Exploring the Performance Improvement of the Oxygen Evolution Reaction in a Stable Bimetal–Organic Framework System
Despite wide applications of bimetallic electrocatalysis in oxygen evolution reaction (OER) owing to their superior performance, the origin of the improved performance remains elusive. The underlying mechanism was explored by designing and synthesizing a series of stable metal–organic frameworks (MO...
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| Published in | Angewandte Chemie International Edition Vol. 57; no. 31; pp. 9660 - 9664 |
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| Main Authors | , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Germany
Wiley Subscription Services, Inc
26.07.2018
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| Edition | International ed. in English |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Despite wide applications of bimetallic electrocatalysis in oxygen evolution reaction (OER) owing to their superior performance, the origin of the improved performance remains elusive. The underlying mechanism was explored by designing and synthesizing a series of stable metal–organic frameworks (MOFs: NNU‐21–24) based on trinuclear metal carboxylate clusters and tridentate carboxylate ligands. Among the examined stable MOFs, NNU‐23 exhibits the best OER performance; particularly, compared with monometallic MOFs, all the bimetallic MOFs display improved OER activity. DFT calculations and experimental results demonstrate that introduction of the second metal atom can improve the activity of the original atom. The proposed model of bimetallic electrocatalysts affecting their OER performance can facilitate design of efficient bimetallic catalysts for energy storage and conversion, and investigation of the related catalytic mechanisms.
An iron atom in an Fe3 cluster is replaced by a second metal to form Fe2M clusters, which can serve as nodes to bridge with organic ligands and construct stable bimetallic MOFs. The introduction of the second metal atom can improve the activity of the original atom and thus improve the oxygen evolution reaction performance of electrocatalysts. |
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| AbstractList | Despite wide applications of bimetallic electrocatalysis in oxygen evolution reaction (OER) owing to their superior performance, the origin of the improved performance remains elusive. The underlying mechanism was explored by designing and synthesizing a series of stable metal–organic frameworks (MOFs: NNU‐21–24) based on trinuclear metal carboxylate clusters and tridentate carboxylate ligands. Among the examined stable MOFs, NNU‐23 exhibits the best OER performance; particularly, compared with monometallic MOFs, all the bimetallic MOFs display improved OER activity. DFT calculations and experimental results demonstrate that introduction of the second metal atom can improve the activity of the original atom. The proposed model of bimetallic electrocatalysts affecting their OER performance can facilitate design of efficient bimetallic catalysts for energy storage and conversion, and investigation of the related catalytic mechanisms.
An iron atom in an Fe3 cluster is replaced by a second metal to form Fe2M clusters, which can serve as nodes to bridge with organic ligands and construct stable bimetallic MOFs. The introduction of the second metal atom can improve the activity of the original atom and thus improve the oxygen evolution reaction performance of electrocatalysts. Despite wide applications of bimetallic electrocatalysis in oxygen evolution reaction (OER) owing to their superior performance, the origin of the improved performance remains elusive. The underlying mechanism was explored by designing and synthesizing a series of stable metal–organic frameworks (MOFs: NNU‐21–24 ) based on trinuclear metal carboxylate clusters and tridentate carboxylate ligands. Among the examined stable MOFs, NNU‐23 exhibits the best OER performance; particularly, compared with monometallic MOFs, all the bimetallic MOFs display improved OER activity. DFT calculations and experimental results demonstrate that introduction of the second metal atom can improve the activity of the original atom. The proposed model of bimetallic electrocatalysts affecting their OER performance can facilitate design of efficient bimetallic catalysts for energy storage and conversion, and investigation of the related catalytic mechanisms. Despite wide applications of bimetallic electrocatalysis in oxygen evolution reaction (OER) owing to their superior performance, the origin of the improved performance remains elusive. The underlying mechanism was explored by designing and synthesizing a series of stable metal-organic frameworks (MOFs: NNU-21-24) based on trinuclear metal carboxylate clusters and tridentate carboxylate ligands. Among the examined stable MOFs, NNU-23 exhibits the best OER performance; particularly, compared with monometallic MOFs, all the bimetallic MOFs display improved OER activity. DFT calculations and experimental results demonstrate that introduction of the second metal atom can improve the activity of the original atom. The proposed model of bimetallic electrocatalysts affecting their OER performance can facilitate design of efficient bimetallic catalysts for energy storage and conversion, and investigation of the related catalytic mechanisms. Despite wide applications of bimetallic electrocatalysis in oxygen evolution reaction (OER) owing to their superior performance, the origin of the improved performance remains elusive. The underlying mechanism was explored by designing and synthesizing a series of stable metal-organic frameworks (MOFs: NNU-21-24) based on trinuclear metal carboxylate clusters and tridentate carboxylate ligands. Among the examined stable MOFs, NNU-23 exhibits the best OER performance; particularly, compared with monometallic MOFs, all the bimetallic MOFs display improved OER activity. DFT calculations and experimental results demonstrate that introduction of the second metal atom can improve the activity of the original atom. The proposed model of bimetallic electrocatalysts affecting their OER performance can facilitate design of efficient bimetallic catalysts for energy storage and conversion, and investigation of the related catalytic mechanisms.Despite wide applications of bimetallic electrocatalysis in oxygen evolution reaction (OER) owing to their superior performance, the origin of the improved performance remains elusive. The underlying mechanism was explored by designing and synthesizing a series of stable metal-organic frameworks (MOFs: NNU-21-24) based on trinuclear metal carboxylate clusters and tridentate carboxylate ligands. Among the examined stable MOFs, NNU-23 exhibits the best OER performance; particularly, compared with monometallic MOFs, all the bimetallic MOFs display improved OER activity. DFT calculations and experimental results demonstrate that introduction of the second metal atom can improve the activity of the original atom. The proposed model of bimetallic electrocatalysts affecting their OER performance can facilitate design of efficient bimetallic catalysts for energy storage and conversion, and investigation of the related catalytic mechanisms. |
| Author | Tang, Yu‐Jia Wang, Xiao‐Li Qiao, Man Lan, Ya‐Qian Liu, Jiang Dong, Long‐Zhang Li, Shun‐Li Li, Yafei Su, Jia‐Xin |
| Author_xml | – sequence: 1 givenname: Xiao‐Li surname: Wang fullname: Wang, Xiao‐Li organization: Nanjing Normal University – sequence: 2 givenname: Long‐Zhang surname: Dong fullname: Dong, Long‐Zhang organization: Nanjing Normal University – sequence: 3 givenname: Man surname: Qiao fullname: Qiao, Man organization: Nanjing Normal University – sequence: 4 givenname: Yu‐Jia surname: Tang fullname: Tang, Yu‐Jia organization: Nanjing Normal University – sequence: 5 givenname: Jiang surname: Liu fullname: Liu, Jiang organization: Nanjing Normal University – sequence: 6 givenname: Yafei surname: Li fullname: Li, Yafei email: liyafei.abc@gmail.com organization: Nanjing Normal University – sequence: 7 givenname: Shun‐Li surname: Li fullname: Li, Shun‐Li organization: Nanjing Normal University – sequence: 8 givenname: Jia‐Xin surname: Su fullname: Su, Jia‐Xin organization: Nanjing Normal University – sequence: 9 givenname: Ya‐Qian orcidid: 0000-0002-2140-7980 surname: Lan fullname: Lan, Ya‐Qian email: yqlan@njnu.edu.cn organization: Nanjing Normal University |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/29660248$$D View this record in MEDLINE/PubMed |
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| SubjectTerms | bimetallic electrocatalysts Bimetals Catalysts Catalytic converters clusters Electrocatalysts Energy storage iron Metal-organic frameworks Oxygen oxygen evolution reaction Oxygen evolution reactions |
| Title | Exploring the Performance Improvement of the Oxygen Evolution Reaction in a Stable Bimetal–Organic Framework System |
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