Rational Design of Multicolor‐Emitting Chiral Carbonized Polymer Dots for Full‐Color and White Circularly Polarized Luminescence
Light‐emitting chiral carbonized polymer dots (Ch‐CPDs) are attracting great interest because of their extraordinary photonic properties, but modulating their band‐gap emission, especially at long wavelength, and maintaining their chiral structure to achieve multicolor, high‐emission Ch‐CPDs remains...
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| Published in | Angewandte Chemie International Edition Vol. 60; no. 25; pp. 14091 - 14099 |
|---|---|
| Main Authors | , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Germany
Wiley Subscription Services, Inc
14.06.2021
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| Edition | International ed. in English |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Light‐emitting chiral carbonized polymer dots (Ch‐CPDs) are attracting great interest because of their extraordinary photonic properties, but modulating their band‐gap emission, especially at long wavelength, and maintaining their chiral structure to achieve multicolor, high‐emission Ch‐CPDs remains challenging. Reported here for the first time is the synthesis of red‐ and multicolor‐emitting Ch‐CPDs using the common precursors L‐/D‐tryptophan and o‐phenylenediamine, and a solvothermal approach at one temperature. The quantum yield of the Ch‐CPDs was between 31 % and 54 %. Supramolecular self‐assembly provided multicolor‐emitting Ch‐CPDs showing novel circularly polarized luminescence, with the highest dissymmetric factor (glum) of 1×10−2. Importantly, circularly polarized white‐emitting CPDs were fabricated for the first time by tuning the mixing ratio of the three colored Ch‐CPDs in a gel. This strategy affords exciting opportunities for designing functional chiroptical materials.
The synthesis of red‐ and multicolor‐emitting chiral carbonized polymer dots (Ch‐CPDs) is reported for the first time. The quantum yield of the Ch‐CPDs is between 31 % and 54 %. Furthermore, these Ch‐CPDs were combined with chiral gels through supramolecular self‐assembly, thereby yielding their multicolor and white circularly polarized luminescence. |
|---|---|
| AbstractList | Light‐emitting chiral carbonized polymer dots (Ch‐CPDs) are attracting great interest because of their extraordinary photonic properties, but modulating their band‐gap emission, especially at long wavelength, and maintaining their chiral structure to achieve multicolor, high‐emission Ch‐CPDs remains challenging. Reported here for the first time is the synthesis of red‐ and multicolor‐emitting Ch‐CPDs using the common precursors L‐/D‐tryptophan and o‐phenylenediamine, and a solvothermal approach at one temperature. The quantum yield of the Ch‐CPDs was between 31 % and 54 %. Supramolecular self‐assembly provided multicolor‐emitting Ch‐CPDs showing novel circularly polarized luminescence, with the highest dissymmetric factor (glum) of 1×10−2. Importantly, circularly polarized white‐emitting CPDs were fabricated for the first time by tuning the mixing ratio of the three colored Ch‐CPDs in a gel. This strategy affords exciting opportunities for designing functional chiroptical materials. Light‐emitting chiral carbonized polymer dots (Ch‐CPDs) are attracting great interest because of their extraordinary photonic properties, but modulating their band‐gap emission, especially at long wavelength, and maintaining their chiral structure to achieve multicolor, high‐emission Ch‐CPDs remains challenging. Reported here for the first time is the synthesis of red‐ and multicolor‐emitting Ch‐CPDs using the common precursors L‐/D‐tryptophan and o‐phenylenediamine, and a solvothermal approach at one temperature. The quantum yield of the Ch‐CPDs was between 31 % and 54 %. Supramolecular self‐assembly provided multicolor‐emitting Ch‐CPDs showing novel circularly polarized luminescence, with the highest dissymmetric factor (glum) of 1×10−2. Importantly, circularly polarized white‐emitting CPDs were fabricated for the first time by tuning the mixing ratio of the three colored Ch‐CPDs in a gel. This strategy affords exciting opportunities for designing functional chiroptical materials. The synthesis of red‐ and multicolor‐emitting chiral carbonized polymer dots (Ch‐CPDs) is reported for the first time. The quantum yield of the Ch‐CPDs is between 31 % and 54 %. Furthermore, these Ch‐CPDs were combined with chiral gels through supramolecular self‐assembly, thereby yielding their multicolor and white circularly polarized luminescence. Light‐emitting chiral carbonized polymer dots (Ch‐CPDs) are attracting great interest because of their extraordinary photonic properties, but modulating their band‐gap emission, especially at long wavelength, and maintaining their chiral structure to achieve multicolor, high‐emission Ch‐CPDs remains challenging. Reported here for the first time is the synthesis of red‐ and multicolor‐emitting Ch‐CPDs using the common precursors L ‐/ D ‐tryptophan and o ‐phenylenediamine, and a solvothermal approach at one temperature. The quantum yield of the Ch‐CPDs was between 31 % and 54 %. Supramolecular self‐assembly provided multicolor‐emitting Ch‐CPDs showing novel circularly polarized luminescence, with the highest dissymmetric factor (g lum ) of 1×10 −2 . Importantly, circularly polarized white‐emitting CPDs were fabricated for the first time by tuning the mixing ratio of the three colored Ch‐CPDs in a gel. This strategy affords exciting opportunities for designing functional chiroptical materials. Light-emitting chiral carbonized polymer dots (Ch-CPDs) are attracting great interest because of their extraordinary photonic properties, but modulating their band-gap emission, especially at long wavelength, and maintaining their chiral structure to achieve multicolor, high-emission Ch-CPDs remains challenging. Reported here for the first time is the synthesis of red- and multicolor-emitting Ch-CPDs using the common precursors L-/D-tryptophan and o-phenylenediamine, and a solvothermal approach at one temperature. The quantum yield of the Ch-CPDs was between 31 % and 54 %. Supramolecular self-assembly provided multicolor-emitting Ch-CPDs showing novel circularly polarized luminescence, with the highest dissymmetric factor (g ) of 1×10 . Importantly, circularly polarized white-emitting CPDs were fabricated for the first time by tuning the mixing ratio of the three colored Ch-CPDs in a gel. This strategy affords exciting opportunities for designing functional chiroptical materials. Light-emitting chiral carbonized polymer dots (Ch-CPDs) are attracting great interest because of their extraordinary photonic properties, but modulating their band-gap emission, especially at long wavelength, and maintaining their chiral structure to achieve multicolor, high-emission Ch-CPDs remains challenging. Reported here for the first time is the synthesis of red- and multicolor-emitting Ch-CPDs using the common precursors L-/D-tryptophan and o-phenylenediamine, and a solvothermal approach at one temperature. The quantum yield of the Ch-CPDs was between 31 % and 54 %. Supramolecular self-assembly provided multicolor-emitting Ch-CPDs showing novel circularly polarized luminescence, with the highest dissymmetric factor (glum ) of 1×10-2 . Importantly, circularly polarized white-emitting CPDs were fabricated for the first time by tuning the mixing ratio of the three colored Ch-CPDs in a gel. This strategy affords exciting opportunities for designing functional chiroptical materials.Light-emitting chiral carbonized polymer dots (Ch-CPDs) are attracting great interest because of their extraordinary photonic properties, but modulating their band-gap emission, especially at long wavelength, and maintaining their chiral structure to achieve multicolor, high-emission Ch-CPDs remains challenging. Reported here for the first time is the synthesis of red- and multicolor-emitting Ch-CPDs using the common precursors L-/D-tryptophan and o-phenylenediamine, and a solvothermal approach at one temperature. The quantum yield of the Ch-CPDs was between 31 % and 54 %. Supramolecular self-assembly provided multicolor-emitting Ch-CPDs showing novel circularly polarized luminescence, with the highest dissymmetric factor (glum ) of 1×10-2 . Importantly, circularly polarized white-emitting CPDs were fabricated for the first time by tuning the mixing ratio of the three colored Ch-CPDs in a gel. This strategy affords exciting opportunities for designing functional chiroptical materials. |
| Author | Tang, Zhiyong Ru, Yi Song, Haoqiang Liu, Xingjiang Zang, Shuang‐Quan Yang, Bai Sui, Laizhi Lu, Siyu |
| Author_xml | – sequence: 1 givenname: Yi surname: Ru fullname: Ru, Yi organization: Zhengzhou University – sequence: 2 givenname: Laizhi surname: Sui fullname: Sui, Laizhi organization: Chinese Academy of Sciences – sequence: 3 givenname: Haoqiang surname: Song fullname: Song, Haoqiang organization: Zhengzhou University – sequence: 4 givenname: Xingjiang surname: Liu fullname: Liu, Xingjiang organization: Zhengzhou University – sequence: 5 givenname: Zhiyong surname: Tang fullname: Tang, Zhiyong organization: National Center for Nanoscience and Technology – sequence: 6 givenname: Shuang‐Quan surname: Zang fullname: Zang, Shuang‐Quan organization: Zhengzhou University – sequence: 7 givenname: Bai surname: Yang fullname: Yang, Bai organization: Jilin University – sequence: 8 givenname: Siyu orcidid: 0000-0003-4538-7846 surname: Lu fullname: Lu, Siyu email: sylu2013@zzu.edu.cn organization: Zhengzhou University |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/33830583$$D View this record in MEDLINE/PubMed |
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| Copyright | 2021 Wiley‐VCH GmbH 2021 Wiley-VCH GmbH. |
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| Snippet | Light‐emitting chiral carbonized polymer dots (Ch‐CPDs) are attracting great interest because of their extraordinary photonic properties, but modulating their... Light-emitting chiral carbonized polymer dots (Ch-CPDs) are attracting great interest because of their extraordinary photonic properties, but modulating their... |
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| SubjectTerms | carbonized polymer dots chirality Circular polarization Emission Emissions Luminescence Mixing ratio nanomaterials Phenylenediamine Polymers self-assembly Tryptophan |
| Title | Rational Design of Multicolor‐Emitting Chiral Carbonized Polymer Dots for Full‐Color and White Circularly Polarized Luminescence |
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