Inhibiting Solvent Co‐Intercalation in a Graphite Anode by a Localized High‐Concentration Electrolyte in Fast‐Charging Batteries
Lithium‐ion batteries with routine carbonate electrolytes cannot exhibit satisfactory fast‐charging performance and lithium plating is widely observed at low temperatures. Herein we demonstrate that a localized high‐concentration electrolyte consisting of 1.5 M lithium bis(fluorosulfonyl)imide in di...
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| Published in | Angewandte Chemie International Edition Vol. 60; no. 7; pp. 3402 - 3406 |
|---|---|
| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Germany
Wiley Subscription Services, Inc
15.02.2021
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| Edition | International ed. in English |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Lithium‐ion batteries with routine carbonate electrolytes cannot exhibit satisfactory fast‐charging performance and lithium plating is widely observed at low temperatures. Herein we demonstrate that a localized high‐concentration electrolyte consisting of 1.5 M lithium bis(fluorosulfonyl)imide in dimethoxyethane with bis(2,2,2‐trifluoroethyl) ether as the diluent, enables fast‐charging of working batteries. A uniform and robust solid electrolyte interphase (SEI) can be achieved on graphite surface through the preferential decomposition of anions. The established SEI can significantly inhibit ether solvent co‐intercalation into graphite and achieve highly reversible Li+ intercalation/de‐intercalation. The graphite | Li cells exhibit fast‐charging potential (340 mAh g−1 at 0.2 C and 220 mAh g−1 at 4 C), excellent cycling stability (ca. 85.5 % initial capacity retention for 200 cycles at 4 C), and impressive low‐temperature performance.
The unique solvation structure in a localized high‐concentration electrolyte can suppress co‐intercalation of ether solvent into the graphite interlayers and render fast‐charging of practical lithium‐ion batteries. |
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| AbstractList | Lithium-ion batteries with routine carbonate electrolytes cannot exhibit satisfactory fast-charging performance and lithium plating is widely observed at low temperatures. Herein we demonstrate that a localized high-concentration electrolyte consisting of 1.5 M lithium bis(fluorosulfonyl)imide in dimethoxyethane with bis(2,2,2-trifluoroethyl) ether as the diluent, enables fast-charging of working batteries. A uniform and robust solid electrolyte interphase (SEI) can be achieved on graphite surface through the preferential decomposition of anions. The established SEI can significantly inhibit ether solvent co-intercalation into graphite and achieve highly reversible Li+ intercalation/de-intercalation. The graphite | Li cells exhibit fast-charging potential (340 mAh g-1 at 0.2 C and 220 mAh g-1 at 4 C), excellent cycling stability (ca. 85.5 % initial capacity retention for 200 cycles at 4 C), and impressive low-temperature performance.Lithium-ion batteries with routine carbonate electrolytes cannot exhibit satisfactory fast-charging performance and lithium plating is widely observed at low temperatures. Herein we demonstrate that a localized high-concentration electrolyte consisting of 1.5 M lithium bis(fluorosulfonyl)imide in dimethoxyethane with bis(2,2,2-trifluoroethyl) ether as the diluent, enables fast-charging of working batteries. A uniform and robust solid electrolyte interphase (SEI) can be achieved on graphite surface through the preferential decomposition of anions. The established SEI can significantly inhibit ether solvent co-intercalation into graphite and achieve highly reversible Li+ intercalation/de-intercalation. The graphite | Li cells exhibit fast-charging potential (340 mAh g-1 at 0.2 C and 220 mAh g-1 at 4 C), excellent cycling stability (ca. 85.5 % initial capacity retention for 200 cycles at 4 C), and impressive low-temperature performance. Lithium-ion batteries with routine carbonate electrolytes cannot exhibit satisfactory fast-charging performance and lithium plating is widely observed at low temperatures. Herein we demonstrate that a localized high-concentration electrolyte consisting of 1.5 M lithium bis(fluorosulfonyl)imide in dimethoxyethane with bis(2,2,2-trifluoroethyl) ether as the diluent, enables fast-charging of working batteries. A uniform and robust solid electrolyte interphase (SEI) can be achieved on graphite surface through the preferential decomposition of anions. The established SEI can significantly inhibit ether solvent co-intercalation into graphite and achieve highly reversible Li intercalation/de-intercalation. The graphite | Li cells exhibit fast-charging potential (340 mAh g at 0.2 C and 220 mAh g at 4 C), excellent cycling stability (ca. 85.5 % initial capacity retention for 200 cycles at 4 C), and impressive low-temperature performance. Lithium‐ion batteries with routine carbonate electrolytes cannot exhibit satisfactory fast‐charging performance and lithium plating is widely observed at low temperatures. Herein we demonstrate that a localized high‐concentration electrolyte consisting of 1.5 M lithium bis(fluorosulfonyl)imide in dimethoxyethane with bis(2,2,2‐trifluoroethyl) ether as the diluent, enables fast‐charging of working batteries. A uniform and robust solid electrolyte interphase (SEI) can be achieved on graphite surface through the preferential decomposition of anions. The established SEI can significantly inhibit ether solvent co‐intercalation into graphite and achieve highly reversible Li+ intercalation/de‐intercalation. The graphite | Li cells exhibit fast‐charging potential (340 mAh g−1 at 0.2 C and 220 mAh g−1 at 4 C), excellent cycling stability (ca. 85.5 % initial capacity retention for 200 cycles at 4 C), and impressive low‐temperature performance. The unique solvation structure in a localized high‐concentration electrolyte can suppress co‐intercalation of ether solvent into the graphite interlayers and render fast‐charging of practical lithium‐ion batteries. Lithium‐ion batteries with routine carbonate electrolytes cannot exhibit satisfactory fast‐charging performance and lithium plating is widely observed at low temperatures. Herein we demonstrate that a localized high‐concentration electrolyte consisting of 1.5 M lithium bis(fluorosulfonyl)imide in dimethoxyethane with bis(2,2,2‐trifluoroethyl) ether as the diluent, enables fast‐charging of working batteries. A uniform and robust solid electrolyte interphase (SEI) can be achieved on graphite surface through the preferential decomposition of anions. The established SEI can significantly inhibit ether solvent co‐intercalation into graphite and achieve highly reversible Li+ intercalation/de‐intercalation. The graphite | Li cells exhibit fast‐charging potential (340 mAh g−1 at 0.2 C and 220 mAh g−1 at 4 C), excellent cycling stability (ca. 85.5 % initial capacity retention for 200 cycles at 4 C), and impressive low‐temperature performance. Lithium‐ion batteries with routine carbonate electrolytes cannot exhibit satisfactory fast‐charging performance and lithium plating is widely observed at low temperatures. Herein we demonstrate that a localized high‐concentration electrolyte consisting of 1.5 M lithium bis(fluorosulfonyl)imide in dimethoxyethane with bis(2,2,2‐trifluoroethyl) ether as the diluent, enables fast‐charging of working batteries. A uniform and robust solid electrolyte interphase (SEI) can be achieved on graphite surface through the preferential decomposition of anions. The established SEI can significantly inhibit ether solvent co‐intercalation into graphite and achieve highly reversible Li + intercalation/de‐intercalation. The graphite | Li cells exhibit fast‐charging potential (340 mAh g −1 at 0.2 C and 220 mAh g −1 at 4 C), excellent cycling stability (ca. 85.5 % initial capacity retention for 200 cycles at 4 C), and impressive low‐temperature performance. |
| Author | Huang, Jia‐Qi Jiang, Li‐Li Cai, Wenlong Yao, Yu‐Xing Zhang, Qiang Yan, Chong |
| Author_xml | – sequence: 1 givenname: Li‐Li surname: Jiang fullname: Jiang, Li‐Li organization: Jilin Institute of Chemical Technology – sequence: 2 givenname: Chong surname: Yan fullname: Yan, Chong organization: Tsinghua University – sequence: 3 givenname: Yu‐Xing surname: Yao fullname: Yao, Yu‐Xing organization: Tsinghua University – sequence: 4 givenname: Wenlong surname: Cai fullname: Cai, Wenlong organization: Tsinghua University – sequence: 5 givenname: Jia‐Qi surname: Huang fullname: Huang, Jia‐Qi organization: Beijing Institute of Technology – sequence: 6 givenname: Qiang orcidid: 0000-0002-3929-1541 surname: Zhang fullname: Zhang, Qiang email: zhang-qiang@mails.tsinghua.edu.cn organization: Tsinghua University |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/33107707$$D View this record in MEDLINE/PubMed |
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| Snippet | Lithium‐ion batteries with routine carbonate electrolytes cannot exhibit satisfactory fast‐charging performance and lithium plating is widely observed at low... Lithium-ion batteries with routine carbonate electrolytes cannot exhibit satisfactory fast-charging performance and lithium plating is widely observed at low... |
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| SubjectTerms | Anions Charging Electrolytes Electrolytic cells fast-charging Graphite graphite anodes Intercalation Lithium Lithium-ion batteries localized high-concentration electrolyte Low temperature Solid electrolytes solvent co-intercalation Solvents |
| Title | Inhibiting Solvent Co‐Intercalation in a Graphite Anode by a Localized High‐Concentration Electrolyte in Fast‐Charging Batteries |
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