Columnar Lithium Metal Anodes
The rechargeable lithium metal anode is of utmost importance for high‐energy‐density batteries. Regulating the deposition/dissolution characteristics of Li metal is critical in both fundamental researches and practical applications. In contrast to gray Li deposits featured with dendritic and mossy m...
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| Published in | Angewandte Chemie International Edition Vol. 56; no. 45; pp. 14207 - 14211 |
|---|---|
| Main Authors | , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Germany
Wiley Subscription Services, Inc
06.11.2017
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| Edition | International ed. in English |
| Subjects | |
| Online Access | Get full text |
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| Abstract | The rechargeable lithium metal anode is of utmost importance for high‐energy‐density batteries. Regulating the deposition/dissolution characteristics of Li metal is critical in both fundamental researches and practical applications. In contrast to gray Li deposits featured with dendritic and mossy morphologies, columnar and uniform Li is herein plated on lithium‐fluoride (LiF)‐protected copper (Cu) current collectors. The electrochemical properties strongly depended on the microscale morphologies of deposited Li, which were further embodied as macroscale colors. The as‐obtained ultrathin and columnar Li anodes contributed to stable cycling in working batteries with a dendrite‐free feature. This work deepens the fundamental understanding of the role of LiF in the nucleation/growth of Li and provides emerging approaches to stabilize rechargeable Li metal anodes.
Columnar Li deposition is obtained on uniform and dense nucleation sites formed by regulation of LiF. The obvious relation between microstructure and macroscale color provides an emerging descriptor to judge the uniformity of the deposited Li. Ultrathin and stable Li anodes are further developed to meet the intensive demand for high‐energy‐density batteries. |
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| AbstractList | The rechargeable lithium metal anode is of utmost importance for high-energy-density batteries. Regulating the deposition/dissolution characteristics of Li metal is critical in both fundamental researches and practical applications. In contrast to gray Li deposits featured with dendritic and mossy morphologies, columnar and uniform Li is herein plated on lithium-fluoride (LiF)-protected copper (Cu) current collectors. The electrochemical properties strongly depended on the microscale morphologies of deposited Li, which were further embodied as macroscale colors. The as-obtained ultrathin and columnar Li anodes contributed to stable cycling in working batteries with a dendrite-free feature. This work deepens the fundamental understanding of the role of LiF in the nucleation/growth of Li and provides emerging approaches to stabilize rechargeable Li metal anodes. The rechargeable lithium metal anode is of utmost importance for high‐energy‐density batteries. Regulating the deposition/dissolution characteristics of Li metal is critical in both fundamental researches and practical applications. In contrast to gray Li deposits featured with dendritic and mossy morphologies, columnar and uniform Li is herein plated on lithium‐fluoride (LiF)‐protected copper (Cu) current collectors. The electrochemical properties strongly depended on the microscale morphologies of deposited Li, which were further embodied as macroscale colors. The as‐obtained ultrathin and columnar Li anodes contributed to stable cycling in working batteries with a dendrite‐free feature. This work deepens the fundamental understanding of the role of LiF in the nucleation/growth of Li and provides emerging approaches to stabilize rechargeable Li metal anodes. Columnar Li deposition is obtained on uniform and dense nucleation sites formed by regulation of LiF. The obvious relation between microstructure and macroscale color provides an emerging descriptor to judge the uniformity of the deposited Li. Ultrathin and stable Li anodes are further developed to meet the intensive demand for high‐energy‐density batteries. The rechargeable lithium metal anode is of utmost importance for high-energy-density batteries. Regulating the deposition/dissolution characteristics of Li metal is critical in both fundamental researches and practical applications. In contrast to gray Li deposits featured with dendritic and mossy morphologies, columnar and uniform Li is herein plated on lithium-fluoride (LiF)-protected copper (Cu) current collectors. The electrochemical properties strongly depended on the microscale morphologies of deposited Li, which were further embodied as macroscale colors. The as-obtained ultrathin and columnar Li anodes contributed to stable cycling in working batteries with a dendrite-free feature. This work deepens the fundamental understanding of the role of LiF in the nucleation/growth of Li and provides emerging approaches to stabilize rechargeable Li metal anodes.The rechargeable lithium metal anode is of utmost importance for high-energy-density batteries. Regulating the deposition/dissolution characteristics of Li metal is critical in both fundamental researches and practical applications. In contrast to gray Li deposits featured with dendritic and mossy morphologies, columnar and uniform Li is herein plated on lithium-fluoride (LiF)-protected copper (Cu) current collectors. The electrochemical properties strongly depended on the microscale morphologies of deposited Li, which were further embodied as macroscale colors. The as-obtained ultrathin and columnar Li anodes contributed to stable cycling in working batteries with a dendrite-free feature. This work deepens the fundamental understanding of the role of LiF in the nucleation/growth of Li and provides emerging approaches to stabilize rechargeable Li metal anodes. |
| Author | Huang, Jia‐Qi Xu, Rui Zhang, Qiang Cheng, Xin‐Bing Zhang, Rui Peng, Hong‐Jie Zhang, Xue‐Qiang Chen, Xiang |
| Author_xml | – sequence: 1 givenname: Xue‐Qiang surname: Zhang fullname: Zhang, Xue‐Qiang organization: Tsinghua University – sequence: 2 givenname: Xiang surname: Chen fullname: Chen, Xiang organization: Tsinghua University – sequence: 3 givenname: Rui surname: Xu fullname: Xu, Rui organization: Beijing Institute of Technology – sequence: 4 givenname: Xin‐Bing surname: Cheng fullname: Cheng, Xin‐Bing organization: Tsinghua University – sequence: 5 givenname: Hong‐Jie surname: Peng fullname: Peng, Hong‐Jie organization: Tsinghua University – sequence: 6 givenname: Rui surname: Zhang fullname: Zhang, Rui organization: Tsinghua University – sequence: 7 givenname: Jia‐Qi surname: Huang fullname: Huang, Jia‐Qi organization: Beijing Institute of Technology – sequence: 8 givenname: Qiang orcidid: 0000-0002-3929-1541 surname: Zhang fullname: Zhang, Qiang email: zhang-qiang@mails.tsinghua.edu.cn organization: Tsinghua University |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/28868626$$D View this record in MEDLINE/PubMed |
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| Keywords | dendrites lithium fluoride nucleation lithium deposition electrochemistry |
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| Snippet | The rechargeable lithium metal anode is of utmost importance for high‐energy‐density batteries. Regulating the deposition/dissolution characteristics of Li... The rechargeable lithium metal anode is of utmost importance for high-energy-density batteries. Regulating the deposition/dissolution characteristics of Li... |
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| SubjectTerms | Accumulators Anodes Anodic dissolution Copper dendrites Dendritic structure Dissolution Electrochemical analysis Electrochemistry Fluorides Lithium lithium deposition lithium fluoride Metals nucleation Rechargeable batteries |
| Title | Columnar Lithium Metal Anodes |
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