A Flexible Solid Electrolyte Interphase Layer for Long‐Life Lithium Metal Anodes
Lithium (Li) metal is a promising anode material for high‐energy density batteries. However, the unstable and static solid electrolyte interphase (SEI) can be destroyed by the dynamic Li plating/stripping behavior on the Li anode surface, leading to side reactions and Li dendrites growth. Herein, we...
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| Published in | Angewandte Chemie International Edition Vol. 57; no. 6; pp. 1505 - 1509 |
|---|---|
| Main Authors | , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Germany
Wiley Subscription Services, Inc
05.02.2018
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| Edition | International ed. in English |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Lithium (Li) metal is a promising anode material for high‐energy density batteries. However, the unstable and static solid electrolyte interphase (SEI) can be destroyed by the dynamic Li plating/stripping behavior on the Li anode surface, leading to side reactions and Li dendrites growth. Herein, we design a smart Li polyacrylic acid (LiPAA) SEI layer high elasticity to address the dynamic Li plating/stripping processes by self‐adapting interface regulation, which is demonstrated by in situ AFM. With the high binding ability and excellent stability of the LiPAA polymer, the smart SEI can significantly reduce the side reactions and improve battery safety markedly. Stable cycling of 700 h is achieved in the LiPAA‐Li/LiPAA‐Li symmetrical cell. The innovative strategy of self‐adapting SEI design is broadly applicable, providing opportunities for use in Li metal anodes
Stretching exercises: A flexible lithium polyacrylic acid (LiPAA) solid electrolyte interphase (SEI) layer which is highly stretchable is designed to address the dynamic volume changes during Li plating/stripping on the Li anode surface in Li ion batteries. The LiPAA polymer SEI can significantly reduce the side reactions and improve the safety performance. |
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| AbstractList | Lithium (Li) metal is a promising anode material for high‐energy density batteries. However, the unstable and static solid electrolyte interphase (SEI) can be destroyed by the dynamic Li plating/stripping behavior on the Li anode surface, leading to side reactions and Li dendrites growth. Herein, we design a smart Li polyacrylic acid (LiPAA) SEI layer high elasticity to address the dynamic Li plating/stripping processes by self‐adapting interface regulation, which is demonstrated by in situ AFM. With the high binding ability and excellent stability of the LiPAA polymer, the smart SEI can significantly reduce the side reactions and improve battery safety markedly. Stable cycling of 700 h is achieved in the LiPAA‐Li/LiPAA‐Li symmetrical cell. The innovative strategy of self‐adapting SEI design is broadly applicable, providing opportunities for use in Li metal anodes Lithium (Li) metal is a promising anode material for high-energy density batteries. However, the unstable and static solid electrolyte interphase (SEI) can be destroyed by the dynamic Li plating/stripping behavior on the Li anode surface, leading to side reactions and Li dendrites growth. Herein, we design a smart Li polyacrylic acid (LiPAA) SEI layer high elasticity to address the dynamic Li plating/stripping processes by self-adapting interface regulation, which is demonstrated by in situ AFM. With the high binding ability and excellent stability of the LiPAA polymer, the smart SEI can significantly reduce the side reactions and improve battery safety markedly. Stable cycling of 700 h is achieved in the LiPAA-Li/LiPAA-Li symmetrical cell. The innovative strategy of self-adapting SEI design is broadly applicable, providing opportunities for use in Li metal anodes.Lithium (Li) metal is a promising anode material for high-energy density batteries. However, the unstable and static solid electrolyte interphase (SEI) can be destroyed by the dynamic Li plating/stripping behavior on the Li anode surface, leading to side reactions and Li dendrites growth. Herein, we design a smart Li polyacrylic acid (LiPAA) SEI layer high elasticity to address the dynamic Li plating/stripping processes by self-adapting interface regulation, which is demonstrated by in situ AFM. With the high binding ability and excellent stability of the LiPAA polymer, the smart SEI can significantly reduce the side reactions and improve battery safety markedly. Stable cycling of 700 h is achieved in the LiPAA-Li/LiPAA-Li symmetrical cell. The innovative strategy of self-adapting SEI design is broadly applicable, providing opportunities for use in Li metal anodes. Lithium (Li) metal is a promising anode material for high‐energy density batteries. However, the unstable and static solid electrolyte interphase (SEI) can be destroyed by the dynamic Li plating/stripping behavior on the Li anode surface, leading to side reactions and Li dendrites growth. Herein, we design a smart Li polyacrylic acid (LiPAA) SEI layer high elasticity to address the dynamic Li plating/stripping processes by self‐adapting interface regulation, which is demonstrated by in situ AFM. With the high binding ability and excellent stability of the LiPAA polymer, the smart SEI can significantly reduce the side reactions and improve battery safety markedly. Stable cycling of 700 h is achieved in the LiPAA‐Li/LiPAA‐Li symmetrical cell. The innovative strategy of self‐adapting SEI design is broadly applicable, providing opportunities for use in Li metal anodes Stretching exercises: A flexible lithium polyacrylic acid (LiPAA) solid electrolyte interphase (SEI) layer which is highly stretchable is designed to address the dynamic volume changes during Li plating/stripping on the Li anode surface in Li ion batteries. The LiPAA polymer SEI can significantly reduce the side reactions and improve the safety performance. Lithium (Li) metal is a promising anode material for high-energy density batteries. However, the unstable and static solid electrolyte interphase (SEI) can be destroyed by the dynamic Li plating/stripping behavior on the Li anode surface, leading to side reactions and Li dendrites growth. Herein, we design a smart Li polyacrylic acid (LiPAA) SEI layer high elasticity to address the dynamic Li plating/stripping processes by self-adapting interface regulation, which is demonstrated by in situ AFM. With the high binding ability and excellent stability of the LiPAA polymer, the smart SEI can significantly reduce the side reactions and improve battery safety markedly. Stable cycling of 700 h is achieved in the LiPAA-Li/LiPAA-Li symmetrical cell. The innovative strategy of self-adapting SEI design is broadly applicable, providing opportunities for use in Li metal anodes. Lithium (Li) metal is a promising anode material for high-energy density batteries. However, the unstable and static solid electrolyte interphase (SEI) can be destroyed by the dynamic Li plating/stripping behavior on the Li anode surface, leading to side reactions and Li dendrites growth. Herein, we design a smart Li polyacrylic acid (LiPAA) SEI layer high elasticity to address the dynamic Li plating/stripping processes by self-adapting interface regulation, which is demonstrated by insitu AFM. With the high binding ability and excellent stability of the LiPAA polymer, the smart SEI can significantly reduce the side reactions and improve battery safety markedly. Stable cycling of 700h is achieved in the LiPAA-Li/LiPAA-Li symmetrical cell. The innovative strategy of self-adapting SEI design is broadly applicable, providing opportunities for use in Li metal anodes |
| Author | Li, Jin‐Yi Shi, Yang Wan, Li‐Jun Li, Nian‐Wu Yin, Ya‐Xia Li, Cong‐Ju Zeng, Xian‐Xiang Guo, Yu‐Guo Wen, Rui |
| Author_xml | – sequence: 1 givenname: Nian‐Wu surname: Li fullname: Li, Nian‐Wu organization: Chinese Academy of Sciences – sequence: 2 givenname: Yang surname: Shi fullname: Shi, Yang organization: University of Chinese Academy of Sciences – sequence: 3 givenname: Ya‐Xia surname: Yin fullname: Yin, Ya‐Xia organization: University of Chinese Academy of Sciences – sequence: 4 givenname: Xian‐Xiang surname: Zeng fullname: Zeng, Xian‐Xiang organization: University of Chinese Academy of Sciences – sequence: 5 givenname: Jin‐Yi surname: Li fullname: Li, Jin‐Yi organization: University of Chinese Academy of Sciences – sequence: 6 givenname: Cong‐Ju surname: Li fullname: Li, Cong‐Ju organization: Chinese Academy of Sciences – sequence: 7 givenname: Li‐Jun surname: Wan fullname: Wan, Li‐Jun organization: University of Chinese Academy of Sciences – sequence: 8 givenname: Rui surname: Wen fullname: Wen, Rui email: ruiwen@iccas.ac.cn organization: University of Chinese Academy of Sciences – sequence: 9 givenname: Yu‐Guo orcidid: 0000-0003-0322-8476 surname: Guo fullname: Guo, Yu‐Guo email: ygguo@iccas.ac.cn organization: University of Chinese Academy of Sciences |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/29239079$$D View this record in MEDLINE/PubMed |
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| Copyright | 2018 Wiley‐VCH Verlag GmbH & Co. KGaA, Weinheim 2018 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim. 2018 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim |
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| DOI | 10.1002/anie.201710806 |
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| Discipline | Chemistry |
| EISSN | 1521-3773 |
| Edition | International ed. in English |
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| Keywords | lithium dendrites lithium ion batteries solid electrolyte interphase in situ AFM lithium metal anodes |
| Language | English |
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| Snippet | Lithium (Li) metal is a promising anode material for high‐energy density batteries. However, the unstable and static solid electrolyte interphase (SEI) can be... Lithium (Li) metal is a promising anode material for high-energy density batteries. However, the unstable and static solid electrolyte interphase (SEI) can be... |
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| SubjectTerms | Anodes Batteries Dendrites Elasticity Electrode materials Electrolytes Flux density in situ AFM Interphase Lithium lithium dendrites lithium ion batteries lithium metal anodes Polyacrylic acid Polymers Product safety Side reactions solid electrolyte interphase Solid electrolytes Stripping |
| Title | A Flexible Solid Electrolyte Interphase Layer for Long‐Life Lithium Metal Anodes |
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