Phase‐Selective Syntheses of Cobalt Telluride Nanofleeces for Efficient Oxygen Evolution Catalysts
Cobalt‐based nanomaterials have been intensively explored as promising noble‐metal‐free oxygen evolution reaction (OER) electrocatalysts. Herein, we report phase‐selective syntheses of novel hierarchical CoTe2 and CoTe nanofleeces for efficient OER catalysts. The CoTe2 nanofleeces exhibited excellen...
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| Published in | Angewandte Chemie International Edition Vol. 56; no. 27; pp. 7769 - 7773 |
|---|---|
| Main Authors | , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Germany
Wiley Subscription Services, Inc
26.06.2017
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| Edition | International ed. in English |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Cobalt‐based nanomaterials have been intensively explored as promising noble‐metal‐free oxygen evolution reaction (OER) electrocatalysts. Herein, we report phase‐selective syntheses of novel hierarchical CoTe2 and CoTe nanofleeces for efficient OER catalysts. The CoTe2 nanofleeces exhibited excellent electrocatalytic activity and stablity for OER in alkaline media. The CoTe2 catalyst exhibited superior OER activity compared to the CoTe catalyst, which is comparable to the state‐of‐the‐art RuO2 catalyst. Density functional theory calculations showed that the binding strength and lateral interaction of the reaction intermediates on CoTe2 and CoTe are essential for determining the overpotential required under different conditions. This study provides valuable insights for the rational design of noble‐metal‐free OER catalysts with high performance and low cost by use of Co‐based chalcogenides.
Fleeced: Hierarchical CoTe2 nanofleeces were synthesized by using ultrathin Te nanowires as templates. They exhibited excellent electrocatalytic activity and stablity for the oxygen evolution reaction (OER) in alkaline media. The CoTe2 catalyst exhibited superior OER activity to the CoTe catalyst and was comparable to the state‐of‐the‐art RuO2 catalyst. |
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| AbstractList | Cobalt‐based nanomaterials have been intensively explored as promising noble‐metal‐free oxygen evolution reaction (OER) electrocatalysts. Herein, we report phase‐selective syntheses of novel hierarchical CoTe2 and CoTe nanofleeces for efficient OER catalysts. The CoTe2 nanofleeces exhibited excellent electrocatalytic activity and stablity for OER in alkaline media. The CoTe2 catalyst exhibited superior OER activity compared to the CoTe catalyst, which is comparable to the state‐of‐the‐art RuO2 catalyst. Density functional theory calculations showed that the binding strength and lateral interaction of the reaction intermediates on CoTe2 and CoTe are essential for determining the overpotential required under different conditions. This study provides valuable insights for the rational design of noble‐metal‐free OER catalysts with high performance and low cost by use of Co‐based chalcogenides.
Fleeced: Hierarchical CoTe2 nanofleeces were synthesized by using ultrathin Te nanowires as templates. They exhibited excellent electrocatalytic activity and stablity for the oxygen evolution reaction (OER) in alkaline media. The CoTe2 catalyst exhibited superior OER activity to the CoTe catalyst and was comparable to the state‐of‐the‐art RuO2 catalyst. Cobalt-based nanomaterials have been intensively explored as promising noble-metal-free oxygen evolution reaction (OER) electrocatalysts. Herein, we report phase-selective syntheses of novel hierarchical CoTe2 and CoTe nanofleeces for efficient OER catalysts. The CoTe2 nanofleeces exhibited excellent electrocatalytic activity and stablity for OER in alkaline media. The CoTe2 catalyst exhibited superior OER activity compared to the CoTe catalyst, which is comparable to the state-of-the-art RuO2 catalyst. Density functional theory calculations showed that the binding strength and lateral interaction of the reaction intermediates on CoTe2 and CoTe are essential for determining the overpotential required under different conditions. This study provides valuable insights for the rational design of noble-metal-free OER catalysts with high performance and low cost by use of Co-based chalcogenides. Cobalt-based nanomaterials have been intensively explored as promising noble-metal-free oxygen evolution reaction (OER) electrocatalysts. Herein, we report phase-selective syntheses of novel hierarchical CoTe2 and CoTe nanofleeces for efficient OER catalysts. The CoTe2 nanofleeces exhibited excellent electrocatalytic activity and stablity for OER in alkaline media. The CoTe2 catalyst exhibited superior OER activity compared to the CoTe catalyst, which is comparable to the state-of-the-art RuO2 catalyst. Density functional theory calculations showed that the binding strength and lateral interaction of the reaction intermediates on CoTe2 and CoTe are essential for determining the overpotential required under different conditions. This study provides valuable insights for the rational design of noble-metal-free OER catalysts with high performance and low cost by use of Co-based chalcogenides.Cobalt-based nanomaterials have been intensively explored as promising noble-metal-free oxygen evolution reaction (OER) electrocatalysts. Herein, we report phase-selective syntheses of novel hierarchical CoTe2 and CoTe nanofleeces for efficient OER catalysts. The CoTe2 nanofleeces exhibited excellent electrocatalytic activity and stablity for OER in alkaline media. The CoTe2 catalyst exhibited superior OER activity compared to the CoTe catalyst, which is comparable to the state-of-the-art RuO2 catalyst. Density functional theory calculations showed that the binding strength and lateral interaction of the reaction intermediates on CoTe2 and CoTe are essential for determining the overpotential required under different conditions. This study provides valuable insights for the rational design of noble-metal-free OER catalysts with high performance and low cost by use of Co-based chalcogenides. Cobalt-based nanomaterials have been intensively explored as promising noble-metal-free oxygen evolution reaction (OER) electrocatalysts. Herein, we report phase-selective syntheses of novel hierarchical CoTe and CoTe nanofleeces for efficient OER catalysts. The CoTe nanofleeces exhibited excellent electrocatalytic activity and stablity for OER in alkaline media. The CoTe catalyst exhibited superior OER activity compared to the CoTe catalyst, which is comparable to the state-of-the-art RuO catalyst. Density functional theory calculations showed that the binding strength and lateral interaction of the reaction intermediates on CoTe and CoTe are essential for determining the overpotential required under different conditions. This study provides valuable insights for the rational design of noble-metal-free OER catalysts with high performance and low cost by use of Co-based chalcogenides. Cobalt‐based nanomaterials have been intensively explored as promising noble‐metal‐free oxygen evolution reaction (OER) electrocatalysts. Herein, we report phase‐selective syntheses of novel hierarchical CoTe 2 and CoTe nanofleeces for efficient OER catalysts. The CoTe 2 nanofleeces exhibited excellent electrocatalytic activity and stablity for OER in alkaline media. The CoTe 2 catalyst exhibited superior OER activity compared to the CoTe catalyst, which is comparable to the state‐of‐the‐art RuO 2 catalyst. Density functional theory calculations showed that the binding strength and lateral interaction of the reaction intermediates on CoTe 2 and CoTe are essential for determining the overpotential required under different conditions. This study provides valuable insights for the rational design of noble‐metal‐free OER catalysts with high performance and low cost by use of Co‐based chalcogenides. |
| Author | Liu, Jian‐Wei Huang, Chuan‐Qi Li, Wei‐Xue Gao, Min‐Rui Ju, Yi‐Ming Zheng, Ya‐Rong An, Duo Yu, Shu‐Hong Gao, Qiang Cui, Chun‐Hua |
| Author_xml | – sequence: 1 givenname: Qiang surname: Gao fullname: Gao, Qiang organization: University of Science and Technology of China – sequence: 2 givenname: Chuan‐Qi surname: Huang fullname: Huang, Chuan‐Qi organization: University of Science and Technology of China – sequence: 3 givenname: Yi‐Ming surname: Ju fullname: Ju, Yi‐Ming organization: University of Science and Technology of China – sequence: 4 givenname: Min‐Rui surname: Gao fullname: Gao, Min‐Rui organization: University of Science and Technology of China – sequence: 5 givenname: Jian‐Wei surname: Liu fullname: Liu, Jian‐Wei organization: University of Science and Technology of China – sequence: 6 givenname: Duo surname: An fullname: An, Duo organization: University of Science and Technology of China – sequence: 7 givenname: Chun‐Hua surname: Cui fullname: Cui, Chun‐Hua organization: University of Science and Technology of China – sequence: 8 givenname: Ya‐Rong surname: Zheng fullname: Zheng, Ya‐Rong organization: University of Science and Technology of China – sequence: 9 givenname: Wei‐Xue surname: Li fullname: Li, Wei‐Xue email: wxli70@ustc.edu.cn organization: University of Science and Technology of China – sequence: 10 givenname: Shu‐Hong orcidid: 0000-0003-3732-1011 surname: Yu fullname: Yu, Shu‐Hong email: shyu@ustc.edu.cn organization: University of Science and Technology of China |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/28467678$$D View this record in MEDLINE/PubMed |
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| Copyright | 2017 Wiley‐VCH Verlag GmbH & Co. KGaA, Weinheim 2017 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim. 2017 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim |
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| Keywords | tellurium electrocatalyst oxygen evolution reaction cobalt hierarchical structure |
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| Snippet | Cobalt‐based nanomaterials have been intensively explored as promising noble‐metal‐free oxygen evolution reaction (OER) electrocatalysts. Herein, we report... Cobalt-based nanomaterials have been intensively explored as promising noble-metal-free oxygen evolution reaction (OER) electrocatalysts. Herein, we report... |
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| SubjectTerms | Catalysts Chalcogenides Cobalt Density functional theory electrocatalyst Electrocatalysts Evolution hierarchical structure Intermediates Intermetallic compounds Low cost Nanomaterials Nanotechnology Oxygen oxygen evolution reaction Reaction intermediates Ruthenium oxide Tellurides tellurium |
| Title | Phase‐Selective Syntheses of Cobalt Telluride Nanofleeces for Efficient Oxygen Evolution Catalysts |
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