Coupling of Solar Energy and Thermal Energy for Carbon Dioxide Reduction: Status and Prospects
Enormous efforts have been devoted to the reduction of carbon dioxide (CO2) by utilizing various driving forces, such as heat, electricity, and radiation. However, the efficient reduction of CO2 is still challenging because of sluggish kinetics. Recent pioneering studies from several groups, includi...
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| Published in | Angewandte Chemie International Edition Vol. 59; no. 21; pp. 8016 - 8035 |
|---|---|
| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
| Published |
Germany
Wiley Subscription Services, Inc
18.05.2020
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| Edition | International ed. in English |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Enormous efforts have been devoted to the reduction of carbon dioxide (CO2) by utilizing various driving forces, such as heat, electricity, and radiation. However, the efficient reduction of CO2 is still challenging because of sluggish kinetics. Recent pioneering studies from several groups, including us, have demonstrated that the coupling of solar energy and thermal energy offers a novel and promising strategy to promote the activity and/or manipulate selectivity in CO2 reduction. Herein, we clarify the definition and principles of coupling solar energy and thermal energy, and comprehensively review the status and prospects of CO2 reduction by coupling solar energy and thermal energy. Catalyst design, reactor configuration, photo‐mediated activity/selectivity, and mechanism studies in photo‐thermo CO2 reduction will be emphasized. The aim of this Review is to promote understanding towards CO2 activation and provide guidelines for the design of new catalysts for the efficient reduction of CO2.
A bundle of energy: The coupling of solar energy and thermal energy is a promising strategy to mediate the activity and/or selectivity of CO2 reduction. The status and prospects of this topic are reviewed, with the aim of providing guidelines for the design of new catalysts. |
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| AbstractList | Enormous efforts have been devoted to the reduction of carbon dioxide (CO
) by utilizing various driving forces, such as heat, electricity, and radiation. However, the efficient reduction of CO
is still challenging because of sluggish kinetics. Recent pioneering studies from several groups, including us, have demonstrated that the coupling of solar energy and thermal energy offers a novel and promising strategy to promote the activity and/or manipulate selectivity in CO
reduction. Herein, we clarify the definition and principles of coupling solar energy and thermal energy, and comprehensively review the status and prospects of CO
reduction by coupling solar energy and thermal energy. Catalyst design, reactor configuration, photo-mediated activity/selectivity, and mechanism studies in photo-thermo CO
reduction will be emphasized. The aim of this Review is to promote understanding towards CO
activation and provide guidelines for the design of new catalysts for the efficient reduction of CO
. Enormous efforts have been devoted to the reduction of carbon dioxide (CO2) by utilizing various driving forces, such as heat, electricity, and radiation. However, the efficient reduction of CO2 is still challenging because of sluggish kinetics. Recent pioneering studies from several groups, including us, have demonstrated that the coupling of solar energy and thermal energy offers a novel and promising strategy to promote the activity and/or manipulate selectivity in CO2 reduction. Herein, we clarify the definition and principles of coupling solar energy and thermal energy, and comprehensively review the status and prospects of CO2 reduction by coupling solar energy and thermal energy. Catalyst design, reactor configuration, photo‐mediated activity/selectivity, and mechanism studies in photo‐thermo CO2 reduction will be emphasized. The aim of this Review is to promote understanding towards CO2 activation and provide guidelines for the design of new catalysts for the efficient reduction of CO2. A bundle of energy: The coupling of solar energy and thermal energy is a promising strategy to mediate the activity and/or selectivity of CO2 reduction. The status and prospects of this topic are reviewed, with the aim of providing guidelines for the design of new catalysts. Enormous efforts have been devoted to the reduction of carbon dioxide (CO2) by utilizing various driving forces, such as heat, electricity, and radiation. However, the efficient reduction of CO2 is still challenging because of sluggish kinetics. Recent pioneering studies from several groups, including us, have demonstrated that the coupling of solar energy and thermal energy offers a novel and promising strategy to promote the activity and/or manipulate selectivity in CO2 reduction. Herein, we clarify the definition and principles of coupling solar energy and thermal energy, and comprehensively review the status and prospects of CO2 reduction by coupling solar energy and thermal energy. Catalyst design, reactor configuration, photo‐mediated activity/selectivity, and mechanism studies in photo‐thermo CO2 reduction will be emphasized. The aim of this Review is to promote understanding towards CO2 activation and provide guidelines for the design of new catalysts for the efficient reduction of CO2. Enormous efforts have been devoted to the reduction of carbon dioxide (CO 2 ) by utilizing various driving forces, such as heat, electricity, and radiation. However, the efficient reduction of CO 2 is still challenging because of sluggish kinetics. Recent pioneering studies from several groups, including us, have demonstrated that the coupling of solar energy and thermal energy offers a novel and promising strategy to promote the activity and/or manipulate selectivity in CO 2 reduction. Herein, we clarify the definition and principles of coupling solar energy and thermal energy, and comprehensively review the status and prospects of CO 2 reduction by coupling solar energy and thermal energy. Catalyst design, reactor configuration, photo‐mediated activity/selectivity, and mechanism studies in photo‐thermo CO 2 reduction will be emphasized. The aim of this Review is to promote understanding towards CO 2 activation and provide guidelines for the design of new catalysts for the efficient reduction of CO 2 . Enormous efforts have been devoted to the reduction of carbon dioxide (CO2 ) by utilizing various driving forces, such as heat, electricity, and radiation. However, the efficient reduction of CO2 is still challenging because of sluggish kinetics. Recent pioneering studies from several groups, including us, have demonstrated that the coupling of solar energy and thermal energy offers a novel and promising strategy to promote the activity and/or manipulate selectivity in CO2 reduction. Herein, we clarify the definition and principles of coupling solar energy and thermal energy, and comprehensively review the status and prospects of CO2 reduction by coupling solar energy and thermal energy. Catalyst design, reactor configuration, photo-mediated activity/selectivity, and mechanism studies in photo-thermo CO2 reduction will be emphasized. The aim of this Review is to promote understanding towards CO2 activation and provide guidelines for the design of new catalysts for the efficient reduction of CO2 .Enormous efforts have been devoted to the reduction of carbon dioxide (CO2 ) by utilizing various driving forces, such as heat, electricity, and radiation. However, the efficient reduction of CO2 is still challenging because of sluggish kinetics. Recent pioneering studies from several groups, including us, have demonstrated that the coupling of solar energy and thermal energy offers a novel and promising strategy to promote the activity and/or manipulate selectivity in CO2 reduction. Herein, we clarify the definition and principles of coupling solar energy and thermal energy, and comprehensively review the status and prospects of CO2 reduction by coupling solar energy and thermal energy. Catalyst design, reactor configuration, photo-mediated activity/selectivity, and mechanism studies in photo-thermo CO2 reduction will be emphasized. The aim of this Review is to promote understanding towards CO2 activation and provide guidelines for the design of new catalysts for the efficient reduction of CO2 . |
| Author | Ye, Jinhua Wang, Zhou‐jun Song, Hui Liu, Huimin |
| Author_xml | – sequence: 1 givenname: Zhou‐jun orcidid: 0000-0002-9196-8062 surname: Wang fullname: Wang, Zhou‐jun organization: National Institute for Materials Science (NIMS) – sequence: 2 givenname: Hui orcidid: 0000-0001-6424-7959 surname: Song fullname: Song, Hui organization: Hokkaido University – sequence: 3 givenname: Huimin surname: Liu fullname: Liu, Huimin organization: The University of Sydney – sequence: 4 givenname: Jinhua orcidid: 0000-0002-8105-8903 surname: Ye fullname: Ye, Jinhua email: Jinhua.YE@nims.go.jp organization: Collaborative Innovation Center of Chemical Science and Engineering (Tianjin) |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/31309678$$D View this record in MEDLINE/PubMed |
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| Snippet | Enormous efforts have been devoted to the reduction of carbon dioxide (CO2) by utilizing various driving forces, such as heat, electricity, and radiation.... Enormous efforts have been devoted to the reduction of carbon dioxide (CO 2 ) by utilizing various driving forces, such as heat, electricity, and radiation.... Enormous efforts have been devoted to the reduction of carbon dioxide (CO ) by utilizing various driving forces, such as heat, electricity, and radiation.... Enormous efforts have been devoted to the reduction of carbon dioxide (CO2 ) by utilizing various driving forces, such as heat, electricity, and radiation.... |
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| SubjectTerms | Carbon dioxide Catalysts Configuration management Coupling heterogeneous catalysis nanostructures photocatalysis Reaction kinetics Reduction Selectivity Solar energy Thermal energy |
| Title | Coupling of Solar Energy and Thermal Energy for Carbon Dioxide Reduction: Status and Prospects |
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