A New Dimension for Coordination Polymers and Metal–Organic Frameworks: Towards Functional Glasses and Liquids

There are two categories of coordination polymers (CPs): inorganic CPs (i‐CPs) and organic ligand bridged CPs (o‐CPs). Based on the successful crystal engineering of CPs, we here propose noncrystalline states and functionalities as a new research direction for CPs. Control over the liquid or glassy...

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Published inAngewandte Chemie International Edition Vol. 59; no. 17; pp. 6652 - 6664
Main Authors Horike, Satoshi, Nagarkar, Sanjog S., Ogawa, Tomohiro, Kitagawa, Susumu
Format Journal Article
LanguageEnglish
Published Germany Wiley Subscription Services, Inc 20.04.2020
EditionInternational ed. in English
Subjects
Computer applications
Coordination polymers
Feasibility studies
Glass
Ionic liquids
Ions
Ligands
Material properties
melting
Metal ions
Metal-organic frameworks
metal–organic frameworks (MOFs)
phase transition
Phase transitions
Polymers
Porosity
coordination polymers
glass
melting
phase transition
metal-organic frameworks (MOFs)
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Abstract There are two categories of coordination polymers (CPs): inorganic CPs (i‐CPs) and organic ligand bridged CPs (o‐CPs). Based on the successful crystal engineering of CPs, we here propose noncrystalline states and functionalities as a new research direction for CPs. Control over the liquid or glassy states in materials is essential to obtain specific properties and functions. Several studies suggest the feasibility of obtaining liquid/glassy states in o‐CPs by design principles. The combination of metal ions and organic bridging ligands, together with the liquid/glass phase transformation, offer the possibility to transform o‐CPs into ionic liquids and other ionic soft materials. Synchrotron measurements and computational approaches contribute to elucidating the structures and dynamics of the liquid/glassy states of o‐CPs. This offers the opportunity to tune the porosity, conductivity, transparency, and other material properties. The unique energy landscape of liquid/glass o‐CPs offers opportunities for properties and functions that are complementary to those of the crystalline state. Heart of glass: The liquid/glass states of coordination polymers (CPs) and metal‐organic frameworks (MOFs) constitute a new class of amorphous materials and are related to ionic liquids and other ionic soft materials. The unique energy landscape and dynamics of liquid/glass CPs/MOFs with coordination networks offer additional opportunities for properties and functions that are complementary to those of the crystalline state.
AbstractList There are two categories of coordination polymers (CPs): inorganic CPs (i-CPs) and organic ligand bridged CPs (o-CPs). Based on the successful crystal engineering of CPs, we here propose noncrystalline states and functionalities as a new research direction for CPs. Control over the liquid or glassy states in materials is essential to obtain specific properties and functions. Several studies suggest the feasibility of obtaining liquid/glassy states in o-CPs by design principles. The combination of metal ions and organic bridging ligands, together with the liquid/glass phase transformation, offer the possibility to transform o-CPs into ionic liquids and other ionic soft materials. Synchrotron measurements and computational approaches contribute to elucidating the structures and dynamics of the liquid/glassy states of o-CPs. This offers the opportunity to tune the porosity, conductivity, transparency, and other material properties. The unique energy landscape of liquid/glass o-CPs offers opportunities for properties and functions that are complementary to those of the crystalline state.There are two categories of coordination polymers (CPs): inorganic CPs (i-CPs) and organic ligand bridged CPs (o-CPs). Based on the successful crystal engineering of CPs, we here propose noncrystalline states and functionalities as a new research direction for CPs. Control over the liquid or glassy states in materials is essential to obtain specific properties and functions. Several studies suggest the feasibility of obtaining liquid/glassy states in o-CPs by design principles. The combination of metal ions and organic bridging ligands, together with the liquid/glass phase transformation, offer the possibility to transform o-CPs into ionic liquids and other ionic soft materials. Synchrotron measurements and computational approaches contribute to elucidating the structures and dynamics of the liquid/glassy states of o-CPs. This offers the opportunity to tune the porosity, conductivity, transparency, and other material properties. The unique energy landscape of liquid/glass o-CPs offers opportunities for properties and functions that are complementary to those of the crystalline state.
There are two categories of coordination polymers (CPs): inorganic CPs (i‐CPs) and organic ligand bridged CPs (o‐CPs). Based on the successful crystal engineering of CPs, we here propose noncrystalline states and functionalities as a new research direction for CPs. Control over the liquid or glassy states in materials is essential to obtain specific properties and functions. Several studies suggest the feasibility of obtaining liquid/glassy states in o‐CPs by design principles. The combination of metal ions and organic bridging ligands, together with the liquid/glass phase transformation, offer the possibility to transform o‐CPs into ionic liquids and other ionic soft materials. Synchrotron measurements and computational approaches contribute to elucidating the structures and dynamics of the liquid/glassy states of o‐CPs. This offers the opportunity to tune the porosity, conductivity, transparency, and other material properties. The unique energy landscape of liquid/glass o‐CPs offers opportunities for properties and functions that are complementary to those of the crystalline state.
There are two categories of coordination polymers (CPs): inorganic CPs (i‐CPs) and organic ligand bridged CPs (o‐CPs). Based on the successful crystal engineering of CPs, we here propose noncrystalline states and functionalities as a new research direction for CPs. Control over the liquid or glassy states in materials is essential to obtain specific properties and functions. Several studies suggest the feasibility of obtaining liquid/glassy states in o‐CPs by design principles. The combination of metal ions and organic bridging ligands, together with the liquid/glass phase transformation, offer the possibility to transform o‐CPs into ionic liquids and other ionic soft materials. Synchrotron measurements and computational approaches contribute to elucidating the structures and dynamics of the liquid/glassy states of o‐CPs. This offers the opportunity to tune the porosity, conductivity, transparency, and other material properties. The unique energy landscape of liquid/glass o‐CPs offers opportunities for properties and functions that are complementary to those of the crystalline state. Heart of glass: The liquid/glass states of coordination polymers (CPs) and metal‐organic frameworks (MOFs) constitute a new class of amorphous materials and are related to ionic liquids and other ionic soft materials. The unique energy landscape and dynamics of liquid/glass CPs/MOFs with coordination networks offer additional opportunities for properties and functions that are complementary to those of the crystalline state.
Author Kitagawa, Susumu
Ogawa, Tomohiro
Horike, Satoshi
Nagarkar, Sanjog S.
Author_xml – sequence: 1
  givenname: Satoshi
  orcidid: 0000-0001-8530-6364
  surname: Horike
  fullname: Horike, Satoshi
  email: horike@icems.kyoto-u.ac.jp
  organization: Vidyasirimedhi Institute of Science and Technology
– sequence: 2
  givenname: Sanjog S.
  orcidid: 0000-0001-5487-6225
  surname: Nagarkar
  fullname: Nagarkar, Sanjog S.
  organization: National Institute of Advanced Industrial Science and Technology (AIST), Yoshida-Honmachi, Sakyo-ku
– sequence: 3
  givenname: Tomohiro
  orcidid: 0000-0001-7298-0149
  surname: Ogawa
  fullname: Ogawa, Tomohiro
  organization: Kyoto University, Yoshida-Honmachi, Sakyo-ku
– sequence: 4
  givenname: Susumu
  orcidid: 0000-0001-6956-9543
  surname: Kitagawa
  fullname: Kitagawa, Susumu
  email: kitagawa@icems.kyoto-u.ac.jp
  organization: Kyoto University, Yoshida-Honmachi, Sakyo-ku
BackLink https://www.ncbi.nlm.nih.gov/pubmed/31631497$$D View this record in MEDLINE/PubMed
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Copyright 2019 Wiley‐VCH Verlag GmbH & Co. KGaA, Weinheim
2019 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim.
2020 Wiley‐VCH Verlag GmbH & Co. KGaA, Weinheim
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IsPeerReviewed true
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Issue 17
Keywords coordination polymers
glass
melting
phase transition
metal-organic frameworks (MOFs)
Language English
License 2019 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim.
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Snippet There are two categories of coordination polymers (CPs): inorganic CPs (i‐CPs) and organic ligand bridged CPs (o‐CPs). Based on the successful crystal...
There are two categories of coordination polymers (CPs): inorganic CPs (i-CPs) and organic ligand bridged CPs (o-CPs). Based on the successful crystal...
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SubjectTerms Computer applications
Coordination polymers
Feasibility studies
Glass
Ionic liquids
Ions
Ligands
Material properties
melting
Metal ions
Metal-organic frameworks
metal–organic frameworks (MOFs)
phase transition
Phase transitions
Polymers
Porosity
Title A New Dimension for Coordination Polymers and Metal–Organic Frameworks: Towards Functional Glasses and Liquids
URI https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fanie.201911384
https://www.ncbi.nlm.nih.gov/pubmed/31631497
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https://www.proquest.com/docview/2307399504
Volume 59
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