Chiral Lead‐Free Hybrid Perovskites for Self‐Powered Circularly Polarized Light Detection
Metal‐halide perovskites are recently emerging as the promising alternative for CPL detection owing to their CPL‐sensitive property induced by chiral organics and efficient charge transport of inorganic frameworks. However, most of these reported chiral perovskites involve high concentrations of tox...
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| Published in | Angewandte Chemie International Edition Vol. 60; no. 15; pp. 8415 - 8418 |
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| Main Authors | , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Germany
Wiley Subscription Services, Inc
06.04.2021
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| Edition | International ed. in English |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Metal‐halide perovskites are recently emerging as the promising alternative for CPL detection owing to their CPL‐sensitive property induced by chiral organics and efficient charge transport of inorganic frameworks. However, most of these reported chiral perovskites involve high concentrations of toxic Pb which will become the potential bottleneck for their further application. Herein, we successfully developed two lead‐free halide double perovskites, [(R)‐β‐MPA]4AgBiI8 ((R)‐β‐MPA=(R)‐(+)‐β‐methylphenethylammonium, 1‐R), and [(S)‐β‐MPA]4AgBiI8 ((S)‐β‐MPA=(S)‐(−)‐β‐methylphenethylammonium, 1‐S). Circular dichroism measurements reveal that these perovskites exhibit notable chirality induced by organic cations to distinguish different polarization states of CPL photons. Significantly, they present unique chiral polar photovoltaic, and resulting self‐powered CPL detection without an external power source is unprecedentedly achieved. Furthermore, an anisotropy factor up to 0.3 is acquired for the self‐powered CPL detection, reaching the highest value among reported chiral perovskites. This work suggests hybrid double perovskites are promising photoelectronic candidates, and provides a new approach for exploring new “green” circularly polarized light‐sensitive materials with high performance.
Chiral lead‐free double hybrid perovskites are successfully acquired by assembling chiral organic cation with Ag+ and Bi3+ double metals. Benefitting from chiral polar bulk photovoltaic effects induced by polar structure, self‐powered circularly polarized light detection with a high anisotropy factor of 0.3 is unprecedentedly achieved in chiral hybrid perovskites. |
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| AbstractList | Metal‐halide perovskites are recently emerging as the promising alternative for CPL detection owing to their CPL‐sensitive property induced by chiral organics and efficient charge transport of inorganic frameworks. However, most of these reported chiral perovskites involve high concentrations of toxic Pb which will become the potential bottleneck for their further application. Herein, we successfully developed two lead‐free halide double perovskites, [(R)‐β‐MPA]4AgBiI8 ((R)‐β‐MPA=(R)‐(+)‐β‐methylphenethylammonium, 1‐R), and [(S)‐β‐MPA]4AgBiI8 ((S)‐β‐MPA=(S)‐(−)‐β‐methylphenethylammonium, 1‐S). Circular dichroism measurements reveal that these perovskites exhibit notable chirality induced by organic cations to distinguish different polarization states of CPL photons. Significantly, they present unique chiral polar photovoltaic, and resulting self‐powered CPL detection without an external power source is unprecedentedly achieved. Furthermore, an anisotropy factor up to 0.3 is acquired for the self‐powered CPL detection, reaching the highest value among reported chiral perovskites. This work suggests hybrid double perovskites are promising photoelectronic candidates, and provides a new approach for exploring new “green” circularly polarized light‐sensitive materials with high performance.
Chiral lead‐free double hybrid perovskites are successfully acquired by assembling chiral organic cation with Ag+ and Bi3+ double metals. Benefitting from chiral polar bulk photovoltaic effects induced by polar structure, self‐powered circularly polarized light detection with a high anisotropy factor of 0.3 is unprecedentedly achieved in chiral hybrid perovskites. Metal‐halide perovskites are recently emerging as the promising alternative for CPL detection owing to their CPL‐sensitive property induced by chiral organics and efficient charge transport of inorganic frameworks. However, most of these reported chiral perovskites involve high concentrations of toxic Pb which will become the potential bottleneck for their further application. Herein, we successfully developed two lead‐free halide double perovskites, [(R)‐β‐MPA]4AgBiI8 ((R)‐β‐MPA=(R)‐(+)‐β‐methylphenethylammonium, 1‐R), and [(S)‐β‐MPA]4AgBiI8 ((S)‐β‐MPA=(S)‐(−)‐β‐methylphenethylammonium, 1‐S). Circular dichroism measurements reveal that these perovskites exhibit notable chirality induced by organic cations to distinguish different polarization states of CPL photons. Significantly, they present unique chiral polar photovoltaic, and resulting self‐powered CPL detection without an external power source is unprecedentedly achieved. Furthermore, an anisotropy factor up to 0.3 is acquired for the self‐powered CPL detection, reaching the highest value among reported chiral perovskites. This work suggests hybrid double perovskites are promising photoelectronic candidates, and provides a new approach for exploring new “green” circularly polarized light‐sensitive materials with high performance. Metal‐halide perovskites are recently emerging as the promising alternative for CPL detection owing to their CPL‐sensitive property induced by chiral organics and efficient charge transport of inorganic frameworks. However, most of these reported chiral perovskites involve high concentrations of toxic Pb which will become the potential bottleneck for their further application. Herein, we successfully developed two lead‐free halide double perovskites, [( R )‐β‐MPA] 4 AgBiI 8 (( R )‐β‐MPA=( R )‐(+)‐β‐methylphenethylammonium, 1‐ R ), and [( S )‐β‐MPA] 4 AgBiI 8 (( S )‐β‐MPA=( S )‐(−)‐β‐methylphenethylammonium, 1‐ S ). Circular dichroism measurements reveal that these perovskites exhibit notable chirality induced by organic cations to distinguish different polarization states of CPL photons. Significantly, they present unique chiral polar photovoltaic, and resulting self‐powered CPL detection without an external power source is unprecedentedly achieved. Furthermore, an anisotropy factor up to 0.3 is acquired for the self‐powered CPL detection, reaching the highest value among reported chiral perovskites. This work suggests hybrid double perovskites are promising photoelectronic candidates, and provides a new approach for exploring new “green” circularly polarized light‐sensitive materials with high performance. Metal-halide perovskites are recently emerging as the promising alternative for CPL detection owing to their CPL-sensitive property induced by chiral organics and efficient charge transport of inorganic frameworks. However, most of these reported chiral perovskites involve high concentrations of toxic Pb which will become the potential bottleneck for their further application. Herein, we successfully developed two lead-free halide double perovskites, [(R)-β-MPA] AgBiI ((R)-β-MPA=(R)-(+)-β-methylphenethylammonium, 1-R), and [(S)-β-MPA] AgBiI ((S)-β-MPA=(S)-(-)-β-methylphenethylammonium, 1-S). Circular dichroism measurements reveal that these perovskites exhibit notable chirality induced by organic cations to distinguish different polarization states of CPL photons. Significantly, they present unique chiral polar photovoltaic, and resulting self-powered CPL detection without an external power source is unprecedentedly achieved. Furthermore, an anisotropy factor up to 0.3 is acquired for the self-powered CPL detection, reaching the highest value among reported chiral perovskites. This work suggests hybrid double perovskites are promising photoelectronic candidates, and provides a new approach for exploring new "green" circularly polarized light-sensitive materials with high performance. Metal-halide perovskites are recently emerging as the promising alternative for CPL detection owing to their CPL-sensitive property induced by chiral organics and efficient charge transport of inorganic frameworks. However, most of these reported chiral perovskites involve high concentrations of toxic Pb which will become the potential bottleneck for their further application. Herein, we successfully developed two lead-free halide double perovskites, [(R)-β-MPA]4 AgBiI8 ((R)-β-MPA=(R)-(+)-β-methylphenethylammonium, 1-R), and [(S)-β-MPA]4 AgBiI8 ((S)-β-MPA=(S)-(-)-β-methylphenethylammonium, 1-S). Circular dichroism measurements reveal that these perovskites exhibit notable chirality induced by organic cations to distinguish different polarization states of CPL photons. Significantly, they present unique chiral polar photovoltaic, and resulting self-powered CPL detection without an external power source is unprecedentedly achieved. Furthermore, an anisotropy factor up to 0.3 is acquired for the self-powered CPL detection, reaching the highest value among reported chiral perovskites. This work suggests hybrid double perovskites are promising photoelectronic candidates, and provides a new approach for exploring new "green" circularly polarized light-sensitive materials with high performance.Metal-halide perovskites are recently emerging as the promising alternative for CPL detection owing to their CPL-sensitive property induced by chiral organics and efficient charge transport of inorganic frameworks. However, most of these reported chiral perovskites involve high concentrations of toxic Pb which will become the potential bottleneck for their further application. Herein, we successfully developed two lead-free halide double perovskites, [(R)-β-MPA]4 AgBiI8 ((R)-β-MPA=(R)-(+)-β-methylphenethylammonium, 1-R), and [(S)-β-MPA]4 AgBiI8 ((S)-β-MPA=(S)-(-)-β-methylphenethylammonium, 1-S). Circular dichroism measurements reveal that these perovskites exhibit notable chirality induced by organic cations to distinguish different polarization states of CPL photons. Significantly, they present unique chiral polar photovoltaic, and resulting self-powered CPL detection without an external power source is unprecedentedly achieved. Furthermore, an anisotropy factor up to 0.3 is acquired for the self-powered CPL detection, reaching the highest value among reported chiral perovskites. This work suggests hybrid double perovskites are promising photoelectronic candidates, and provides a new approach for exploring new "green" circularly polarized light-sensitive materials with high performance. |
| Author | Li, Lina Zhao, Sangen Li, Dong Peng, Yu Liu, Xitao Wu, Wentao Luo, Junhua Hong, Maochun |
| Author_xml | – sequence: 1 givenname: Dong surname: Li fullname: Li, Dong organization: Fujian Science & Technology Innovation Laboratory for, Optoelectronic Information of China – sequence: 2 givenname: Xitao surname: Liu fullname: Liu, Xitao organization: University of Chinese Academy of Sciences – sequence: 3 givenname: Wentao surname: Wu fullname: Wu, Wentao organization: Fujian Science & Technology Innovation Laboratory for, Optoelectronic Information of China – sequence: 4 givenname: Yu surname: Peng fullname: Peng, Yu organization: Fujian Science & Technology Innovation Laboratory for, Optoelectronic Information of China – sequence: 5 givenname: Sangen surname: Zhao fullname: Zhao, Sangen organization: Fujian Science & Technology Innovation Laboratory for, Optoelectronic Information of China – sequence: 6 givenname: Lina surname: Li fullname: Li, Lina email: lilina@fjirsm.ac.cn organization: University of Chinese Academy of Sciences – sequence: 7 givenname: Maochun surname: Hong fullname: Hong, Maochun organization: University of Chinese Academy of Sciences – sequence: 8 givenname: Junhua orcidid: 0000-0002-3179-7652 surname: Luo fullname: Luo, Junhua email: jhluo@fjirsm.ac.cn organization: University of Chinese Academy of Sciences |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/33347688$$D View this record in MEDLINE/PubMed |
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| Keywords | double hybrid perovskite self-powered photodetection circularly polarized light detection lead-free chiral polar photovoltaic |
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| Snippet | Metal‐halide perovskites are recently emerging as the promising alternative for CPL detection owing to their CPL‐sensitive property induced by chiral organics... Metal-halide perovskites are recently emerging as the promising alternative for CPL detection owing to their CPL-sensitive property induced by chiral organics... |
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| SubjectTerms | Anisotropy Cations Charge transport chiral polar photovoltaic Chirality Circular dichroism Circular polarization circularly polarized light detection Dichroism double hybrid perovskite Lead lead-free Perovskites Photons Photovoltaics Polarized light self-powered photodetection |
| Title | Chiral Lead‐Free Hybrid Perovskites for Self‐Powered Circularly Polarized Light Detection |
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