An Update on Formic Acid Dehydrogenation by Homogeneous Catalysis
Formic acid (FA) has been extensively studied as one of the most promising hydrogen energy carriers today. The catalytic decarboxylation of FA ideally leads to the formation of CO2 and H2 that can be applied in fuel cells. A large number of transition‐metal based homogeneous catalysts with high acti...
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| Published in | Chemistry, an Asian journal Vol. 15; no. 7; pp. 937 - 946 |
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| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
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01.04.2020
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| Abstract | Formic acid (FA) has been extensively studied as one of the most promising hydrogen energy carriers today. The catalytic decarboxylation of FA ideally leads to the formation of CO2 and H2 that can be applied in fuel cells. A large number of transition‐metal based homogeneous catalysts with high activity and selectivity have been reported for the selective FA dehydrogentaion. In this review, we discussed the recent development of C,N/N,N‐ligand and pincer ligand‐based homogeneous catalysts for the FA dehydrogenation reaction. Some representative catalysts are further evaluated by the CON/COF assessment (catalyst on‐cost number)/(catalyst on‐cost frequency). Conclusive remarks are provided with future challenges and opportunities.
Fueling the future: Formic acid (FA) has been extensively studied as one of the most promising hydrogen energy carriers today. In this review, we discussed the recent development of C,N/N,N‐ligand and pincer ligand‐based homogeneous catalysts for the FA dehydrogenation reaction. The CON/COF assessment (catalyst on‐cost number)/(catalyst on‐cost frequency) was highlighted with conclusive remarks on the future challenges and opportunities. |
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| AbstractList | Formic acid (FA) has been extensively studied as one of the most promising hydrogen energy carriers today. The catalytic decarboxylation of FA ideally leads to the formation of CO2 and H2 that can be applied in fuel cells. A large number of transition-metal based homogeneous catalysts with high activity and selectivity have been reported for the selective FA dehydrogentaion. In this review, we discussed the recent development of C,N/N,N-ligand and pincer ligand-based homogeneous catalysts for the FA dehydrogenation reaction. Some representative catalysts are further evaluated by the CON/COF assessment (catalyst on-cost number)/(catalyst on-cost frequency). Conclusive remarks are provided with future challenges and opportunities.Formic acid (FA) has been extensively studied as one of the most promising hydrogen energy carriers today. The catalytic decarboxylation of FA ideally leads to the formation of CO2 and H2 that can be applied in fuel cells. A large number of transition-metal based homogeneous catalysts with high activity and selectivity have been reported for the selective FA dehydrogentaion. In this review, we discussed the recent development of C,N/N,N-ligand and pincer ligand-based homogeneous catalysts for the FA dehydrogenation reaction. Some representative catalysts are further evaluated by the CON/COF assessment (catalyst on-cost number)/(catalyst on-cost frequency). Conclusive remarks are provided with future challenges and opportunities. Formic acid (FA) has been extensively studied as one of the most promising hydrogen energy carriers today. The catalytic decarboxylation of FA ideally leads to the formation of CO2 and H2 that can be applied in fuel cells. A large number of transition‐metal based homogeneous catalysts with high activity and selectivity have been reported for the selective FA dehydrogentaion. In this review, we discussed the recent development of C,N/N,N‐ligand and pincer ligand‐based homogeneous catalysts for the FA dehydrogenation reaction. Some representative catalysts are further evaluated by the CON/COF assessment (catalyst on‐cost number)/(catalyst on‐cost frequency). Conclusive remarks are provided with future challenges and opportunities. Formic acid (FA) has been extensively studied as one of the most promising hydrogen energy carriers today. The catalytic decarboxylation of FA ideally leads to the formation of CO 2 and H 2 that can be applied in fuel cells. A large number of transition‐metal based homogeneous catalysts with high activity and selectivity have been reported for the selective FA dehydrogentaion. In this review, we discussed the recent development of C,N/N,N‐ligand and pincer ligand‐based homogeneous catalysts for the FA dehydrogenation reaction. Some representative catalysts are further evaluated by the CON/COF assessment (catalyst on‐cost number)/(catalyst on‐cost frequency). Conclusive remarks are provided with future challenges and opportunities. Formic acid (FA) has been extensively studied as one of the most promising hydrogen energy carriers today. The catalytic decarboxylation of FA ideally leads to the formation of CO2 and H2 that can be applied in fuel cells. A large number of transition‐metal based homogeneous catalysts with high activity and selectivity have been reported for the selective FA dehydrogentaion. In this review, we discussed the recent development of C,N/N,N‐ligand and pincer ligand‐based homogeneous catalysts for the FA dehydrogenation reaction. Some representative catalysts are further evaluated by the CON/COF assessment (catalyst on‐cost number)/(catalyst on‐cost frequency). Conclusive remarks are provided with future challenges and opportunities. Fueling the future: Formic acid (FA) has been extensively studied as one of the most promising hydrogen energy carriers today. In this review, we discussed the recent development of C,N/N,N‐ligand and pincer ligand‐based homogeneous catalysts for the FA dehydrogenation reaction. The CON/COF assessment (catalyst on‐cost number)/(catalyst on‐cost frequency) was highlighted with conclusive remarks on the future challenges and opportunities. Formic acid (FA) has been extensively studied as one of the most promising hydrogen energy carriers today. The catalytic decarboxylation of FA ideally leads to the formation of CO and H that can be applied in fuel cells. A large number of transition-metal based homogeneous catalysts with high activity and selectivity have been reported for the selective FA dehydrogentaion. In this review, we discussed the recent development of C,N/N,N-ligand and pincer ligand-based homogeneous catalysts for the FA dehydrogenation reaction. Some representative catalysts are further evaluated by the CON/COF assessment (catalyst on-cost number)/(catalyst on-cost frequency). Conclusive remarks are provided with future challenges and opportunities. |
| Author | Pan, Yupeng Huang, Kuo‐Wei Guan, Chao Ajitha, Manjaly J. Zhang, Tonghuan |
| Author_xml | – sequence: 1 givenname: Chao orcidid: 0000-0002-9430-3488 surname: Guan fullname: Guan, Chao organization: King Abdullah University of Science and Technology – sequence: 2 givenname: Yupeng orcidid: 0000-0002-4471-3219 surname: Pan fullname: Pan, Yupeng organization: Southern University of Science and Technology (SUSTech) – sequence: 3 givenname: Tonghuan orcidid: 0000-0002-6636-0469 surname: Zhang fullname: Zhang, Tonghuan organization: Peking University Shenzhen Graduate School – sequence: 4 givenname: Manjaly J. orcidid: 0000-0002-0613-6270 surname: Ajitha fullname: Ajitha, Manjaly J. organization: King Abdullah University of Science and Technology – sequence: 5 givenname: Kuo‐Wei orcidid: 0000-0003-1900-2658 surname: Huang fullname: Huang, Kuo‐Wei email: hkw@kaust.edu.sa organization: King Abdullah University of Science and Technology |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/32030903$$D View this record in MEDLINE/PubMed |
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| Keywords | formic acid homogeneous catalysis hydrogen energy carrier |
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| Snippet | Formic acid (FA) has been extensively studied as one of the most promising hydrogen energy carriers today. The catalytic decarboxylation of FA ideally leads to... |
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| SubjectTerms | Catalysis Catalysts Chemistry Decarboxylation Dehydrogenation Formic acid Fuel cells homogeneous catalysis hydrogen energy carrier Hydrogen-based energy Ligands Selectivity |
| Title | An Update on Formic Acid Dehydrogenation by Homogeneous Catalysis |
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