Single Tungsten Atoms Supported on MOF‐Derived N‐Doped Carbon for Robust Electrochemical Hydrogen Evolution
Tungsten‐based catalysts are promising candidates to generate hydrogen effectively. In this work, a single‐W‐atom catalyst supported on metal–organic framework (MOF)‐derived N‐doped carbon (W‐SAC) for efficient electrochemical hydrogen evolution reaction (HER), with high activity and excellent stabi...
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| Published in | Advanced materials (Weinheim) Vol. 30; no. 30; pp. e1800396 - n/a |
|---|---|
| Main Authors | , , , , , , , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Germany
Wiley Subscription Services, Inc
26.07.2018
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Tungsten‐based catalysts are promising candidates to generate hydrogen effectively. In this work, a single‐W‐atom catalyst supported on metal–organic framework (MOF)‐derived N‐doped carbon (W‐SAC) for efficient electrochemical hydrogen evolution reaction (HER), with high activity and excellent stability is reported. High‐angle annular dark‐field scanning transmission electron microscopy (HAADF‐STEM) and X‐ray absorption fine structure (XAFS) spectroscopy analysis indicate the atomic dispersion of the W species, and reveal that the W1N1C3 moiety may be the favored local structure for the W species. The W‐SAC exhibits a low overpotential of 85 mV at a current density of 10 mA cm−2 and a small Tafel slope of 53 mV dec−1, in 0.1 m KOH solution. The HER activity of the W‐SAC is almost equal to that of commercial Pt/C. Density functional theory (DFT) calculation suggests that the unique structure of the W1N1C3 moiety plays an important role in enhancing the HER performance. This work gives new insights into the investigation of efficient and practical W‐based HER catalysts.
A single‐tungsten‐atom catalyst supported on metal–organic framework‐derived N‐doped carbon is reported. The catalyst demonstrates a high activity and excellent stability for efficient electrochemical hydrogen evolution. |
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| AbstractList | Tungsten‐based catalysts are promising candidates to generate hydrogen effectively. In this work, a single‐W‐atom catalyst supported on metal–organic framework (MOF)‐derived N‐doped carbon (W‐SAC) for efficient electrochemical hydrogen evolution reaction (HER), with high activity and excellent stability is reported. High‐angle annular dark‐field scanning transmission electron microscopy (HAADF‐STEM) and X‐ray absorption fine structure (XAFS) spectroscopy analysis indicate the atomic dispersion of the W species, and reveal that the W
1
N
1
C
3
moiety may be the favored local structure for the W species. The W‐SAC exhibits a low overpotential of 85 mV at a current density of 10 mA cm
−2
and a small Tafel slope of 53 mV dec
−1
, in 0.1
m
KOH solution. The HER activity of the W‐SAC is almost equal to that of commercial Pt/C. Density functional theory (DFT) calculation suggests that the unique structure of the W
1
N
1
C
3
moiety plays an important role in enhancing the HER performance. This work gives new insights into the investigation of efficient and practical W‐based HER catalysts. Tungsten‐based catalysts are promising candidates to generate hydrogen effectively. In this work, a single‐W‐atom catalyst supported on metal–organic framework (MOF)‐derived N‐doped carbon (W‐SAC) for efficient electrochemical hydrogen evolution reaction (HER), with high activity and excellent stability is reported. High‐angle annular dark‐field scanning transmission electron microscopy (HAADF‐STEM) and X‐ray absorption fine structure (XAFS) spectroscopy analysis indicate the atomic dispersion of the W species, and reveal that the W1N1C3 moiety may be the favored local structure for the W species. The W‐SAC exhibits a low overpotential of 85 mV at a current density of 10 mA cm−2 and a small Tafel slope of 53 mV dec−1, in 0.1 m KOH solution. The HER activity of the W‐SAC is almost equal to that of commercial Pt/C. Density functional theory (DFT) calculation suggests that the unique structure of the W1N1C3 moiety plays an important role in enhancing the HER performance. This work gives new insights into the investigation of efficient and practical W‐based HER catalysts. A single‐tungsten‐atom catalyst supported on metal–organic framework‐derived N‐doped carbon is reported. The catalyst demonstrates a high activity and excellent stability for efficient electrochemical hydrogen evolution. Tungsten-based catalysts are promising candidates to generate hydrogen effectively. In this work, a single-W-atom catalyst supported on metal-organic framework (MOF)-derived N-doped carbon (W-SAC) for efficient electrochemical hydrogen evolution reaction (HER), with high activity and excellent stability is reported. High-angle annular dark-field scanning transmission electron microscopy (HAADF-STEM) and X-ray absorption fine structure (XAFS) spectroscopy analysis indicate the atomic dispersion of the W species, and reveal that the W N C moiety may be the favored local structure for the W species. The W-SAC exhibits a low overpotential of 85 mV at a current density of 10 mA cm and a small Tafel slope of 53 mV dec , in 0.1 m KOH solution. The HER activity of the W-SAC is almost equal to that of commercial Pt/C. Density functional theory (DFT) calculation suggests that the unique structure of the W N C moiety plays an important role in enhancing the HER performance. This work gives new insights into the investigation of efficient and practical W-based HER catalysts. Tungsten‐based catalysts are promising candidates to generate hydrogen effectively. In this work, a single‐W‐atom catalyst supported on metal–organic framework (MOF)‐derived N‐doped carbon (W‐SAC) for efficient electrochemical hydrogen evolution reaction (HER), with high activity and excellent stability is reported. High‐angle annular dark‐field scanning transmission electron microscopy (HAADF‐STEM) and X‐ray absorption fine structure (XAFS) spectroscopy analysis indicate the atomic dispersion of the W species, and reveal that the W1N1C3 moiety may be the favored local structure for the W species. The W‐SAC exhibits a low overpotential of 85 mV at a current density of 10 mA cm−2 and a small Tafel slope of 53 mV dec−1, in 0.1 m KOH solution. The HER activity of the W‐SAC is almost equal to that of commercial Pt/C. Density functional theory (DFT) calculation suggests that the unique structure of the W1N1C3 moiety plays an important role in enhancing the HER performance. This work gives new insights into the investigation of efficient and practical W‐based HER catalysts. Tungsten-based catalysts are promising candidates to generate hydrogen effectively. In this work, a single-W-atom catalyst supported on metal-organic framework (MOF)-derived N-doped carbon (W-SAC) for efficient electrochemical hydrogen evolution reaction (HER), with high activity and excellent stability is reported. High-angle annular dark-field scanning transmission electron microscopy (HAADF-STEM) and X-ray absorption fine structure (XAFS) spectroscopy analysis indicate the atomic dispersion of the W species, and reveal that the W1 N1 C3 moiety may be the favored local structure for the W species. The W-SAC exhibits a low overpotential of 85 mV at a current density of 10 mA cm-2 and a small Tafel slope of 53 mV dec-1 , in 0.1 m KOH solution. The HER activity of the W-SAC is almost equal to that of commercial Pt/C. Density functional theory (DFT) calculation suggests that the unique structure of the W1 N1 C3 moiety plays an important role in enhancing the HER performance. This work gives new insights into the investigation of efficient and practical W-based HER catalysts.Tungsten-based catalysts are promising candidates to generate hydrogen effectively. In this work, a single-W-atom catalyst supported on metal-organic framework (MOF)-derived N-doped carbon (W-SAC) for efficient electrochemical hydrogen evolution reaction (HER), with high activity and excellent stability is reported. High-angle annular dark-field scanning transmission electron microscopy (HAADF-STEM) and X-ray absorption fine structure (XAFS) spectroscopy analysis indicate the atomic dispersion of the W species, and reveal that the W1 N1 C3 moiety may be the favored local structure for the W species. The W-SAC exhibits a low overpotential of 85 mV at a current density of 10 mA cm-2 and a small Tafel slope of 53 mV dec-1 , in 0.1 m KOH solution. The HER activity of the W-SAC is almost equal to that of commercial Pt/C. Density functional theory (DFT) calculation suggests that the unique structure of the W1 N1 C3 moiety plays an important role in enhancing the HER performance. This work gives new insights into the investigation of efficient and practical W-based HER catalysts. |
| Author | Cheong, Weng‐Chon Li, Yadong Wang, Yu Yan, Wensheng Peng, Qing Wang, Dingsheng Chen, Wenxing Ren, Hanlin Wu, Konglin Chen, Chen Dong, Juncai He, Chun‐Ting Pei, Jiajing Wan, Jiawei Zhuang, Zhongbin Zheng, Xusheng Mao, Junjie |
| Author_xml | – sequence: 1 givenname: Wenxing surname: Chen fullname: Chen, Wenxing organization: Beijing Institute of Technology – sequence: 2 givenname: Jiajing surname: Pei fullname: Pei, Jiajing organization: Beijing University of Chemical Technology – sequence: 3 givenname: Chun‐Ting surname: He fullname: He, Chun‐Ting organization: Sun Yat‐Sen University – sequence: 4 givenname: Jiawei surname: Wan fullname: Wan, Jiawei organization: Tsinghua University – sequence: 5 givenname: Hanlin surname: Ren fullname: Ren, Hanlin organization: Tsinghua University – sequence: 6 givenname: Yu surname: Wang fullname: Wang, Yu organization: Chinese Academy of Sciences – sequence: 7 givenname: Juncai surname: Dong fullname: Dong, Juncai organization: Chinese Academy of Sciences – sequence: 8 givenname: Konglin surname: Wu fullname: Wu, Konglin organization: Tsinghua University – sequence: 9 givenname: Weng‐Chon surname: Cheong fullname: Cheong, Weng‐Chon organization: Tsinghua University – sequence: 10 givenname: Junjie surname: Mao fullname: Mao, Junjie organization: Tsinghua University – sequence: 11 givenname: Xusheng surname: Zheng fullname: Zheng, Xusheng organization: University of Science and Technology of China – sequence: 12 givenname: Wensheng surname: Yan fullname: Yan, Wensheng organization: University of Science and Technology of China – sequence: 13 givenname: Zhongbin surname: Zhuang fullname: Zhuang, Zhongbin organization: Beijing University of Chemical Technology – sequence: 14 givenname: Chen surname: Chen fullname: Chen, Chen organization: Tsinghua University – sequence: 15 givenname: Qing surname: Peng fullname: Peng, Qing organization: Tsinghua University – sequence: 16 givenname: Dingsheng orcidid: 0000-0003-0074-7633 surname: Wang fullname: Wang, Dingsheng email: wangdingsheng@mail.tsinghua.edu.cn organization: Tsinghua University – sequence: 17 givenname: Yadong surname: Li fullname: Li, Yadong organization: Tsinghua University |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/29888491$$D View this record in MEDLINE/PubMed |
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| Snippet | Tungsten‐based catalysts are promising candidates to generate hydrogen effectively. In this work, a single‐W‐atom catalyst supported on metal–organic framework... Tungsten-based catalysts are promising candidates to generate hydrogen effectively. In this work, a single-W-atom catalyst supported on metal-organic framework... |
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| SubjectTerms | Atomic absorption analysis Atomic structure Carbon Catalysis Catalysts Density functional theory electrocatalysts Fine structure hydrogen evolution reaction Hydrogen evolution reactions Metal-organic frameworks N‐doped carbon Scanning electron microscopy Scanning transmission electron microscopy single W atoms Transmission electron microscopy Tungsten |
| Title | Single Tungsten Atoms Supported on MOF‐Derived N‐Doped Carbon for Robust Electrochemical Hydrogen Evolution |
| URI | https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fadma.201800396 https://www.ncbi.nlm.nih.gov/pubmed/29888491 https://www.proquest.com/docview/2073260904 https://www.proquest.com/docview/2053270903 |
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