Phosphorene Co‐catalyst Advancing Highly Efficient Visible‐Light Photocatalytic Hydrogen Production
Transitional metals are widely used as co‐catalysts boosting photocatalytic H2 production. However, metal‐based co‐catalysts suffer from high cost, limited abundance and detrimental environment impact. To date, metal‐free co‐catalyst is rarely reported. Here we for the first time utilized density fu...
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| Published in | Angewandte Chemie International Edition Vol. 56; no. 35; pp. 10373 - 10377 |
|---|---|
| Main Authors | , , |
| Format | Journal Article |
| Language | English |
| Published |
Germany
Wiley Subscription Services, Inc
21.08.2017
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| Edition | International ed. in English |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Transitional metals are widely used as co‐catalysts boosting photocatalytic H2 production. However, metal‐based co‐catalysts suffer from high cost, limited abundance and detrimental environment impact. To date, metal‐free co‐catalyst is rarely reported. Here we for the first time utilized density functional calculations to guide the application of phosphorene as a high‐efficiency metal‐free co‐catalyst for CdS, Zn0.8Cd0.2S or ZnS. Particularly, phosphorene modified CdS shows a high apparent quantum yield of 34.7 % at 420 nm. This outstanding activity arises from the strong electronic coupling between phosphorene and CdS, as well as the favorable band structure, high charge mobility and massive active sites of phosphorene, supported by computations and advanced characterizations, for example, synchrotron‐based X‐ray absorption near edge spectroscopy. This work brings new opportunities to prepare highly‐active, cheap and green photocatalysts.
Density functional calculations were used to direct the design of phosphorene as a metal‐free co‐catalyst promoting photocatalytic H2 production in metal sulfide photocatalyst systems. The enhanced photocatalytic performance arises from the pronounced electronic coupling between metal sulfides and phosphorene, together with its advantageous band structure and excellent charge carrier mobility. |
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| AbstractList | Transitional metals are widely used as co-catalysts boosting photocatalytic H
production. However, metal-based co-catalysts suffer from high cost, limited abundance and detrimental environment impact. To date, metal-free co-catalyst is rarely reported. Here we for the first time utilized density functional calculations to guide the application of phosphorene as a high-efficiency metal-free co-catalyst for CdS, Zn
Cd
S or ZnS. Particularly, phosphorene modified CdS shows a high apparent quantum yield of 34.7 % at 420 nm. This outstanding activity arises from the strong electronic coupling between phosphorene and CdS, as well as the favorable band structure, high charge mobility and massive active sites of phosphorene, supported by computations and advanced characterizations, for example, synchrotron-based X-ray absorption near edge spectroscopy. This work brings new opportunities to prepare highly-active, cheap and green photocatalysts. Transitional metals are widely used as co‐catalysts boosting photocatalytic H 2 production. However, metal‐based co‐catalysts suffer from high cost, limited abundance and detrimental environment impact. To date, metal‐free co‐catalyst is rarely reported. Here we for the first time utilized density functional calculations to guide the application of phosphorene as a high‐efficiency metal‐free co‐catalyst for CdS, Zn 0.8 Cd 0.2 S or ZnS. Particularly, phosphorene modified CdS shows a high apparent quantum yield of 34.7 % at 420 nm. This outstanding activity arises from the strong electronic coupling between phosphorene and CdS, as well as the favorable band structure, high charge mobility and massive active sites of phosphorene, supported by computations and advanced characterizations, for example, synchrotron‐based X‐ray absorption near edge spectroscopy. This work brings new opportunities to prepare highly‐active, cheap and green photocatalysts. Transitional metals are widely used as co‐catalysts boosting photocatalytic H2 production. However, metal‐based co‐catalysts suffer from high cost, limited abundance and detrimental environment impact. To date, metal‐free co‐catalyst is rarely reported. Here we for the first time utilized density functional calculations to guide the application of phosphorene as a high‐efficiency metal‐free co‐catalyst for CdS, Zn0.8Cd0.2S or ZnS. Particularly, phosphorene modified CdS shows a high apparent quantum yield of 34.7 % at 420 nm. This outstanding activity arises from the strong electronic coupling between phosphorene and CdS, as well as the favorable band structure, high charge mobility and massive active sites of phosphorene, supported by computations and advanced characterizations, for example, synchrotron‐based X‐ray absorption near edge spectroscopy. This work brings new opportunities to prepare highly‐active, cheap and green photocatalysts. Density functional calculations were used to direct the design of phosphorene as a metal‐free co‐catalyst promoting photocatalytic H2 production in metal sulfide photocatalyst systems. The enhanced photocatalytic performance arises from the pronounced electronic coupling between metal sulfides and phosphorene, together with its advantageous band structure and excellent charge carrier mobility. Transitional metals are widely used as co-catalysts boosting photocatalytic H2 production. However, metal-based co-catalysts suffer from high cost, limited abundance and detrimental environment impact. To date, metal-free co-catalyst is rarely reported. Here we for the first time utilized density functional calculations to guide the application of phosphorene as a high-efficiency metal-free co-catalyst for CdS, Zn0.8Cd0.2S or ZnS. Particularly, phosphorene modified CdS shows a high apparent quantum yield of 34.7% at 420nm. This outstanding activity arises from the strong electronic coupling between phosphorene and CdS, as well as the favorable band structure, high charge mobility and massive active sites of phosphorene, supported by computations and advanced characterizations, for example, synchrotron-based X-ray absorption near edge spectroscopy. This work brings new opportunities to prepare highly-active, cheap and green photocatalysts. Transitional metals are widely used as co-catalysts boosting photocatalytic H2 production. However, metal-based co-catalysts suffer from high cost, limited abundance and detrimental environment impact. To date, metal-free co-catalyst is rarely reported. Here we for the first time utilized density functional calculations to guide the application of phosphorene as a high-efficiency metal-free co-catalyst for CdS, Zn0.8 Cd0.2 S or ZnS. Particularly, phosphorene modified CdS shows a high apparent quantum yield of 34.7 % at 420 nm. This outstanding activity arises from the strong electronic coupling between phosphorene and CdS, as well as the favorable band structure, high charge mobility and massive active sites of phosphorene, supported by computations and advanced characterizations, for example, synchrotron-based X-ray absorption near edge spectroscopy. This work brings new opportunities to prepare highly-active, cheap and green photocatalysts.Transitional metals are widely used as co-catalysts boosting photocatalytic H2 production. However, metal-based co-catalysts suffer from high cost, limited abundance and detrimental environment impact. To date, metal-free co-catalyst is rarely reported. Here we for the first time utilized density functional calculations to guide the application of phosphorene as a high-efficiency metal-free co-catalyst for CdS, Zn0.8 Cd0.2 S or ZnS. Particularly, phosphorene modified CdS shows a high apparent quantum yield of 34.7 % at 420 nm. This outstanding activity arises from the strong electronic coupling between phosphorene and CdS, as well as the favorable band structure, high charge mobility and massive active sites of phosphorene, supported by computations and advanced characterizations, for example, synchrotron-based X-ray absorption near edge spectroscopy. This work brings new opportunities to prepare highly-active, cheap and green photocatalysts. |
| Author | Zhu, Bicheng Qiao, Shi‐Zhang Ran, Jingrun |
| Author_xml | – sequence: 1 givenname: Jingrun surname: Ran fullname: Ran, Jingrun organization: University of Adelaide – sequence: 2 givenname: Bicheng surname: Zhu fullname: Zhu, Bicheng organization: Wuhan University of Technology – sequence: 3 givenname: Shi‐Zhang orcidid: 0000-0002-4568-8422 surname: Qiao fullname: Qiao, Shi‐Zhang email: s.qiao@adelaide.edu.au organization: University of Adelaide |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/28670856$$D View this record in MEDLINE/PubMed |
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| Snippet | Transitional metals are widely used as co‐catalysts boosting photocatalytic H2 production. However, metal‐based co‐catalysts suffer from high cost, limited... Transitional metals are widely used as co‐catalysts boosting photocatalytic H 2 production. However, metal‐based co‐catalysts suffer from high cost, limited... Transitional metals are widely used as co-catalysts boosting photocatalytic H production. However, metal-based co-catalysts suffer from high cost, limited... Transitional metals are widely used as co-catalysts boosting photocatalytic H2 production. However, metal-based co-catalysts suffer from high cost, limited... |
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| SubjectTerms | Abundance Band structure of solids Catalysts co-catalysts density functional calculations Environmental impact Hydrogen production Metals Phosphorene Photocatalysis Spectroscopy Zinc sulfide |
| Title | Phosphorene Co‐catalyst Advancing Highly Efficient Visible‐Light Photocatalytic Hydrogen Production |
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