 1 givenname: Jie surname: Liang fullname: Liang, Jie organization: Chinese Academy of Geological Sciences – sequence: 2 givenname: Zibin surname: Liang fullname: Liang, Zibin organization: Peking University – sequence: 3 givenname: Ruqiang surname: Zou fullname: Zou, Ruqiang email: rzou@pku.edu.cn organization: Peking University – sequence: 4 givenname: Yanli orcidid: 0000-0002-9231-8360 surname: Zhao fullname: Zhao, Yanli email: zhaoyanli@ntu.edu.sg organization: Nanyang Technological University
BackLink	https://www.ncbi.nlm.nih.gov/pubmed/28628246$$D View this record in MEDLINE/PubMed
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Keywords	mesoporous silica porous materials zeolites heterogeneous catalysis metal-organic frameworks
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Snippet	Crystalline porous materials are important in the development of catalytic systems with high scientific and industrial impact. Zeolites, ordered mesoporous...
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SubjectTerms	Catalysis Crystal structure heterogeneous catalysis Hydrogenation mesoporous silica Metal-organic frameworks Oxidation Porous materials Silica Silicon dioxide Zeolites
Title	Heterogeneous Catalysis in Zeolites, Mesoporous Silica, and Metal–Organic Frameworks
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