Nano‐Ferroelectric for High Efficiency Overall Water Splitting under Ultrasonic Vibration
Piezocatalysis, converting mechanical vibration into chemical energy, has emerged as a promising candidate for water‐splitting technology. However, the efficiency of the hydrogen production is quite limited. We herein report well‐defined 10 nm BaTiO3 nanoparticles (NPs) characterized by a large elec...
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| Published in | Angewandte Chemie International Edition Vol. 58; no. 42; pp. 15076 - 15081 |
|---|---|
| Main Authors | , , , , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Germany
Wiley Subscription Services, Inc
14.10.2019
|
| Edition | International ed. in English |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Piezocatalysis, converting mechanical vibration into chemical energy, has emerged as a promising candidate for water‐splitting technology. However, the efficiency of the hydrogen production is quite limited. We herein report well‐defined 10 nm BaTiO3 nanoparticles (NPs) characterized by a large electro‐mechanical coefficient which induces a high piezoelectric effect. Atomic‐resolution high angle annular dark field scanning transmission electron microscopy (HAADF‐STEM) and scanning probe microscopy (SPM) suggests that piezoelectric BaTiO3 NPs display a coexistence of multiple phases with low energy barriers and polarization anisotropy which results in a high electro‐mechanical coefficient. Landau free energy modeling also confirms that the greatly reduced polarization anisotropy facilitates polarization rotation. Employing the high piezoelectric properties of BaTiO3 NPs, we demonstrate an overall water‐splitting process with the highest hydrogen production efficiency hitherto reported, with a H2 production rate of 655 μmol g−1 h−1, which could rival excellent photocatalysis system. This study highlights the potential of piezoelectric catalysis for overall water splitting.
The oscillatory polarization state of a nano‐ferroelectric with the coexistence of three ferroelectric phases (T+O+R) leads to an imbalanced charge state on the sample surface and creates an alternating cascade of a space charge release and attraction under ultrasonic vibration, thus generating hydrogen and oxygen via direct water decomposition. |
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| AbstractList | Piezocatalysis, converting mechanical vibration into chemical energy, has emerged as a promising candidate for water-splitting technology. However, the efficiency of the hydrogen production is quite limited. We herein report well-defined 10 nm BaTiO
nanoparticles (NPs) characterized by a large electro-mechanical coefficient which induces a high piezoelectric effect. Atomic-resolution high angle annular dark field scanning transmission electron microscopy (HAADF-STEM) and scanning probe microscopy (SPM) suggests that piezoelectric BaTiO
NPs display a coexistence of multiple phases with low energy barriers and polarization anisotropy which results in a high electro-mechanical coefficient. Landau free energy modeling also confirms that the greatly reduced polarization anisotropy facilitates polarization rotation. Employing the high piezoelectric properties of BaTiO
NPs, we demonstrate an overall water-splitting process with the highest hydrogen production efficiency hitherto reported, with a H
production rate of 655 μmol g
h
, which could rival excellent photocatalysis system. This study highlights the potential of piezoelectric catalysis for overall water splitting. Piezocatalysis, converting mechanical vibration into chemical energy, has emerged as a promising candidate for water‐splitting technology. However, the efficiency of the hydrogen production is quite limited. We herein report well‐defined 10 nm BaTiO3 nanoparticles (NPs) characterized by a large electro‐mechanical coefficient which induces a high piezoelectric effect. Atomic‐resolution high angle annular dark field scanning transmission electron microscopy (HAADF‐STEM) and scanning probe microscopy (SPM) suggests that piezoelectric BaTiO3 NPs display a coexistence of multiple phases with low energy barriers and polarization anisotropy which results in a high electro‐mechanical coefficient. Landau free energy modeling also confirms that the greatly reduced polarization anisotropy facilitates polarization rotation. Employing the high piezoelectric properties of BaTiO3 NPs, we demonstrate an overall water‐splitting process with the highest hydrogen production efficiency hitherto reported, with a H2 production rate of 655 μmol g−1 h−1, which could rival excellent photocatalysis system. This study highlights the potential of piezoelectric catalysis for overall water splitting. Piezocatalysis, converting mechanical vibration into chemical energy, has emerged as a promising candidate for water-splitting technology. However, the efficiency of the hydrogen production is quite limited. We herein report well-defined 10 nm BaTiO3 nanoparticles (NPs) characterized by a large electro-mechanical coefficient which induces a high piezoelectric effect. Atomic-resolution high angle annular dark field scanning transmission electron microscopy (HAADF-STEM) and scanning probe microscopy (SPM) suggests that piezoelectric BaTiO3 NPs display a coexistence of multiple phases with low energy barriers and polarization anisotropy which results in a high electro-mechanical coefficient. Landau free energy modeling also confirms that the greatly reduced polarization anisotropy facilitates polarization rotation. Employing the high piezoelectric properties of BaTiO3 NPs, we demonstrate an overall water-splitting process with the highest hydrogen production efficiency hitherto reported, with a H2 production rate of 655 μmol g-1 h-1 , which could rival excellent photocatalysis system. This study highlights the potential of piezoelectric catalysis for overall water splitting.Piezocatalysis, converting mechanical vibration into chemical energy, has emerged as a promising candidate for water-splitting technology. However, the efficiency of the hydrogen production is quite limited. We herein report well-defined 10 nm BaTiO3 nanoparticles (NPs) characterized by a large electro-mechanical coefficient which induces a high piezoelectric effect. Atomic-resolution high angle annular dark field scanning transmission electron microscopy (HAADF-STEM) and scanning probe microscopy (SPM) suggests that piezoelectric BaTiO3 NPs display a coexistence of multiple phases with low energy barriers and polarization anisotropy which results in a high electro-mechanical coefficient. Landau free energy modeling also confirms that the greatly reduced polarization anisotropy facilitates polarization rotation. Employing the high piezoelectric properties of BaTiO3 NPs, we demonstrate an overall water-splitting process with the highest hydrogen production efficiency hitherto reported, with a H2 production rate of 655 μmol g-1 h-1 , which could rival excellent photocatalysis system. This study highlights the potential of piezoelectric catalysis for overall water splitting. Piezocatalysis, converting mechanical vibration into chemical energy, has emerged as a promising candidate for water‐splitting technology. However, the efficiency of the hydrogen production is quite limited. We herein report well‐defined 10 nm BaTiO3 nanoparticles (NPs) characterized by a large electro‐mechanical coefficient which induces a high piezoelectric effect. Atomic‐resolution high angle annular dark field scanning transmission electron microscopy (HAADF‐STEM) and scanning probe microscopy (SPM) suggests that piezoelectric BaTiO3 NPs display a coexistence of multiple phases with low energy barriers and polarization anisotropy which results in a high electro‐mechanical coefficient. Landau free energy modeling also confirms that the greatly reduced polarization anisotropy facilitates polarization rotation. Employing the high piezoelectric properties of BaTiO3 NPs, we demonstrate an overall water‐splitting process with the highest hydrogen production efficiency hitherto reported, with a H2 production rate of 655 μmol g−1 h−1, which could rival excellent photocatalysis system. This study highlights the potential of piezoelectric catalysis for overall water splitting. The oscillatory polarization state of a nano‐ferroelectric with the coexistence of three ferroelectric phases (T+O+R) leads to an imbalanced charge state on the sample surface and creates an alternating cascade of a space charge release and attraction under ultrasonic vibration, thus generating hydrogen and oxygen via direct water decomposition. Piezocatalysis, converting mechanical vibration into chemical energy, has emerged as a promising candidate for water‐splitting technology. However, the efficiency of the hydrogen production is quite limited. We herein report well‐defined 10 nm BaTiO 3 nanoparticles (NPs) characterized by a large electro‐mechanical coefficient which induces a high piezoelectric effect. Atomic‐resolution high angle annular dark field scanning transmission electron microscopy (HAADF‐STEM) and scanning probe microscopy (SPM) suggests that piezoelectric BaTiO 3 NPs display a coexistence of multiple phases with low energy barriers and polarization anisotropy which results in a high electro‐mechanical coefficient. Landau free energy modeling also confirms that the greatly reduced polarization anisotropy facilitates polarization rotation. Employing the high piezoelectric properties of BaTiO 3 NPs, we demonstrate an overall water‐splitting process with the highest hydrogen production efficiency hitherto reported, with a H 2 production rate of 655 μmol g −1 h −1 , which could rival excellent photocatalysis system. This study highlights the potential of piezoelectric catalysis for overall water splitting. |
| Author | Su, Ran Chen, Xuemin Yang, Yaodong Li, Fa‐tang Wang, Zhipeng Hu, Xinghao Zhang, Dawei Zhu, Lina Pennycook, Stephen J. Hsain, H. Alex Wu, Ming Wang, Xiaojing Lou, Xiaojie Yang, Yong |
| Author_xml | – sequence: 1 givenname: Ran surname: Su fullname: Su, Ran organization: Hebei University of Science and Technology – sequence: 2 givenname: H. Alex surname: Hsain fullname: Hsain, H. Alex organization: North Carolina State University – sequence: 3 givenname: Ming surname: Wu fullname: Wu, Ming organization: Xi'an Jiaotong University – sequence: 4 givenname: Dawei surname: Zhang fullname: Zhang, Dawei organization: University of New South Wales – sequence: 5 givenname: Xinghao surname: Hu fullname: Hu, Xinghao organization: Jiangsu University – sequence: 6 givenname: Zhipeng surname: Wang fullname: Wang, Zhipeng organization: Sungkyunkwan University – sequence: 7 givenname: Xiaojing surname: Wang fullname: Wang, Xiaojing organization: Hebei University of Science and Technology – sequence: 8 givenname: Fa‐tang orcidid: 0000-0002-8777-090X surname: Li fullname: Li, Fa‐tang email: lifatang@126.com organization: Hebei University of Science and Technology – sequence: 9 givenname: Xuemin surname: Chen fullname: Chen, Xuemin organization: Hebei University of Science and Technology – sequence: 10 givenname: Lina surname: Zhu fullname: Zhu, Lina organization: Hebei University of Science and Technology – sequence: 11 givenname: Yong surname: Yang fullname: Yang, Yong organization: Northwestern Polytechnical University – sequence: 12 givenname: Yaodong surname: Yang fullname: Yang, Yaodong organization: Xi'an Jiaotong University – sequence: 13 givenname: Xiaojie surname: Lou fullname: Lou, Xiaojie organization: Xi'an Jiaotong University – sequence: 14 givenname: Stephen J. surname: Pennycook fullname: Pennycook, Stephen J. organization: National University of Singapore |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/31404487$$D View this record in MEDLINE/PubMed |
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| Copyright | 2019 Wiley‐VCH Verlag GmbH & Co. KGaA, Weinheim 2019 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim. |
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| Snippet | Piezocatalysis, converting mechanical vibration into chemical energy, has emerged as a promising candidate for water‐splitting technology. However, the... Piezocatalysis, converting mechanical vibration into chemical energy, has emerged as a promising candidate for water-splitting technology. However, the... |
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| SubjectTerms | Anisotropy Barium titanates Catalysis Chemical energy Coexistence Efficiency ferroelectric Ferroelectric materials Ferroelectricity Free energy Hydrogen production Microscopy Nanoparticles Organic chemistry phase coexistence piezocatalysis piezoelectric effect Piezoelectricity Polarization Scanning probe microscopy Scanning transmission electron microscopy Splitting Transmission electron microscopy Ultrasonic vibration Water splitting |
| Title | Nano‐Ferroelectric for High Efficiency Overall Water Splitting under Ultrasonic Vibration |
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