Zirconium–Porphyrin‐Based Metal–Organic Framework Hollow Nanotubes for Immobilization of Noble‐Metal Single Atoms
Single atoms immobilized on metal–organic frameworks (MOFs) with unique nanostructures have drawn tremendous attention in the application of catalysis but remain a great challenge. Various single noble‐metal atoms have now been successfully anchored on the well‐defined anchoring sites of the zirconi...
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| Published in | Angewandte Chemie International Edition Vol. 57; no. 13; pp. 3493 - 3498 |
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| Main Authors | , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Germany
Wiley Subscription Services, Inc
19.03.2018
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| Edition | International ed. in English |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Single atoms immobilized on metal–organic frameworks (MOFs) with unique nanostructures have drawn tremendous attention in the application of catalysis but remain a great challenge. Various single noble‐metal atoms have now been successfully anchored on the well‐defined anchoring sites of the zirconium porphyrin MOF hollow nanotubes, which are probed by aberration‐corrected scanning transmission electron microscopy and synchrotron‐radiation‐based X‐ray absorption fine‐structure spectroscopy. Owing to the hollow structure and excellent photoelectrochemical performance, the HNTM‐Ir/Pt exhibits outstanding catalytic activity in the visible‐light photocatalytic H2 evolution via water splitting. The single atom immobilized on MOFs with hollow structures are expected to pave the way to expand the potential applications of MOFs.
Single noble metal atoms can be successfully immobilized on the well‐defined anchoring sites of zirconium–porphyrin MOF hollow nanotubes. Owing to the hollow structure and excellent photoelectrochemical performance, HNTM‐Ir/Pt exhibits outstanding catalytic activity in the visible‐light photocatalytic H2 evolution via water splitting. |
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| AbstractList | Single atoms immobilized on metal–organic frameworks (MOFs) with unique nanostructures have drawn tremendous attention in the application of catalysis but remain a great challenge. Various single noble‐metal atoms have now been successfully anchored on the well‐defined anchoring sites of the zirconium porphyrin MOF hollow nanotubes, which are probed by aberration‐corrected scanning transmission electron microscopy and synchrotron‐radiation‐based X‐ray absorption fine‐structure spectroscopy. Owing to the hollow structure and excellent photoelectrochemical performance, the HNTM‐Ir/Pt exhibits outstanding catalytic activity in the visible‐light photocatalytic H2 evolution via water splitting. The single atom immobilized on MOFs with hollow structures are expected to pave the way to expand the potential applications of MOFs.
Single noble metal atoms can be successfully immobilized on the well‐defined anchoring sites of zirconium–porphyrin MOF hollow nanotubes. Owing to the hollow structure and excellent photoelectrochemical performance, HNTM‐Ir/Pt exhibits outstanding catalytic activity in the visible‐light photocatalytic H2 evolution via water splitting. Single atoms immobilized on metal–organic frameworks (MOFs) with unique nanostructures have drawn tremendous attention in the application of catalysis but remain a great challenge. Various single noble‐metal atoms have now been successfully anchored on the well‐defined anchoring sites of the zirconium porphyrin MOF hollow nanotubes, which are probed by aberration‐corrected scanning transmission electron microscopy and synchrotron‐radiation‐based X‐ray absorption fine‐structure spectroscopy. Owing to the hollow structure and excellent photoelectrochemical performance, the HNTM‐Ir/Pt exhibits outstanding catalytic activity in the visible‐light photocatalytic H2 evolution via water splitting. The single atom immobilized on MOFs with hollow structures are expected to pave the way to expand the potential applications of MOFs. Single atoms immobilized on metal-organic frameworks (MOFs) with unique nanostructures have drawn tremendous attention in the application of catalysis but remain a great challenge. Various single noble-metal atoms have now been successfully anchored on the well-defined anchoring sites of the zirconium porphyrin MOF hollow nanotubes, which are probed by aberration-corrected scanning transmission electron microscopy and synchrotron-radiation-based X-ray absorption fine-structure spectroscopy. Owing to the hollow structure and excellent photoelectrochemical performance, the HNTM-Ir/Pt exhibits outstanding catalytic activity in the visible-light photocatalytic H evolution via water splitting. The single atom immobilized on MOFs with hollow structures are expected to pave the way to expand the potential applications of MOFs. Single atoms immobilized on metal–organic frameworks (MOFs) with unique nanostructures have drawn tremendous attention in the application of catalysis but remain a great challenge. Various single noble‐metal atoms have now been successfully anchored on the well‐defined anchoring sites of the zirconium porphyrin MOF hollow nanotubes, which are probed by aberration‐corrected scanning transmission electron microscopy and synchrotron‐radiation‐based X‐ray absorption fine‐structure spectroscopy. Owing to the hollow structure and excellent photoelectrochemical performance, the HNTM‐Ir/Pt exhibits outstanding catalytic activity in the visible‐light photocatalytic H 2 evolution via water splitting. The single atom immobilized on MOFs with hollow structures are expected to pave the way to expand the potential applications of MOFs. Single atoms immobilized on metal-organic frameworks (MOFs) with unique nanostructures have drawn tremendous attention in the application of catalysis but remain a great challenge. Various single noble-metal atoms have now been successfully anchored on the well-defined anchoring sites of the zirconium porphyrin MOF hollow nanotubes, which are probed by aberration-corrected scanning transmission electron microscopy and synchrotron-radiation-based X-ray absorption fine-structure spectroscopy. Owing to the hollow structure and excellent photoelectrochemical performance, the HNTM-Ir/Pt exhibits outstanding catalytic activity in the visible-light photocatalytic H2 evolution via water splitting. The single atom immobilized on MOFs with hollow structures are expected to pave the way to expand the potential applications of MOFs.Single atoms immobilized on metal-organic frameworks (MOFs) with unique nanostructures have drawn tremendous attention in the application of catalysis but remain a great challenge. Various single noble-metal atoms have now been successfully anchored on the well-defined anchoring sites of the zirconium porphyrin MOF hollow nanotubes, which are probed by aberration-corrected scanning transmission electron microscopy and synchrotron-radiation-based X-ray absorption fine-structure spectroscopy. Owing to the hollow structure and excellent photoelectrochemical performance, the HNTM-Ir/Pt exhibits outstanding catalytic activity in the visible-light photocatalytic H2 evolution via water splitting. The single atom immobilized on MOFs with hollow structures are expected to pave the way to expand the potential applications of MOFs. |
| Author | Gu, Lin Chen, Shuangming Hu, Wenping He, Ting Wang, Xun Song, Li Gong, Yue Ni, Bing Wu, Zhao |
| Author_xml | – sequence: 1 givenname: Ting surname: He fullname: He, Ting organization: Qinghai Normal University – sequence: 2 givenname: Shuangming surname: Chen fullname: Chen, Shuangming organization: University of Science and Technology of China – sequence: 3 givenname: Bing surname: Ni fullname: Ni, Bing organization: Tsinghua University – sequence: 4 givenname: Yue surname: Gong fullname: Gong, Yue organization: Chinese Academy of Sciences – sequence: 5 givenname: Zhao surname: Wu fullname: Wu, Zhao organization: University of Science and Technology of China – sequence: 6 givenname: Li surname: Song fullname: Song, Li organization: University of Science and Technology of China – sequence: 7 givenname: Lin surname: Gu fullname: Gu, Lin organization: Chinese Academy of Sciences – sequence: 8 givenname: Wenping surname: Hu fullname: Hu, Wenping organization: Tianjin University & Collaborative Innovation Center of Chemical Science and Engineering (Tianjin) – sequence: 9 givenname: Xun orcidid: 0000-0002-8066-4450 surname: Wang fullname: Wang, Xun email: wangxun@mail.tsinghua.edu.cn organization: Tsinghua University |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/29380509$$D View this record in MEDLINE/PubMed |
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| Keywords | hollow nanotubes hydrogen evolution photocatalysis zirconium metal-organic frameworks |
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| Snippet | Single atoms immobilized on metal–organic frameworks (MOFs) with unique nanostructures have drawn tremendous attention in the application of catalysis but... Single atoms immobilized on metal-organic frameworks (MOFs) with unique nanostructures have drawn tremendous attention in the application of catalysis but... |
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| SubjectTerms | Anchoring Catalysis Catalytic activity hollow nanotubes hydrogen evolution Immobilization Metal-organic frameworks Metals Nanotechnology Nanotubes photocatalysis Platinum Scanning transmission electron microscopy Spectroscopy Transmission electron microscopy Water splitting X-rays Zirconium |
| Title | Zirconium–Porphyrin‐Based Metal–Organic Framework Hollow Nanotubes for Immobilization of Noble‐Metal Single Atoms |
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